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Register a new userDynamical structure factors in the nematic phase of frustrated ferromagnetic spin chains
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Frustrated spin systems can show phases with spontaneous breaking of spin-rotational symmetry without the formation of local magnetic order. We study the dynamic response of the spin-nematic phase of one-dimensional spin-1/2 systems, characterized by slow large-distance decay of quadrupolar correlations, by numerically computing one-spin and two-spin dynamical structure factors at zero temperature using time-dependent density matrix renormalization group methods. We interpret the results in terms of an effective theory of gapped magnon excitations interacting with a quasi-condensate of bound magnon pairs. This employs an extension of the well-known Tomonaga-Luttinger liquid theory which includes the magnon states as a mobile impurity. A good qualitative understanding of the characteristic thresholds and their intensity in the structure factors is obtained this way. Our results are useful in the interpretation of inelastic neutron scattering and resonant inelastic x-ray scattering experiments.
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We study the frustrated ferromagnetic spin-1 chains, where the ferromagnetic nearest-neighbor coupling competes with the antiferromagnetic next-nearest-neighbor coupling. We use the density matrix renormalization group to obtain the ground states. Through the analysis of spin-spin correlations we identify the double Haldane phase as well as the ferromagnetic phase. It is shown that the ferromagnetic coupling leads to incommensurate correlations in the double Haldane phase. Such short-range correlations transform continuously into the ferromagnetic instability at the transition to the ferromagnetic phase. We also compare the results with the spin-1/2 and classical spin systems, and discuss the string orders in the system.
Frustration in quantum spin systems promote a variety of novel quantum phases. An important example is the frustrated spin-$1$ model on the square lattice with the nearest-neighbor bilinear ($J_1$) and biquadratic ($K_1$) interactions. We provide strong evidence for a nematic spin liquid phase in a range of $K_1/J_1$ near the SU(3)-symmetric point ($J_1 = K_1$), based on the linear flavor-wave theory and extensive density matrix renormalization group calculation. This phase displays no spin dipolar or quadrupolar order, preserves translational symmetry but spontaneously breaks $C_4$ lattice rotational symmetry, and possesses fluctuations peaked at the wavevector $(pi, 2pi/3)$. The spin excitation gap drops rapidly with system size and appears to be gapless, and the nematic order is attributed to the dominant $(pi, 2pi/3)$ fluctuations. Our results provide a novel mechanism for electronic nematic order and, more generally, open up a new avenue to explore frustration-induced exotic ground states.
The static structure factor S(q) of frustrated spin-1/2 chains with isotropic exchange and a singlet ground state (GS) diverges at wave vector q_m when the GS has quasi-long-range order (QLRO) with periodicity 2pi/q_m but S(q_m) is finite in bond-order-wave (BOW) phases with finite-range spin correlations. Exact diagonalization and density matrix renormalization group (DMRG) calculations of S(q) indicate a decoupled phase with QLRO and q_m = pi/2 in chains with large antiferromagnetic exchange between second neighbors. S(q_m) identifies quantum phase transitions based on GS spin correlations.
We show that spin-S chains with SU(2)-symmetric, ferromagnetic nearest-neighbor and frustrating antiferromagnetic next-nearest-neighbor exchange interactions exhibit metamagnetic behavior under the influence of an external magnetic field for small S, in the form of a first-order transition to the fully polarized state. The corresponding magnetization jump increases gradually starting from an S-dependent critical value of exchange couplings and takes a maximum in the vicinity of a ferromagnetic Lifshitz point. The metamagnetism results from resonances in the dilute magnon gas caused by an interplay between quantum fluctuations and frustration.
We study a spin-5/2 antiferromagnetic trimerized chain substance SrMn3P4O14 using neutron powder diffraction experiments. The coplanar spiral magnetic structure appears below T_N1 = 2.2(1) K. Values of several magnetic structure parameters change rapidly at T_N2 = 1.75(5) K, indicating another phase transition, although the magnetic structures above and below T_N2 are the qualitatively same. The spiral magnetic structure can be explained by frustration between nearest-neighbor and next-nearest-neighbor exchange interactions in the trimerized chains.
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