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Register a new userNonequilibrium steady states of electric-field driven Mott insulators
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We present a systematic study of the nonequilibrium steady states (NESS) in Mott insulators driven by DC or AC electric fields, based on the Floquet dynamical mean-field theory. The results are analyzed using a generalized tunneling formula for the current, which is reminiscent of the Meir-Wingreen formula and provides insights into the relevant physical processes. In the DC case, the spectrum of the NESSs exhibits Wannier-Stark (WS) states associated with the lower and upper Hubbard bands. In addition, there emerge WS sidebands from many-body states. Using the tunneling formula, we demonstrate that the tunneling between these WS states leads to peaks or humps in the induced DC current. In the AC case, we cover a wide parameter range of excitation frequencies and field strengths to clarify the crossover from field-induced tunneling behavior in the DC limit to nonequilibrium states dominated by multiphoton absorption in the AC limit. In the crossover regime, the single-particle spectrum is characterized by a coexistence of Floquet sidebands and WS peaks, and the current and double occupation exhibits a nontrivial dependence on the field strength. The tunneling formula works quantitatively well even in the AC case, and we use it to discuss the potential cooperation of tunneling and multi-photon processes in the crossover regime. The tunneling formula and its simplifi
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Laser technology has developed and accelerated photo-induced nonequilibrium physics from both scientific and engineering viewpoints. The Floquet engineering, i.e., controlling material properties and functionalities by time-periodic drives, is a forefront of quantum physics of light-matter interaction, but limited to ideal dissipationless systems. For the Floquet engineering extended to a variety of materials, it is vital to understand the quantum states emerging in a balance of the periodic drive and energy dissipation. Here we derive the general description for nonequilibrium steady states (NESS) in periodically driven dissipative systems by focusing on the systems under high-frequency drive and time-independent Lindblad-type dissipation with the detailed balance condition. Our formula correctly describes the time-average, fluctuation, and symmetry property of the NESS, and can be computed efficiently in numerical calculations. Our approach will play fundamental roles in Floquet engineering in a broad class of dissipative quantum systems such as atoms and molecules, mesoscopic systems, and condensed matter.
The formalism for exactly calculating the retarded and advanced Greens functions of strongly correlated lattice models in a uniform electric field is derived within dynamical mean-field theory. To illustrate the method, we solve for the nonequilibrium density of states of the Hubbard model in both the metallic and Mott insulating phases at half-filling (with an arbitrary strength electric field) by employing the numerical renormalization group as the impurity solver. This general approach can be applied to any strongly correlated lattice model in the limit of large dimensions.
Driven many-body quantum systems where some parameter in the Hamiltonian is varied quasiperiodically in time may exhibit nonequilibrium steady states that are qualitatively different from their periodically driven counterparts. Here we consider a prototypical integrable spin system, the spin-$1/2$ transverse field Ising model in one dimension, in a pulsed magnetic field. The time dependence of the field is taken to be quasiperiodic by choosing the pulses to be of two types that alternate according to a Fibonacci sequence. We show that a novel steady state emerges after an exponentially long time when local properties (or equivalently, reduced density matrices of subsystems with size much smaller than the full system) are considered. We use the temporal evolution of certain coarse-grained quantities in momentum space to understand this nonequilibrium steady state in more detail and show that unlike the previously known cases, this steady state is neither described by a periodic generalized Gibbs ensemble nor by an infinite temperature ensemble. Finally, we study a toy problem with a single two-level system driven by a Fibonacci sequence; this problem shows how sensitive the nature of the final steady state is to the different parameters.
Since the beginnings of the electronic age, a quest for ever faster and smaller switches has been initiated, since this element is ubiquitous and foundational in any electronic circuit to regulate the flow of current. Mott insulators are promising candidates to meet this need as they undergo extremely fast resistive switching under electric field. However the mechanism of this transition is still under debate. Our spatially-resolved {mu}-XRD imaging experiments carried out on the prototypal Mott insulator (V0.95Cr0.05)2O3 show that the resistive switching is associated with the creation of a conducting filamentary path consisting in an isostructural compressed phase without any chemical nor symmetry change. This clearly evidences that the resistive switching mechanism is inherited from the bandwidth-controlled Mott transition. This discovery might hence ease the development of a new branch of electronics dubbed Mottronics.
Does a closed quantum many-body system that is continually driven with a time-dependent Hamiltonian finally reach a steady state? This question has only recently been answered for driving protocols that are periodic in time, where the long time behavior of the local properties synchronize with the drive and can be described by an appropriate periodic ensemble. Here, we explore the consequences of breaking the time-periodic structure of the drive with additional aperiodic noise in a class of integrable systems. We show that the resulting unitary dynamics leads to new emergent steady states in at least two cases. While any typical realization of random noise causes eventual heating to an infinite temperature ensemble for all local properties in spite of the system being integrable, noise which is self-similar in time leads to an entirely different steady state, which we dub as geometric generalized Gibbs ensemble, that emerges only after an astronomically large time scale. To understand the approach to steady state, we study the temporal behavior of certain coarse-grained quantities in momentum space that fully determine the reduced density matrix for a subsystem with size much smaller than the total system. Such quantities provide a concise description for any drive protocol in integrable systems that are reducible to a free fermion representation.
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