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Breaking the energy-symmetry blockade in magneto-optical rotation

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 Added by Chengjie Zhu
 Publication date 2018
  fields Physics
and research's language is English




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The magneto-optical polarization rotation effect has prolific applications in various research areas spanning the scientific spectrum including space and interstellar research, nano-technology and material science, biomedical imaging, and sub-atomic particle research. In nonlinear magneto-optical rotation (NMOR), the intensity of a linearly-polarized probe field affects the rotation of its own polarization plane while propagating in a magnetized medium. However, typical NMOR signals of conventional single-beam $Lambda-$scheme atomic magnetometers are peculiarly small, requiring sophisticated magnetic shielding under complex operational conditions. Here, we show the presence of an energy-symmetry blockade that undermines the NMOR effect in conventional single-beam $Lambda-$scheme atomic magnetometers. We further demonstrate, both experimentally and theoretically, an inelastic wave-mixing technique that breaks this NMOR blockade, resulting in more than five orders of magnitude ($>$300,000-fold) NMOR optical signal power spectral density enhancement never before seen with conventional single-beam $Lambda-$scheme atomic magnetometers. This new technique, demonstrated with substantially reduced light intensities, may lead to many applications, especially in the field of bio-magnetism and high-resolution low-field magnetic imaging.



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We present experimental and numerical studies of nonlinear magneto-optical rotation (NMOR) in rubidium vapor excited with resonant light tuned to the $5^2!S_{1/2}rightarrow 6^2!P_{1/2}$ absorption line (421~nm). Contrary to the experiments performed to date on the strong $D_1$ or $D_2$ lines, in this case, the spontaneous decay of the excited state $6^2!P_{1/2}$ may occur via multiple intermediate states, affecting the dynamics, magnitude and other characteristics of NMOR. Comparing the experimental results with the results of modelling based on Auzinsh et al., Phys. Rev. A 80, 1 (2009), we demonstrate that despite the complexity of the structure, NMOR can be adequately described with a model, where only a single excited-state relaxation rate is used.
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