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Register a new userEnhancing of nonlinear thermoelectric response of a correlated quantum dot in the Kondo regime by asymmetrically coupling to the leads
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We study the low temperature properties of the differential response of the current to a temperature gradient at finite voltage in a single level quantum dot including electron-electron interaction, non-symmetric couplings to the leads and non-linear effects. The calculated response is significantly enhanced in setups with large asymmetries between the tunnel couplings. In the investigated range of voltages and temperatures with corresponding energies up to several times the Kondo energy scale, the maximum response is enhanced nearly an order of magnitude with respect to symmetric coupling to the leads.
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We study nonequilibrium thermoelectric transport properties of a correlated impurity connected to two leads for temperatures below the Kondo scale. At finite bias, for which a current flows across the leads, we investigate the differential response of the current to a temperature gradient. In particular, we compare the influence of a bias voltage and of a finite temperature on this thermoelectric response. This is of interest from a fundamental point of view to better understand the two different decoherence mechanisms produced by a bias voltage and by temperature. Our results show that in this respect the thermoelectric response behaves differently from the electric conductance. In particular, while the latter displays a similar qualitative behavior as a function of voltage and temperature, both in theoretical and experimental investigations, qualitative differences occur in the case of the thermoelectric response. In order to understand this effect, we analyze the different contributions in connection to the behavior of the impurity spectral function versus temperature. Especially in the regime of strong interactions and large enough bias voltages we obtain a simple picture based on the asymmetric suppression or enhancement of the split Kondo peaks as a function of the temperature gradient. Besides the academic interest, these studies could additionally provide valuable information to assess the applicability of quantum dot devices as responsive nanoscale temperature sensors.
The time-dependent non-crossing approximation is used to study the transient current in a single electron transistor attached asymmetrically to two leads following a sudden change in the energy of the dot level. We show that for asymmetric coupling, sharp features in the density of states of the leads can induce oscillations in the current through the dot. These oscillations persist to much longer timescales than the timescale for charge fluctuations. The amplitude of the oscillations increases as the temperature or source-drain bias across the dot is reduced and saturates for values below the Kondo temperature. We discuss the microscopic origin of these oscillations and comment on the possibility for their experimental detection.
The zero-bias anomaly at low temperatures, originated by the Kondo effect when an electric current flows through a system formed by a spin-$1/2$ quantum dot and two metallic contacts is theoretically investigated. In particular, we compare the width of this anomaly $2T_{rm NE}$ with that of the Kondo resonance in the spectral density of states $2T_{K}^{rho}$, obtained from a Fano fit of the corresponding curves and also with the Kondo temperature, $T_K^G$, defined from the temperature evolution of the equilibrium conductance $G(T)$. In contrast to $T_K^G$ and $2T_{K}^{rho}$, we found that the scale $2T_{rm NE}$ strongly depends on the asymmetry between the couplings of the quantum dot to the leads while the total hybridization is kept constant. While the three scales are of the same order of magnitude, $2T_{rm NE}$ and $T_{K}^{rho}$ agree only in the case of large asymmetry between the different tunneling couplings of the contacts and the quantum dot. On the other hand, for similar couplings, $T_{rm NE}$ becomes larger than $T_{K}^{rho}$, reaching the maximum deviation, of the order of $30%$, for identical couplings. The fact that an additional parameter to $T_{rm NE}$ is needed to characterize the Kondo effect, weakenig the universality properties, points that some caution should be taken in the usual identification in experiments of the low temperature width of the zero-bias anomaly with the Kondo scale. Furthermore, our results indicate that the ratios $T_{rm NE}/T_K^G$ and $T_{K}^{rho}/T_K^G$ depend on the range used for the fitting.
Spin exchange between a single-electron charged quantum dot and itinerant electrons leads to an emergence of Kondo correlations. When the quantum dot is driven resonantly by weak laser light, the resulting emission spectrum allows for a direct probe of these correlations. In the opposite limit of vanishing exchange interaction and strong laser drive, the quantum dot exhibits coherent oscillations between the single-spin and optically excited states. Here, we show that the interplay between strong exchange and non-perturbative laser coupling leads to the formation of a new nonequilibrium quantum-correlated state, characterized by the emergence of a laser-induced secondary spin screening cloud, and examine the implications for the emission spectrum.
Kondo correlations are responsible for the emergence of a zero-bias peak in the low temperature differential conductance of Coulomb blockaded quantum dots. In the presence of a global SU(2)$otimes$SU(2) symmetry, which can be realized in carbon nanotubes, they also inhibit inelastic transitions which preserve the Kramers pseudospins associated to the symmetry. We report on magnetotransport experiments on a Kondo correlated carbon nanotube where resonant features at the bias corresponding to the pseudospin-preserving transitions are observed. We attribute this effect to a simultaneous enhancement of pseudospin-non-preserving transitions occurring at that bias. This process is boosted by asymmetric tunneling couplings of the two Kramers doublets to the leads and by asymmetries in the potential drops at the leads. Hence, the present work discloses a fundamental microscopic mechanisms ruling transport in Kondo systems far from equilibrium.
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