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Register a new userDynamical Signature of Symmetry Fractionalization in Frustrated Magnets
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The nontrivialness of quantum spin liquid (QSL) typically manifests in the non-local observables that signifies their existence, however, this fact actually casts shadow on detecting QSL with experimentally accessible probes. Here, we provide a solution by unbiasedly demonstrating dynamical signature of anyonic excitations and symmetry fractionalization in QSL. Employing large-scale quantum Monte Carlo simulation and stochastic analytic continuation, we investigate the extended XXZ model on the kagome lattice, and find out that across the phase transitions from Z2 QSLs to different symmetry breaking phases, spin spectral functions can reveal the presence and condensation of emergent anyonic spinon and vison excitations, in particular the translational symmetry fractionalization of the latter, which can be served as the unique dynamical signature of the seemingly ephemeral QSLs in spectroscopic techniques such as inelastic neutron or resonance (inelastic) X-ray scatterings.
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Deconfined quantum critical points govern continuous quantum phase transitions at which fractionalized (deconfined) degrees of freedom emerge. Here we study dynamical signatures of the fractionalized excitations in a quantum magnet (the easy-plane J-Q model) that realize a deconfined quantum critical point with emergent O(4) symmetry. By means of large-scale quantum Monte Carlo simulations and stochastic analytic continuation of imaginary-time correlation functions, we obtain the dynamic spin structure factors in the $S^{x}$ and $S^{z}$ channels. In both channels, we observe broad continua that originate from the deconfined excitations. We further identify several distinct spectral features of the deconfined quantum critical point, including the lower edge of the continuum and its form factor on moving through the Brillouin Zone. We provide field-theoretical and lattice model calculations that explain the overall shapes of the computed spectra, which highlight the importance of interactions and gauge fluctuations to explaining the spectral-weight distribution. We make further comparisons with the conventional Landau O(2) transition in a different quantum magnet, at which no signatures of fractionalization are observed. The distinctive spectral signatures of the deconfined quantum critical point suggest the feasibility of its experimental detection in neutron scattering and nuclear magnetic resonance experiments.
Investigation of the inelastic neutron scattering spectra in Fe$_{1+y}$Te$_{1-x}$Se$_{x}$ near a signature wave vector $mathbf{Q} = (1,0,0)$ for the bond-order wave (BOW) formation of parent compound Fe$_{1+y}$Te [Phys. Rev. Lett. 112, 187202 (2014)] reveals an acoustic-phonon-like dispersion present in all structural phases. While a structural Bragg peak accompanies the mode in the low-temperature phase of Fe$_{1+y}$Te, it is absent in the high-temperature tetragonal phase, where Bragg scattering at this $mathbf{Q}$ is forbidden by symmetry. Notably, this mode is also observed in superconducting FeTe$_{0.55}$Se$_{0.45}$, where structural and magnetic transitions are suppressed, and no BOW has been observed. The presence of this forbidden phonon indicates that the lattice symmetry is dynamically or locally broken by magneto-orbital BOW fluctuations, which are strongly coupled to lattice in these materials.
Symmetry fractionalization describes the fascinating phenomena that excitations in a 2D topological system can transform under symmetry in a fractional way. For example in fractional quantum Hall systems, excitations can carry fractional charges while the electrons making up the system have charge one. An important question is to understand what symmetry fractionalization (SF) patterns are possible given different types of topological order and different symmetries. A lot of progress has been made recently in classifying the SF patterns, providing deep insight into the strongly correlated experimental signatures of systems like spin liquids and topological insulators. We review recent developments on this topic. First, it was shown that the SF patterns need to satisfy some simple consistency conditions. More interesting, it was realized that some seemingly consistent SF patterns are actually `anomalous, i.e. they cannot be realized in strictly 2D systems. We review various methods that have been developed to detect such anomalies. Applying such an understanding to 2D spin liquid allows one to enumerate all potentially realizable SF patterns and propose numerical and experimental probing methods to distinguish them. On the other hand, the anomalous SF patterns were shown to exist on the surface of 3D systems and reflect the nontrivial order in the 3D bulk. We review examples of this kind where the bulk states are topological insulators, topological superconductors, or have other symmetry protected topological orders.
We consider Dirac electrons on the honeycomb lattice Kondo coupled to spin-1/2 degrees of freedom on the kagome lattice. The interactions between the spins are chosen along the lines of the Balents-Fisher-Girvin model that is known to host a $mathbb{Z}_2$ spin liquid and a ferromagnetic phase. The model is amenable to sign free auxiliary field quantum Monte Carlo simulations. While in the ferromagnetic phase the Dirac electrons acquire a gap, they remain massless in the $mathbb{Z}_2$ spin liquid phase due to the breakdown of Kondo screening. Since our model has an odd number of spins per unit cell, this phase is a non-Fermi liquid that violates the conventional Luttinger theorem which relates the Fermi surface volume to the particle density in a Fermi liquid. This non-Fermi liquid is a specific realization of the so called fractionalized Fermi liquid proposed in the context of heavy fermions. We probe the Kondo breakdown in this non-Fermi liquid phase via conventional observables such as the spectral function, and also by studying the mutual information between the electrons and the spins.
We overview physical effects of exchange frustration and quantum spin fluctuations in (quasi-) two dimensional (2D) quantum magnets ($S=1/2$) with square, rectangular and triangular structure. Our discussion is based on the $J_1$-$J_2$ type frustrated exchange model and its generalizations. These models are closely related and allow to tune between different phases, magnetically ordered as well as more exotic nonmagnetic quantum phases by changing only one or two control parameters. We survey ground state properties like magnetization, saturation fields, ordered moment and structure factor in the full phase diagram as obtained from numerical exact diagonalization computations and analytical linear spin wave theory. We also review finite temperature properties like susceptibility, specific heat and magnetocaloric effect using the finite temperature Lanczos method. This method is powerful to determine the exchange parameters and g-factors from experimental results. We focus mostly on the observable physical frustration effects in magnetic phases where plenty of quasi-2D material examples exist to identify the influence of quantum fluctuations on magnetism.
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