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A controlled qubit in a rotating frame opens new opportunities to probe fundamental quantum physics, such as geometric phases in physically rotating frames, and can potentially enhance detection of magnetic fields. Realising a single qubit that can be measured and controlled during physical rotation is experimentally challenging. In this work, we demonstrate quantum control of a single nitrogen-vacancy (NV) centre within a diamond rotated at 200,000rpm, a rotational period comparable to the NV spin coherence time $T_2$. We stroboscopically image individual NV centres that execute rapid circular motion in addition to rotation, and demonstrate preparation, control and readout of the qubit quantum state with lasers and microwaves. Using spin-echo interferometry of the rotating qubit, we are able to detect modulation of the NV Zeeman shift arising from the rotating NV axis and an external DC magnetic field. Our work establishes single NV qubits in diamond as quantum sensors in the physically rotating frame, and paves the way for the realisation of single-qubit diamond-based rotation sensors.
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Nuclear spins in certain solids couple weakly to their environment, making them attractive candidates for quantum information processing and inertial sensing. When coupled to the spin of an optically-active electron, nuclear spins can be rapidly polarized, controlled and read via lasers and radiofrequency fields. Possessing coherence times of several milliseconds at room temperature, nuclear spins hosted by a nitrogen-vacancy center in diamond are thus intriguing systems to observe how classical physical rotation at quantum timescales affects a quantum system. Unlocking this potential is hampered by precise and inflexible constraints on magnetic field strength and alignment in order to optically induce nuclear polarization, which restricts the scope for further study and applications. In this work, we demonstrate optical nuclear spin polarization and rapid quantum control of nuclear spins in a diamond physically rotating at $1,$kHz, faster than the nuclear spin coherence time. Free from the need to maintain strict field alignment, we are able to measure and control nuclear spins in hitherto inaccessible regimes, such as in the presence of a large, time-varying magnetic field that makes an angle of more than $100^circ$ to the nitrogen-lattice vacancy axis. The field induces spin mixing between the electron and nuclear states of the qubits, decoupling them from oscillating rf fields. We are able to demonstrate that coherent spin state control is possible at any point of the rotation, and even for up to six rotation periods. We combine continuous dynamical decoupling with quantum feedforward control to eliminate decoherence induced by imperfect mechanical rotation. Our work liberates a previously inaccessible degree of freedom of the NV nuclear spin, unlocking new approaches to quantum control and rotation sensing.
Group-IV color centers in diamond are a promising light-matter interface for quantum networking devices. The negatively charged tin-vacancy center (SnV) is particularly interesting, as its large spin-orbit coupling offers strong protection against phonon dephasing and robust cyclicity of its optical transitions towards spin-photon entanglement schemes. Here, we demonstrate multi-axis coherent control of the SnV spin qubit via an all-optical stimulated Raman drive between the ground and excited states. We use coherent population trapping and optically driven electronic spin resonance to confirm coherent access to the qubit at 1.7 K, and obtain spin Rabi oscillations at a rate of $Omega/2pi$=3.6(1) MHz. All-optical Ramsey interferometry reveals a spin dephasing time of $T_2^*$=1.3(3)$mu$s and two-pulse dynamical decoupling already extends the spin coherence time to $T_2$=0.33(14) ms. Combined with transform-limited photons and integration into photonic nanostructures, our results make the SnV a competitive spin-photon building block for quantum networks.
In this paper, we study the dynamical behavior and quantum metrology in a rotating Nitrogen-Vacancy(NV) center system which is subject to an external magnetic field. Based on the recently realized rapid rotation of nano-rotor [J. Ahn, et. al., Phys. Rev. Lett. 121, 033603 (2018) and R. Reimann, et. al., Phys. Rev. Lett. 121, 033602 (2018)], the frequency of the rotation is close to that of the intrinsic frequency of the NV center system, we predict the quantum beats phenomenon in the time domain and show that the quantum metrology can be enhanced by the superposition effect in our system.
Solid-state spin qubits are a promising platform for quantum computation and quantum networks. Recent experiments have demonstrated high-quality control over multi-qubit systems, elementary quantum algorithms and non-fault-tolerant error correction. Large-scale systems will require using error-corrected logical qubits that are operated fault-tolerantly, so that reliable computation is possible despite noisy operations. Overcoming imperfections in this way remains a major outstanding challenge for quantum science. Here, we demonstrate fault-tolerant operations on a logical qubit using spin qubits in diamond. Our approach is based on the 5-qubit code with a recently discovered flag protocol that enables fault-tolerance using a total of seven qubits. We encode the logical qubit using a novel protocol based on repeated multi-qubit measurements and show that it outperforms non-fault-tolerant encoding schemes. We then fault-tolerantly manipulate the logical qubit through a complete set of single-qubit Clifford gates. Finally, we demonstrate flagged stabilizer measurements with real-time processing of the outcomes. Such measurements are a primitive for fault-tolerant quantum error correction. While future improvements in fidelity and the number of qubits will be required, our realization of fault-tolerant protocols on the logical-qubit level is a key step towards large-scale quantum information processing based on solid-state spins.
Quantum error correction is of crucial importance for fault-tolerant quantum computers. As an essential step towards the implementation of quantum error-correcting codes, quantum non-demolition (QND) measurements are needed to efficiently detect the state of a logical qubit without destroying it. Here we implement QND measurements in a Si/SiGe two-qubit system, with one qubit serving as the logical qubit and the other serving as the ancilla. Making use of a two-qubit controlled-rotation gate, the state of the logical qubit is mapped onto the ancilla, followed by a destructive readout of the ancilla. Repeating this procedure enhances the logical readout fidelity from $75.5pm 0.3%$ to $94.5 pm 0.2%$ after 15 ancilla readouts. In addition, we compare the conventional thresholding method with an improved signal processing method called soft decoding that makes use of analog information in the readout signal to better estimate the state of the logical qubit. We demonstrate that soft decoding leads to a significant reduction in the required number of repetitions when the readout errors become limited by Gaussian noise, for instance in the case of readouts with a low signal-to-noise ratio. These results pave the way for the implementation of quantum error correction with spin qubits in silicon.
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