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Register a new userUltrathin Films of Superconducting Metals as a Platform for Topological Superconductivity
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The ingredients normally required to achieve topological superconductivity (TSC) are Cooper pairing, broken inversion symmetry, and broken time-reversal symmetry. We present a theoretical exploration of the possibility of using ultra-thin films of superconducting metals as a platform for TSC. Because they necessarily break inversion symmetry when prepared on a substrate and have intrinsic Cooper pairing, they can be TSCs when time-reversal symmetry is broken by an external magnetic field. Using microscopic density functional theory calculations we show that for ultrathin Pb and $beta$-Sn superconductors the position of the Fermi level can be tuned to quasi-2D band extrema energies using strain, and that the $g$-factors of these Bloch states can be extremely large enhancing the influence of external magnetic fields.
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The designer approach has become a new paradigm in accessing novel quantum phases of matter. Moreover, the realization of exotic states such as topological insulators, superconductors and quantum spin liquids often poses challenging or even contradictory demands for any single material. For example, it is presently unclear if topological superconductivity, which has been suggested as a key ingredient for topological quantum computing, exists at all in any naturally occurring material . This problem can be circumvented by using designer heterostructures combining different materials, where the desired physics emerges from the engineered interactions between the different components. Here, we employ the designer approach to demonstrate two major breakthroughs - the fabrication of van der Waals (vdW) heterostructures combining 2D ferromagnetism with superconductivity and the observation of 2D topological superconductivity. We use molecular-beam epitaxy (MBE) to grow two-dimensional islands of ferromagnetic chromium tribromide (CrBr$_3$) on superconducting niobium diselenide (NbSe$_2$) and show the signatures of one-dimensional Majorana edge modes using low-temperature scanning tunneling microscopy (STM) and spectroscopy (STS). The fabricated two-dimensional vdW heterostructure provides a high-quality controllable platform that can be integrated in device structures harnessing topological superconductivity. Finally, layered heterostructures can be readily accessed by a large variety of external stimuli potentially allowing external control of 2D topological superconductivity through electrical, mechanical, chemical, or optical means.
We analyze the evidence of Majorana zero modes in nanowires that came from tunneling spectroscopy and other experiments, and scout the path to topologically protected states that are of interest for quantum computing. We illustrate the importance of the superconductor-semiconductor interface quality and sketch out where further progress in materials science of these interfaces can take us. Finally, we discuss the prospects of observing more exotic non-Abelian anyons based on the same materials platform, and how to make connections to high energy physics.
We report transport measurements and tunneling spectroscopy in hybrid nanowires with epitaxial layers of superconducting Al and the ferromagnetic insulator EuS, grown on semiconducting InAs nanowires. In devices where the Al and EuS covered facets overlap, we infer a remanent effective Zeeman field of order 1 T, and observe stable zero-bias conductance peaks in tunneling spectroscopy into the end of the nanowire, consistent with topological superconductivity at zero applied field. Hysteretic features in critical current and tunneling spectra as a function of applied magnetic field support this picture. Nanowires with non-overlapping Al and EuS covered facets do not show comparable features. Topological superconductivity in zero applied field allows new device geometries and types of control.
We report on the precise integration of nm-scale topological insulator Josephson junctions into mm-scale superconducting quantum circuits via selective area epitaxy and local stencil lithography. By studying dielectric losses of superconducting microwave resonators fabricated on top of our selective area growth mask, we verify the compatibility of this in situ technique with microwave applications. We probe the microwave response of on-chip microwave cavities coupled to topological insulator-shunted superconducting qubit devices and observe a power dependence that indicates nonlinear qubit behaviour. Our method enables integration of complex networks of topological insulator nanostructures into superconducting circuits, paving the way for both novel voltage-controlled Josephson and topological qubits.
Majorana zero modes have been proposed as building blocks for fault-tolerant quantum information processing. They can be realized in semiconductors with strong spin-orbit interaction coupled to a superconductor. Experimental advances in the field of topological superconductivity have often been triggered by the development of new hybrid material systems. Among these, two-dimensional electron gases (2DEGs) are of particular interest due to their inherent design flexibility and scalability. Here we discuss results on a hybrid 2D platform based on a ternary 2DEG (InSbAs) coupled to in-situ grown Aluminum. The spin-orbit coupling in these 2DEGs can be tuned with the As concentration, reaching values up to 400 meV$unicode{xC5}$, thus exceeding typical values measured in its binary constituents. In addition to a large Lande g-factor $sim$ 55 (which is comparable to InSb), we show that the clean superconductor-semiconductor interface leads to highly transparent Josephson junctions and a hard induced superconducting gap in the proximitized semiconductor. Using this new platform we demonstrate the basic operation of phase-controllable Josephson junctions, superconducting islands and quasi-1D systems, prototypical device geometries used to study Majoranas. Our results establish InSbAs/Al 2DEGs as a promising material system to realize topological superconductivity.
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