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Register a new userInvestigation of the spin-1 honeycomb antiferromagnet BaNi$_2$V$_2$O$_8$ with easy plane anisotropy
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Added by
Ekaterina S. Klyushina
Publication date
2018
fields
Physics
and research's language is
English
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The magnetic properties of the two-dimensional, S=1 honeycomb antiferromagnet BaNi$_2$V$_2$O$_8$ have been comprehensively studied using DC susceptibility measurements and inelastic neutron scattering techniques. The magnetic excitation spectrum is found to be dispersionless within experimental resolution between the honeycomb layers, while it disperses strongly within the honeycomb plane where it consists of two gapped spin-wave modes. The magnetic excitations are compared to linear spin-wave theory allowing the Hamiltonian to be determined. The first- and second-neighbour magnetic exchange interactions are antiferromagnetic and lie within the ranges 10.90meV$le$J$_n$$le$13.35 meV and 0.85meV$le$J$_{nn}$$le$1.65 meV respectively. The interplane coupling J$_{out}$ is four orders of magnitude weaker than the intraplane interactions, confirming the highly two-dimensional magnetic behaviour of this compound. The sizes of the energy gaps are used to extract the magnetic anisotropies and reveal substantial easy-plane anisotropy and a very weak in-plane easy-axis anisotropy. Together these results reveal that BaNi$_2$V$_2$O$_8$ is a candidate compound for the investigation of vortex excitations and Berezinsky-Kosterliz-Thouless phenomenona.
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We investigate the critical properties of the spin-$1$ honeycomb antiferromagnet BaNi$_2$V$_2$O$_8$, both below and above the ordering temperature $T_N$ using neutron diffraction and muon spin rotation measurements. Our results characterize BaNi$_2$V$_2$O$_8$ as a two-dimensional (2D) antiferromagnet across the entire temperature range, displaying a series of crossovers from 2D Ising-like to 2D XY and then to 2D Heisenberg behavior with increasing temperature. In particular, the extracted critical exponent of the order parameter reveals a narrow temperature regime close to $T_N$, in which the system behaves as a 2D XY antiferromagnet. Above $T_N$, evidence for Berezinsky-Kosterlitz-Thouless behavior driven by vortex excitations is obtained from the scaling of the correlation length. Our experimental results are in accord with classical and quantum Monte Carlo simulations performed for microscopic magnetic model Hamiltonians for BaNi$_2$V$_2$O$_8$.
Combining inelastic neutron scattering and numerical simulations, we study the quasi-one dimensional Ising anisotropic quantum antiferromagnet bacovo in a longitudinal magnetic field. This material shows a quantum phase transition from a Neel ordered phase at zero field to a longitudinal incommensurate spin density wave at a critical magnetic field of 3.8 T. Concomitantly the excitation gap almost closes and a fundamental reconfiguration of the spin dynamics occurs. These experimental results are well described by the universal Tomonaga-Luttinger liquid theory developed for interacting spinless fermions in one dimension. We especially observe the rise of mainly longitudinal excitations, a hallmark of the unconventional low-field regime in Ising-like quantum antiferromagnet chains.
We report $^{51}$V nuclear magnetic resonance (NMR) and inelastic neutron scattering (INS) measurements on a quasi-1D antiferromagnet BaCo$_2$V$_2$O$_8$ under transverse field along the [010] direction. The scaling behavior of the spin-lattice relaxation rate above the N{e}el temperatures unveils a 1D quantum critical point (QCP) at $H_c^{1D}approx 4.7$ T, which is masked by the 3D magnetic order. With the aid of accurate analytical analysis and numerical calculations, we show that the zone center INS spectrum at $H_c^{1D}$ is precisely described by the pattern of the 1D quantum Ising model in a magnetic field, a class of universality described in terms of the exceptional $E_8$ Lie algebra. These excitations keep to be non-diffusive over a certain field range when the system is away from the 1D QCP. Our results provide an unambiguous experimental realization of the massive $E_8$ phase in the compound, and open new experimental route for exploring the dynamics of quantum integrable systems as well as physics beyond integrability.
Large single crystals of the new compound SrMn$_2$V$_2$O$_8$ have been grown by the floating-zone method. This transition-metal based oxide is isostructural to SrNi$_2$V$_2$O$_8$, described by the tetragonal space group $I4_1cd$. Magnetic properties were investigated by means of susceptibility, magnetization, and specific heat measurements. The title compound behaves like a one-dimensional magnetic system above the ordering temperature ($T_N$ = 43 K). The magnetic ground state can be described as a classical long-range ordered antiferromagnet with weak anisotropy.
Magnetocrystalline anisotropy is a fundamental property of magnetic materials that determines the dynamics of magnetic precession, the frequency of spin waves, the thermal stability of magnetic domains, and the efficiency of spintronic devices. We combine torque magnetometry and density functional theory calculations to determine the magnetocrystalline anisotropy of the metallic antiferromagnet Fe$_2$As. Fe$_2$As has a tetragonal crystal structure with the Neel vector lying in the (001) plane. We report that the four-fold magnetocrystalline anisotropy in the (001)-plane of Fe$_2$As is extremely small, ${K_{22}} = - 150~{rm{ J/}}{{rm{m}}^{rm{3}}}$ at T = 4 K, much smaller than perpendicular magnetic anisotropy of ferromagnetic structure widely used in spintronics device. ${K_{22}}$ is strongly temperature dependent and close to zero at T > 150 K. The anisotropy ${K_1}$ in the (010) plane is too large to be measured by torque magnetometry and we determine ${K_1} = -830~{rm{ kJ/}}{{rm{m}}^{rm{3}}}$ using first-principles density functional theory. Our simulations show that the contribution to the anisotropy from classical magnetic dipole-dipole interactions is comparable to the contribution from spin-orbit coupling. The calculated four-fold anisotropy in the (001) plane ${K_{22}}$ ranges from $- 292~{rm{ J/}}{{rm{m}}^{rm{3}}}$ to $280~{rm{ J/}}{{rm{m}}^{rm{3}}}$, the same order of magnitude as the measured value. We use ${K_1}$ from theory to predict the frequency and polarization of the lowest frequency antiferromagnetic resonance mode and find that the mode is linearly polarized in the (001)-plane with $f = $ 670 GHz.
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