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Register a new userEvidence of s-wave superconductivity in the noncentrosymmetric La$_7$Ir$_3$
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Superconductivity in noncentrosymmetric compounds has attracted sustained interest in the last decades. Here we present a detailed study on the transport, thermodynamic properties and the band structure of the noncentrosymmetric superconductor La$_7$Ir$_3$ ($T_c$ $sim$2.3 K) that was recently proposed to break the time-reversal symmetry. It is found that La$_7$Ir$_3$ displays a moderately large electronic heat capacity (Sommerfeld coefficient $gamma_n$ $sim$ 53.1 mJ/mol $text{K}^2$) and a significantly enhanced Kadowaki-Woods ratio (KWR $sim$ 32 $muOmega$ cm mol$^2$ K$^2$ J$^{-2}$) that is greater than the typical value ($sim$ 10 $muOmega$ cm mol$^2$ K$^2$ J$^{-2}$) for strongly correlated electron systems. The upper critical field $H_{c2}$ was seen to be nicely described by the single-band Werthamer-Helfand-Hohenberg model down to very low temperatures. The hydrostatic pressure effects on the superconductivity were also investigated. The heat capacity below $T_c$ reveals a dominant s-wave gap with the magnitude close to the BCS value. The first-principles calculations yield the electron-phonon coupling constant $lambda$ = 0.81 and the logarithmically averaged frequency $omega_{ln}$ = 78.5 K, resulting in a theoretical $T_c$ = 2.5 K, close to the experimental value. Our calculations suggest that the enhanced electronic heat capacity is more likely due to electron-phonon coupling, rather than the electron-electron correlation effects. Collectively, these results place severe constraints on any theory of exotic superconductivity in this system.
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We report a $^{71}$Ga nuclear-quadrupole-resonance (NQR) study on the characteristics of superconductivity in noncentrosymmetric Ir$_2$Ga$_9$ at zero field (H=0). The $^{71}$Ga-NQR measurements have revealed that $1/T_1$ has the clear coherence peak just below $T_{rm c}$, and decreases exponentially upon further cooling in Ir$_2$Ga$_9$. From these results, Ir$_2$Ga$_9$ is concluded to be the conventional s-wave superconductor. Despite the lack of spatial centrosymmetry, there are no evidence for unconventional superconducting state ascribed to ASOC in Ir$_2$Ga$_9$.
We report a comprehensive study of the centrosymmetric Re$_3$B and noncentrosymmetric Re$_7$B$_3$ superconductors. At a macroscopic level, their bulk superconductivity (SC), with $T_c$ = 5.1 K (Re$_3$B) and 3.3 K (Re$_7$B$_3$), was characterized via electrical-resistivity, magnetization, and heat-capacity measurements, while their microscopic superconducting properties were investigated by means of muon-spin rotation/relaxation ($mu$SR). In both Re$_3$B and Re$_7$B$_3$ the low-$T$ zero-field electronic specific heat and the superfluid density (determined via tranverse-field $mu$SR) suggest a nodeless SC. Both compounds exhibit some features of multigap SC, as evidenced by temperature-dependent upper critical fields $H_mathrm{c2}(T)$, as well as by electronic band-structure calculations. The absence of spontaneous magnetic fields below the onset of SC, as determined from zero-field $mu$SR measurements, indicates a preserved time-reversal symmetry in the superconducting state of both Re$_3$B and Re$_7$B$_3$. Our results suggest that a lack of inversion symmetry and the accompanying antisymmetric spin-orbit coupling effects are not essential for the occurrence of multigap SC in these rhenium-boron compounds.
The recently discovered kagome superconductor CsV$_3$Sb$_5$ ($T_c simeq 2.5$ K) has been found to host charge order as well as a non-trivial band topology, encompassing multiple Dirac points and probable surface states. Such a complex and phenomenologically rich system is, therefore, an ideal playground for observing unusual electronic phases. Here, we report on microscopic studies of its anisotropic superconducting properties by means of transverse-field muon spin rotation ($mu$SR) experiments. The temperature dependences of the in-plane and out-of-plane components of the magnetic penetration depth $lambda_{ab}^{-2}(T)$ and $lambda_{c}^{-2}(T)$ indicate that the superconducting order parameter exhibits a two-gap ($s+s$)-wave symmetry, reflecting the multiple Fermi surfaces of CsV3Sb5. The multiband nature of its superconductivity is further validated by the different temperature dependences of the anisotropic magnetic penetration depth $gamma_lambda(T)$ and upper critical field $gamma_{rm B_{c2}}(T)$, both in close analogy with the well known two-gap superconductor MgB$_2$. Remarkably, the high value of the $T_c/lambda^{-2}(0)$ ratio in both field orientations strongly suggests the unconventional nature of superconductivity. The relaxation rates obtained from zero field $mu$SR experiments do not show noticeable change across the superconducting transition, indicating that superconductivity does not break time reversal symmetry.
We report a comprehensive study of the noncentrosymmetric superconductor Mo$_3$P. Its bulk superconductivity, with $T_c = 5.5$ K, was characterized via electrical resistivity, magnetization, and heat-capacity measurements, while its microscopic electronic properties were investigated by means of muon-spin rotation/relaxation ($mu$SR) and nuclear magnetic resonance (NMR) techniques. In the normal state, NMR relaxation data indicate an almost ideal metallic behavior, confirmed by band-structure calculations, which suggest a relatively high electron density of states, dominated by the Mo $4d$-orbitals. The low-temperature superfluid density, determined via transverse-field $mu$SR and electronic specific heat, suggest a fully-gapped superconducting state in Mo$_3$P, with $Delta_0= 0.83$ meV, the same as the BCS gap value in the weak-coupling case, and a zero-temperature magnetic penetration depth $lambda_0 = 126$ nm. The absence of spontaneous magnetic fields below the onset of superconductivity, as determined from zero-field $mu$SR measurements, indicates a preserved time-reversal symmetry in the superconducting state of Mo$_3$P and, hence, spin-singlet pairing.
In general, magnetism and superconductivity are antagonistic to each other. However, there are several families of superconductors, in which superconductivity may coexist with magnetism, and only a few examples are known, when superconductivity itself induces spontaneous magnetism. The most known compounds are Sr$_2$RuO$_4$ and some noncentrosymmetric superconductors. Here, we report the finding of a narrow dome of a novel $s+is$ superconducting (SC) phase with broken time-reversal symmetry (BTRS) inside the broad $s$-wave SC region of the centrosymmetric multiband superconductor Ba$_{rm 1-x}$K$_{rm x}$Fe$_2$As$_2$ ($0.7 lesssim x lesssim 0.85$). We observe spontaneous magnetic fields inside this dome using the muon spin relaxation ($mu$SR) technique. Furthermore, our detailed specific heat study reveals that the BTRS dome appears very close to a change in the topology of the Fermi surface (Lifshitz transition). With this, we experimentally demonstrate the emergence of a novel quantum state due to topological changes of the electronic system.
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