Magnetic State Selected by Magnetic Dipole Interaction in Kagome Antiferromagnet NaBa$_{2}$Mn$_{3}$F$_{11}$


Abstract in English

We have studied the ground state of the classical Kagome antiferromagnet NaBa$_{2}$Mn$_{3}$F$_{11}$. Strong magnetic Bragg peaks observed in the $d$-spacing shorter than 6.0 AA were indexed by the propagation vectors of $boldsymbol{k}_{0} = (0,0,0)$. Additional peaks with weak intensities in the range of the $d$-spacing longer than 8.0 AA were indexed by the incommensurate vectors of $boldsymbol{k}_{1}=(0.3209(2),0.3209(2),0)$ and $boldsymbol{k}_{2}=(0.3338(4),0.3338(4),0)$. Magnetic structure analysis exhibits that the 120$^{circ}$ structure with the {it tail-chase} geometry having $boldsymbol{k}_0$ is modulated by the incommensurate vectors. The classical calculation of the Kagome Heisenberg antiferromagnet having the antiferromagnetic 2nd-neighbor interaction, the ground state of which is degenerated 120$^{circ}$ structures with $boldsymbol{k}_0$, reveals that the magnetic dipole-dipole (MDD) interaction including up to the 4th neighbor terms selects the tail-chase structure. The observed modulation of the tail-chase structure is indicated to be due to a small perturbation such as the long-range MDD interaction or the interlayer interaction.

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