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Register a new userDynamical density functional theory analysis of the laning instability in sheared soft matter
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Using dynamical density functional theory (DDFT) methods we investigate the laning instability of a sheared colloidal suspension. The nonequilibrium ordering at the laning transition is driven by non-affine particle motion arising from interparticle interactions. Starting from a DDFT which incorporates the non-affine motion, we perform a linear stability analysis that enables identification of the regions of parameter space where lanes form. We illustrate our general approach by applying it to a simple one-component fluid of soft penetrable particles.
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When a block made of an elastomer is subjected to large shear, its surface remains flat. When a block of biological soft tissue is subjected to large shear, it is likely that its surface in the plane of shear will buckle (apparition of wrinkles). One factor that distinguishes soft tissues from rubber-like solids is the presence -- sometimes visible to the naked eye -- of oriented collagen fibre bundles, which are stiffer than the elastin matrix into which they are embedded but are nonetheless flexible and extensible. Here we show that the simplest model of isotropic nonlinear elasticity, namely the incompressible neo-Hookean model, suffers surface instability in shear only at tremendous amounts of shear, i.e., above 3.09, which corresponds to a 72 degrees angle of shear. Next we incorporate a family of parallel fibres in the model and show that the resulting solid can be either reinforced or strongly weakened with respect to surface instability, depending on the angle between the fibres and the direction of shear, and depending on the ratio E/mu between the stiffness of the fibres and that of the matrix. For this ratio we use values compatible with experimental data on soft tissues. Broadly speaking, we find that the surface becomes rapidly unstable when the shear takes place against the fibres, and that as E/mu increases, so does the sector of angles where early instability is expected to occur.
This paper has been withdrawn by the author due to the incorrect application of the divergence theorem to Eqs 7, 8 and 9.
While the theory of diffusion of a single Brownian particle in confined geometries is well-established by now, we discuss here the theoretical framework necessary to generalize the theory of diffusion to dense suspensions of strongly interacting Brownian particles. Dynamical density functional theory (DDFT) for classical Brownian particles represents an ideal tool for this purpose. After outlining the basic ingredients to DDFT we show that it can be readily applied to flowing suspensions with time-dependent particle sources. Particle interactions lead to considerable layering in the mean density profiles, a feature that is absent in the trivial case of noninteracting, freely diffusing particles. If the particle injection rate varies periodically in time with a suitable frequency, a resonance in the layering of the mean particle density profile is predicted.
A density functional theory for colloidal dynamics is presented which includes hydrodynamic interactions between the colloidal particles. The theory is applied to the dynamics of colloidal particles in an optical trap which switches periodically in time from a stable to unstable confining potential. In the absence of hydrodynamic interactions, the resulting density breathing mode, exhibits huge oscillations in the trap center which are almost completely damped by hydrodynamic interactions. The predicted dynamical density fields are in good agreement with Brownian dynamics computer simulations.
Under shear, a system of particles changes its contact network and becomes unstable as it transitions between mechanically stable states. For hard spheres at zero pressure, contact breaking events necessarily generate an instability, but this is not the case at finite pressure, where we identify two types of contact changes: network events that do not correspond to instabilities and rearrangement events that do. The relative fraction of such events is constant as a function of system size, pressure and interaction potential, consistent with our observation that both nonlinearities obey the same finite-size scaling. Thus, the zero-pressure limit of the nonlinear response is highly singular.
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