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Register a new userOptimization of photon storage fidelity in ordered atomic arrays
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A major application for atomic ensembles consists of a quantum memory for light, in which an optical state can be reversibly converted to a collective atomic excitation on demand. There exists a well-known fundamental bound on the storage error, when the ensemble is describable by a continuous medium governed by the Maxwell-Bloch equations. The validity of this model can break down, however, in systems such as dense, ordered atomic arrays, where strong interference in emission can give rise to phenomena such as subradiance and selective radiance. Here, we develop a general formalism that finds the maximum storage efficiency for a collection of atoms with discrete, known positions, and a given spatial mode in which an optical field is sent. As an example, we apply this technique to study a finite two-dimensional square array of atoms. We show that such a system enables a storage error that scales with atom number $N_mathrm{a}$ like $sim (log N_mathrm{a})^2/N_mathrm{a}^2$, and that, remarkably, an array of just $4 times 4$ atoms in principle allows for an efficiency comparable to a disordered ensemble with optical depth of around 600.
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A central goal within quantum optics is to realize efficient interactions between photons and atoms. A fundamental limit in nearly all applications based on such systems arises from spontaneous emission, in which photons are absorbed by atoms and then re-scattered into undesired channels. In typical treatments of atomic ensembles, it is assumed that this re-scattering occurs independently, and at a rate given by a single isolated atom, which in turn gives rise to standard limits of fidelity in applications such as quantum memories or quantum gates. However, this assumption can be violated. In particular, spontaneous emission of a collective atomic excitation can be significantly suppressed through strong interference in emission. Thus far the physics underlying the phenomenon of subradiance and techniques to exploit it have not been well-understood. In this work, we provide a comprehensive treatment of this problem. First, we show that in ordered atomic arrays in free space, subradiant states acquire an interpretation in terms of optical modes that are guided by the array, which only emit due to scattering from the ends of the finite chain. We also elucidate the properties of subradiant states in the many-excitation limit. Finally, we introduce the new concept of selective radiance. Whereas subradiant states experience a reduced coupling to all optical modes, selectively radiant states are tailored to simultaneously radiate efficiently into a desired channel while scattering into undesired channels is suppressed, thus enabling an enhanced atom-light interface. We show that these states naturally appear in chains of atoms coupled to nanophotonic structures, and we analyze the performance of photon storage exploiting such states. We find that selectively radiant states allow for a photon storage error that scales exponentially better with number of atoms than previously known bounds.
We investigate the interaction of weak light fields with two-dimensional lattices of atoms, in which two-photon coupling establishes conditions of electromagnetically induced transparency and excites high lying atomic Rydberg states. This system features different interactions that act on disparate length scales, from zero-range defect scattering of atomic excitations and finite-range dipole exchange interactions to long-range Rydberg-state interactions that span the entire array. Analyzing their interplay, we identify conditions that yield a nonlinear quantum mirror which coherently splits incident fields into correlated photon-pairs in a single transverse mode, while transmitting single photons unaffected. Such strong photon-photon interactions in the absence of otherwise detrimental photon losses in Rydberg-EIT arrays opens up a promising approach for the generation and manipulation of quantum light, and the exploration of many-body phenomena with interacting photons.
We demonstrate a dual-rail optical Raman memory inside a polarization interferometer; this enables us to store polarization-encoded information at GHz bandwidths in a room-temperature atomic ensemble. By performing full process tomography on the system we measure up to 97pm1% process fidelity for the storage and retrieval process. At longer storage times, the process fidelity remains high, despite a loss of efficiency. The fidelity is 86pm4% for 1.5 mu s storage time, which is 5,000 times the pulse duration. Hence high fidelity is combined with a large time-bandwidth product. This high performance, with an experimentally simple setup, demonstrates the suitability of the Raman memory for integration into large-scale quantum networks.
Multiplexed quantum memories capable of storing and processing entangled photons are essential for the development of quantum networks. In this context, we demonstrate the simultaneous storage and retrieval of two entangled photons inside a solid-state quantum memory and measure a temporal multimode capacity of ten modes. This is achieved by producing two polarization entangled pairs from parametric down conversion and mapping one photon of each pair onto a rare-earth-ion doped (REID) crystal using the atomic frequency comb (AFC) protocol. We develop a concept of indirect entanglement witnesses, which can be used as Schmidt number witness, and we use it to experimentally certify the presence of more than one entangled pair retrieved from the quantum memory. Our work puts forward REID-AFC as a platform compatible with temporal multiplexing of several entangled photon pairs along with a new entanglement certification method useful for the characterisation of multiplexed quantum memories.
Building a quantum repeater network for long distance quantum communication requires photons and quantum registers that comprise qubits for interaction with light, good memory capabilities and processing qubits for storage and manipulation of photons. Here we demonstrate a key step, the coherent transfer of a photon in a single solid-state nuclear spin qubit with an average fidelity of 98% and storage over 10 seconds. The storage process is achieved by coherently transferring a photon to an entangled electron-nuclear spin state of a nitrogen vacancy centre in diamond, confirmed by heralding through high fidelity single-shot readout of the electronic spin states. Stored photon states are robust against repetitive optical writing operations, required for repeater nodes. The photon-electron spin interface and the nuclear spin memory demonstrated here constitutes a major step towards practical quantum networks, and surprisingly also paves the way towards a novel entangled photon source for photonic quantum computing.
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