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Register a new userOn the formation of a conducting surface channel by ionic liquid gating of an insulator
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Ionic liquid gating has become a popular tool for tuning the charge carrier densities of complex oxides. Among these the band insulator SrTiO$_3$ is one of the most extensively studied materials. While experiments have succeeded in inducing (super)conductivity, the process by which ionic liquid gating turns this insulator into a conductor is still under scrutiny. Recent experiments have suggested an electrochemical rather than electrostatic origin of the induced charge carriers. Here, we report experiments probing the time evolution of conduction of SrTiO$_3$ near the glass transition temperature of the ionic liquid. By cooling down to temperatures near the glass transition of the ionic liquid the process develops slowly and can be seen to evolve in time. The experiments reveal a process characterized by waiting times that can be as long as several minutes preceding a sudden appearance of conduction. For the conditions applied in our experiments we find a consistent interpretation in terms of an electrostatic mechanism for the formation of a conducting path at the surface of SrTiO$_3$. The mechanism by which the conducting surface channel develops relies on a nearly homogeneous lowering of the surface potential until the conduction band edge of SrTiO$_3$ reaches the Fermi level of the electrodes.
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Ionic liquid gating can markedly modulate the materials carrier density so as to induce metallization, superconductivity, and quantum phase transitions. One of the main issues is whether the mechanism of ionic liquid gating is an electrostatic field effect or an electrochemical effect, especially for oxide materials. Recent observation of the suppression of the ionic liquid gate-induced metallization in the presence of oxygen for oxide materials suggests the electrochemical effect. However, in more general scenarios, the role of oxygen in ionic liquid gating effect is still unclear. Here, we perform the ionic liquid gating experiments on a non-oxide material: two-dimensional ferromagnetic Cr2Ge2Te6. Our results demonstrate that despite the large increase of the gate leakage current in the presence of oxygen, the oxygen does not affect the ionic liquid gating effect (< 5 % difference), which suggests the electrostatic field effect as the mechanism on non-oxide materials. Moreover, our results show that the ionic liquid gating is more effective on the modulation of the channel resistances compared to the back gating across the 300 nm thick SiO2.
The type-II terminated 1T-TaS$_2$ surface of a three-dimensional 1T-TaS$_2$ bulk material realizes the effective spin-1/2 degree of freedom on each David-star cluster with ${T^2=-1}$ such that the time reversal symmetry is realized anomalously, despite the bulk three-dimensional 1T-TaS$_2$ material has an even number of electrons per unit cell with ${T^2=+1}$. This surface is effectively viewed as a spin-1/2 triangular lattice magnet, except with a symmetry-protected topological bulk. We further propose this surface termination realizes a spinon Fermi surface spin liquid with the surface fractionalization but with a non-exotic three-dimensional bulk. We analyze possible experimental consequences of the type-II terminated surface spin liquid.
Since its discovery as a Kondo insulator 50 years ago, SmB6 recently received a revival of interest due to detection of unexpected quantum oscillations in the insulating state, discovery of disorder-immune bulk transport, and proposals of correlation-driven topological physics. While recent transport results attribute the anomalous low temperature conduction to two-dimensional surface states, important alternatives, such as conduction channel residing in one-dimensional dislocation lines, have not been adequately explored. Here we study SmB6 with scanning microwave impedance microscopy and uncover evidence for conducting one-dimensional states terminating at surface step edges. These states remain conducting up to room temperature, indicating unusual robustness against scattering and an unconventional origin. Our results bring to light a heretofore undetected conduction route in SmB6 that contributes to the low temperature transport. The unique scenario of intrinsic one-dimensional conducting channels in a highly insulating correlated bulk offers a one-dimensional platform that may host exotic physics.
We study the surface states and chiral hinge states of a 3D second-order topological insulator in the presence of an external magnetic gauge field. Surfaces pierced by flux host Landau levels, while surfaces parallel to the applied field are not significantly affected. The chiral hinge modes mediate spectral flow between neighbouring surfaces. As the magnetic field strength is increased, the surface Landau quantization deviates from that of a massive Dirac cone. Quantitatively, the $n = 0$ Landau level falls inside the surface Dirac gap, and not at the gap edge. The $n e 0$ levels exhibit a further, qualitative discrepancy: while the massive Dirac cone is expected to produce pairs of levels ($pm n$) which are symmetric around zero energy, the $n$ and $-n$ levels become asymmetric in our lattice model -- one of the pair may even be absent from the spectrum, or hybridized with the continuum. In order to resolve the issue, we extend the standard 2D massive Dirac surface theory, by including additional Hamiltonian terms at $mathcal{O} (k^2)$. While these terms do not break particle-hole symmetry in the absence of magnetic field, they lead to the aforementioned Landau level asymmetry once the magnetic field is applied. We argue that similar $mathcal{O}(k^2)$ correction terms are generically expected in lattice models containing gapped Dirac fermions, using the BHZ model of a 2D topological insulator as an example.
We study the spectral density of electrons rho in an interacting quantum dot (QD) with a hybridization lambda to a non-interacting QD, which in turn is coupled to a non-interacting conduction band. The system corresponds to an impurity Anderson model in which the conduction band has a Lorentzian density of states of width Delta2. We solved the model using perturbation theory in the Coulomb repulsion U (PTU) up to second order and a slave-boson mean-field approximation (SBMFA). The PTU works surprisingly well near the exactly solvable limit Delta2 -> 0. For fixed U and large enough lambda or small enough Delta2, the Kondo peak in rho(omega) splits into two peaks. This splitting can be understood in terms of weakly interacting quasiparticles. Before the splitting takes place the universal properties of the model in the Kondo regime are lost. Using the SBMFA, simple analytical expressions for the occurrence of split peaks are obtained. For small or moderate Delta2, the side bands of rho(omega) have the form of narrow resonances, that were missed in previous studies using the numerical renormalization group. This technique also has shortcomings for describing properly the split Kondo peaks. As the temperature is increased, the intensity of the split Kondo peaks decreases, but it is not completely suppressed at high temperatures.
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