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Register a new userFractionalized excitations in the partially magnetized spin liquid candidate YbMgGaO4
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Quantum spin liquids (QSLs) are exotic states of matter characterized by emergent gauge structures and fractionalized elementary excitations. The recently discovered triangular lattice antiferromagnet YbMgGaO$_4$ is a promising QSL candidate, and the nature of its ground state is still under debate. Here, we use neutron scattering to study the spin excitations in YbMgGaO$_4$ under various magnetic fields. Our data reveal a dispersive spin excitation continuum with clear upper and lower excitation edges under a weak magnetic field ($H=2.5$ T). Moreover, a spectral crossing emerges at the $Gamma$ point at the Zeeman-split energy. The corresponding redistribution of the spectral weight and its field-dependent evolution are consistent with the theoretical prediction based on the inter-band and intra-band spinon particle-hole excitations associated with the Zeeman-split spinon bands, implying the presence of fractionalized excitations and spinon Fermi surfaces in the partially magnetized YbMgGaO$_4$.
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A quantum spin liquid (QSL) is an exotic state of matter in which electrons spins are quantum entangled over long distances, but do not show symmetry-breaking magnetic order in the zero-temperature limit. The observation of QSL states is a central aim of experimental physics, because they host collective excitations that transcend our knowledge of quantum matter; however, examples in real materials are scarce. Here, we report neutron-scattering measurements on YbMgGaO4, a QSL candidate in which Yb3+ ions with effective spin-1/2 occupy a triangular lattice. Our measurements reveal a continuum of magnetic excitations - the essential experimental hallmark of a QSL - at very low temperature (0.06 K). The origin of this peculiar excitation spectrum is a crucial question, because isotropic nearest-neighbor interactions do not yield a QSL ground state on the triangular lattice. Using measurements of the magnetic excitations close to the field-polarized state, we identify antiferromagnetic next-nearest-neighbor interactions in the presence of planar anisotropy as key ingredients for QSL formation in YbMgGaO4.
The elementary excitations from the conventional magnetic ordered states, such as ferromagnets and antiferromagnets, are magnons. Here, we elaborate a case where the well-defined magnons are absent completely and the spin excitation spectra exhibit an entire continuum in the itinerant edge ferromagnetic state of graphene arising from the flatband edge electronic states. Based on the further studies of the entanglement entropy and finite-size analysis, we show that the continuum other than the Stoner part results from the spin-1/2 spinons deconfined from magnons. The spinon continuum in a magnetically ordered state is ascribed to a ferromagnetic Luttinger liquid in this edge ferromagnet. The investigation is carried out by using the numerical exact diagonalization method with a projection of the interacting Hamiltonian onto the flat band.
Theoretical models of the spin-orbital liquid (SOL) FeSc$_2$S$_4$ have predicted it to be in close proximity to a quantum critical point separating a spin-orbital liquid phase from a long-range ordered magnetic phase. Here, we examine the magnetic excitations of FeSc$_2$S$_4$ through time-domain terahertz spectroscopy under an applied magnetic field. At low temperatures an excitation emerges that we attribute to a singlet-triplet excitation from the SOL ground state. A three-fold splitting of this excitation is observed as a function of applied magnetic field. As singlet-triplet excitations are forbidden in inversion symmetric pure spin systems, our results demonstrate the non-trivial character of the entangled spin-orbital singlet ground state. Using experimentally obtained parameters we compare to existing theoretical models to determine FeSc$_2$S$_4$s proximity to the quantum critical point. In the context of these models, we estimate that the characteristic length of the singlet correlations to be $xi/ (textbf{a}/2) approx 8.2$ (where $textbf{a}/2$ is the nearest neighbor lattice constant) which establishes FeSc$_2$S$_4$ as a SOL with long-range entanglement.
DC-magnetization data measured down to 40 mK speak against conventional freezing and reinstate YbMgGaO$_4$ as a triangular spin-liquid candidate. Magnetic susceptibility measured parallel and perpendicular to the $c$-axis reaches constant values below 0.1 and 0.2 K, respectively, thus indicating the presence of gapless low-energy spin excitations. We elucidate their nature in the triple-axis inelastic neutron scattering experiment that pinpoints the low-energy ($E$ $leq$ $J_0$ $sim$ 0.2 meV) part of the excitation continuum present at low temperatures ($T$ $<$ $J_0$/$k_B$), but emph{completely} disappearing upon warming the system above $T$ $gg$ $J_0$/$k_B$. In contrast to the high-energy part at $E$ $>$ $J_0$ that is rooted in the breaking of nearest-neighbor valence bonds and persists to temperatures well above $J_0$/$k_B$, the low-energy one originates from the rearrangement of the valence bonds and thus from the propagation of unpaired spins. We further extend this picture to herbertsmithite, the spin-liquid candidate on the kagome lattice, and argue that such a hierarchy of magnetic excitations may be a universal feature of quantum spin liquids.
We develop an approach to describe antiferromagnetic magnons on a bipartite lattice supporting the N{e}el state using fractionalized degrees of freedom typically inherent to quantum spin liquids. In particular we consider a long-range magnetically ordered state of interacting two-dimensional quantum spin$-1/2$ models using the Chern-Simons (CS) fermion representation of interacting spins. The interaction leads to Cooper instability and pairing of CS fermions, and to CS superconductivity which spontaneously violates the continuous $mathrm{U}(1)$ symmetry generating a linearly-dispersing gapless Nambu-Goldstone mode due to phase fluctuations. We evaluate this mode and show that it is in high-precision agreement with magnons of the corresponding N{e}el antiferromagnet irrespective to the lattice symmetry. Using the fermion formulation of a system with competing interactions, we show that the frustration gives raise to nontrivial long-range four, six, and higher-leg interaction vertices mediated by the CS gauge field, which are responsible for restoring of the continuous symmetry at sufficiently strong frustration. We identify these new interaction vertices and discuss their implications to unconventional phase transitions. We also apply the proposed theory to a model of anyons that can be tuned continuously from fermions to bosons.
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