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Ultrafast nanoscale magnetic switching via intense picosecond electron bunches

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 Publication date 2017
  fields Physics
and research's language is English




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The magnetic field associated with a picosecond intense electron pulse is shown to switch locally the magnetization of extended films and nanostructures and to ignite locally spin waves excitations. Also, topologically protected magnetic textures such as skyrmions can be imprinted swiftly in a sample with a residual Dzyaloshinskii-Moriya spin-orbital coupling. Characteristics of the created excitations such as the topological charge or the width of the magnon spectrum can be steered via the duration and the strength of the electron pulses. The study points to a possible way for a spatiotemporally controlled generation of magnetic and skyrmionic excitations.



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Magnetic chiral skyrmions are vortex like spin structures that appear as stable or meta-stable states in magnetic materials due to the interplay between the symmetric and antisymmetric exchange interactions, applied magnetic field and/or uniaxial anisotropy. Their small size and internal stability make them prospective objects for data storage but for this, the controlled switching between skyrmion states of opposite polarity and topological charge is essential. Here we present a study of magnetic skyrmion switching by an applied magnetic field pulse based on a discrete model of classical spins and atomistic spin dynamics. We found a finite range of coupling parameters corresponding to the coexistence of two degenerate isolated skyrmions characterized by mutually inverted spin structures with opposite polarity and topological charge. We demonstrate how for a wide range of material parameters a short inclined magnetic field pulse can initiate the reliable switching between these states at GHz rates. Detailed analysis of the switching mechanism revealed the complex path of the system accompanied with the excitation of a chiral-achiral meron pair and the formation of an achiral skyrmion.
The ability to perform nanoscale electric field imaging of elementary charges at ambient temperatures will have diverse interdisciplinary applications. While the nitrogen-vacancy (NV) center in diamond is capable of high-sensitivity electrometry, demonstrations have so far been limited to macroscopic field features or detection of single charges internal to diamond itself. In this work we greatly extend these capabilities by using a shallow NV center to image the electric field of a charged atomic force microscope tip with nanoscale resolution. This is achieved by measuring Stark shifts in the NV spin-resonance due to AC electric fields. To achieve this feat we employ for the first time, the integration of Qdyne with scanning quantum microscopy. We demonstrate near single charge sensitivity of $eta_e = 5.3$ charges/$sqrt{text{Hz}}$, and sub-charge detection ($0.68e$). This proof-of-concept experiment provides the motivation for further sensing and imaging of electric fields using NV centers in diamond.
We demonstrate the fabrication of a single electron transistor device based on a single ultra-small silicon quantum dot connected to a gold break junction with a nanometer scale separation. The gold break junction is created through a controllable electromigration process and the individual silicon quantum dot in the junction is determined to be a Si_170 cluster. Differential conductance as a function of the bias and gate voltage clearly shows the Coulomb diamond which confirms that the transport is dominated by a single silicon quantum dot. It is found that the charging energy can be as large as 300meV, which is a result of the large capacitance of a small silicon quantum dot (1.8 nm). This large Coulomb interaction can potentially enable a single electron transistor to work at room temperature. The level spacing of the excited state can be as large as 10 meV, which enables us to manipulate individual spin via an external magnetic field. The resulting Zeeman splitting is measured and the lande factor of 2.3 is obtained, suggesting relatively weak electron-electron interaction in the silicon quantum dot which is beneficial for spin coherence time.
The Landau-Lifshitz-Gilbert (LLG) equation, used to model magneto-dynamics in ferromagnets, tacitly assumes that the angular momentum associated with spin precession can relax instantaneously when the real or effective magnetic field causing the precession is turned off. This neglect of spin inertia is unphysical and would violate energy conservation. Recently, the LLG equation was modified to account for inertia effects. The consensus, however, seems to be that such effects would be unimportant in slow magneto-dynamics that take place over time scales much longer that the relaxation time of the angular momentum, which is typically few fs to perhaps ~100 ps in ferromagnets. Here, we show that there is at least one very serious and observable effect of spin inertia even in slow magneto-dynamics. It involves the switching error probability associated with flipping the magnetization of a nanoscale ferromagnet with an external agent, such as a magnetic field. The switching may take ~ns to complete when the field strength is close to the threshold value for switching, which is much longer than the angular momentum relaxation time, and yet the effect of spin inertia is felt in the switching error probability. This is because the ultimate fate of a switching trajectory, i.e. whether it results in success or failure, is influenced by what happens in the first few ps of the switching action when nutational dynamics due to spin inertia holds sway. Spin inertia increases the error probability, which makes the switching more error-prone. This has vital technological significance because it relates to the reliability of magnetic logic and memory.
The detection of ensembles of spins under ambient conditions has revolutionized the biological, chemical, and physical sciences through magnetic resonance imaging and nuclear magnetic resonance. Pushing sensing capabilities to the individual-spin level would enable unprecedented applications such as single molecule structural imaging; however, the weak magnetic fields from single spins are undetectable by conventional far-field resonance techniques. In recent years, there has been a considerable effort to develop nanoscale scanning magnetometers, which are able to measure fewer spins by bringing the sensor in close proximity to its target. The most sensitive of these magnetometers generally require low temperatures for operation, but measuring under ambient conditions (standard temperature and pressure) is critical for many imaging applications, particularly in biological systems. Here we demonstrate detection and nanoscale imaging of the magnetic field from a single electron spin under ambient conditions using a scanning nitrogen-vacancy (NV) magnetometer. Real-space, quantitative magnetic-field images are obtained by deterministically scanning our NV magnetometer 50 nanometers above a target electron spin, while measuring the local magnetic field using dynamically decoupled magnetometry protocols. This single-spin detection capability could enable single-spin magnetic resonance imaging of electron spins on the nano- and atomic scales and opens the door for unique applications such as mechanical quantum state transfer.
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