We present observations of CO(3-2) and $^{13}$CO(3-2) emission near the supernebula in the dwarf galaxy NGC 5253, which contains one of the best examples of a potential globular cluster in formation. The 0.3 resolution images reveal an unusual molecular cloud, Cloud D1, coincident with the radio-infrared supernebula. The ~6-pc diameter cloud has a linewidth, $Delta$ v = 21.7 km/s, that reflects only the gravitational potential of the star cluster residing within it. The corresponding virial mass is 2.5 x 10$^5$ M$_odot$. The cluster appears to have a top-heavy initial mass function, with $M_{low}$~1-2 M$_odot$. Cloud D1 is optically thin in CO(3-2) probably because the gas is hot. Molecular gas mass is very uncertain but constitutes < 35% of the dynamical mass within the cloud boundaries. In spite of the presence of an estimated ~1500-2000 O stars within the small cloud, the CO appears relatively undisturbed. We propose that Cloud D1 consists of molecular clumps or cores, possibly star-forming, orbiting with more evolved stars in the core of the giant cluster.