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Register a new userStudy of systematic effects in the HfF$^+$ ion experiment to search for the electron electric dipole moment
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A.N. Petrov
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The energy splitings for $J = 1$, $F=3/2$, $|M_F|=3/2$ hyperfine levels of the $^3Delta_1$ electronic state of $^{180}$Hf$^{19}$F$^+$ ion are calculated as functions of the external variable electric and magnetic fields within two approaches. In the first one transition to the rotating frame is performed, whereas in the second approach the quantization of rotating electromagnetic field is performed. Calculations are required for understanding possible systematic errors in the experiment to search for electron electric dipole moment (eEDM) on $^{180}$Hf$^{19}$F$^+$ ion.
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We report the theoretical investigation of the suppression of magnetic systematic effects in HfF$^+$ cation for the experiment to search for the electron electric dipole moment. The g-factors for $J = 1$, $F=3/2$, $|M_F|=3/2$ hyperfine levels of the $^3Delta_1$ state are calculated as functions of the external electric field. The lowest value for the difference between the g-factors of $Omega$-doublet levels, $Delta g = 3 times 10^{-6}$, is attained at the electric field 7 V/cm. The body-fixed g-factor, $G_{parallel}$, was obtained both within the electronic structure calculations and with our fit of the experimental data from [H. Loh, K. C. Cossel, M. C. Grau, K.-K. Ni, E. R. Meyer, J. L. Bohn, J. Ye, and E. A. Cornell, Science {bf 342}, 1220 (2013)]. For the electronic structure calculations we used a combined scheme to perform correlation calculations of HfF$^+$ which includes both the direct 4-component all-electron and generalized relativistic effective core potential approaches. The electron correlation effects were treated using the coupled cluster methods. The calculated value $G_{parallel}=0.0115$ agrees very well with the $G_{parallel}=0.0118$ obtained in the our fitting procedure. The calculated value $D_{parallel}=-1.53$ a.u. of the molecule frame dipole moment (with the origin in the center of mass) is in agreement with the experimental value $D_{parallel}=-1.54(1)$ a.u. [H. Loh, Ph.D. thesis, Massachusetts Institute of Technology (2006)].
We recently set a new limit on the electric dipole moment of the electron (eEDM) (J. Baron et al., ACME collaboration, Science 343 (2014), 269-272), which represented an order-of-magnitude improvement on the previous limit and placed more stringent constraints on many CP-violating extensions to the Standard Model. In this paper we discuss the measurement in detail. The experimental method and associated apparatus are described, together with the techniques used to isolate the eEDM signal. In particular, we detail the way experimental switches were used to suppress effects that can mimic the signal of interest. The methods used to search for systematic errors, and models explaining observed systematic errors, are also described. We briefly discuss possible improvements to the experiment.
A Cs fountain electron electric dipole moment (EDM) experiment using electric-field quantization is demonstrated. With magnetic fields reduced to 200 pT or less, the electric field lifts the degeneracy between hyperfine levels of different|mF| and, along with the slow beam and fountain geometry, suppresses systematics from motional magnetic fields. Transitions are induced and the atoms polarized and analyzed in field-free regions. The feasibility of reaching a sensitivity to an electron EDM of 2 x 10 exp(-50) C-m [1.3 x 10 exp(-29) e-cm] in a cesium fountain experiment is discussed.
We investigate the merits of a measurement of the permanent electric dipole moment of the electron ($e$EDM) with barium monofluoride molecules, thereby searching for phenomena of CP violation beyond those incorporated in the Standard Model of particle physics. Although the BaF molecule has a smaller enhancement factor in terms of the effective electric field than other molecules used in current studies (YbF, ThO and ThF$^+$), we show that a competitive measurement is possible by combining Stark-deceleration, laser-cooling and an intense primary cold source of BaF molecules. With the long coherent interaction times obtainable in a cold beam of BaF, a sensitivity of $5times10^{-30}$ e$cdot$cm for an $e$EDM is feasible. We describe the rationale, the challenges and the experimental methods envisioned to achieve this target.
Experiments dedicated to the measurement of the electric dipole moment of the neutron require outstanding control of the magnetic field uniformity. The neutron electric dipole moment (nEDM) experiment at the Paul Scherrer Institute uses a 199Hg co-magnetometer to precisely monitor magnetic field variations. This co-magnetometer, in the presence of field non-uniformity, is responsible for the largest systematic effect of this measurement. To evaluate and correct that effect, offline measurements of the field non-uniformity were performed during mapping campaigns in 2013, 2014 and 2017. We present the results of these campaigns, and the improvement the correction of this effect brings to the neutron electric dipole moment measurement.
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