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Register a new userElectronic anisotropies revealed by detwinned ARPES measurements of FeSe
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We report high resolution ARPES measurements of detwinned FeSe single crystals. The application of a mechanical strain is used to promote the volume fraction of one of the orthorhombic domains in the sample, which we estimate to be 80$%$ detwinned. While the full structure of the electron pockets consisting of two crossed ellipses may be observed in the tetragonal phase at temperatures above 90~K, we find that remarkably, only one peanut-shaped electron pocket oriented along the longer $a$ axis contributes to the ARPES measurement at low temperatures in the nematic phase, with the expected pocket along $b$ being not observed. Thus the low temperature Fermi surface of FeSe as experimentally determined by ARPES consists of one elliptical hole pocket and one orthogonally-oriented peanut-shaped electron pocket. Our measurements clarify the long-standing controversies over the interpretation of ARPES measurements of FeSe.
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Using angle-resolved photoemission spectroscopy it is revealed that in the vicinity of optimal doping the electronic structure of La2-xSrxCuO4 cuprate undergoes an electronic reconstruction associated with a wave vector q_a=(pi, 0). The reconstructed Fermi surface and folded band are distinct to the shadow bands observed in BSCCO cuprates and in underdoped La2-xSrxCuO4 with x <= 0.12, which shift the primary band along the zone diagonal direction. Furthermore the folded bands appear only with q_a=(pi, 0) vector, but not with q_b= (0, pi). We demonstrate that the absence of q_b reconstruction is not due to the matrix-element effects in the photoemission process, which indicates the four-fold symmetry is broken in the system.
The origin of the electronic nematicity in FeSe, which occurs below a tetragonal-to-orthorhombic structural transition temperature $T_s$ ~ 90 K, well above the superconducting transition temperature $T_c = 9$ K, is one of the most important unresolved puzzles in the study of iron-based superconductors. In both spin- and orbital-nematic models, the intrinsic magnetic excitations at $mathbf{Q}_1=(1, 0)$ and $mathbf{Q}_2=(0, 1)$ of twin-free FeSe are expected to behave differently below $T_s$. Although anisotropic spin fluctuations below 10 meV between $mathbf{Q}_1$ and $mathbf{Q}_2$ have been unambiguously observed by inelastic neutron scattering around $T_c (<<T_s)$, it remains unclear whether such an anisotropy also persists at higher energies and associates with the nematic transition $T_s$. Here we use resonant inelastic x-ray scattering (RIXS) to probe the high-energy magnetic excitations of uniaxial-strain detwinned FeSe. A prominent anisotropy between the magnetic excitations along the $H$ and $K$ directions is found to persist to $sim200$ meV, which is even more pronounced than the anisotropy of spin waves in BaFe$_2$As$_2$. This anisotropy decreases gradually with increasing temperature and finally vanishes at a temperature around the nematic transition temperature $T_s$. Our results reveal an unprecedented strong spin-excitation anisotropy with a large energy scale well above the $d_{xz}/d_{yz}$ orbital splitting, suggesting that the nematic phase transition is primarily spin-driven. Moreover, the measured high-energy spin excitations are dispersive and underdamped, which can be understood from a local-moment perspective. Our findings provide the much-needed understanding of the mechanism for the nematicity of FeSe and point to a unified description of the correlation physics across seemingly distinct classes of Fe-based superconductors.
A nematic transition preceding a long-range spin density wave antiferromagnetic phase is a common feature of many Fe based superconductors. However, in the FeSe system with a nematic transition at $T_{rm s} approx$ 90 K no evidence for long-range static magnetism down to very low temperature was found. The lack of magnetism is a challenge for the theoretical description of FeSe. Here, we investigated high-quality single crystals of FeSe using high-field (up to 9.5 Tesla) muon spin rotation ($mu$SR) measurements. The $mu$SR Knight shift and the bulk susceptibility linearly scale at high temperatures but deviate from this behavior around $T^{*} sim 10$ K, where the Knight shift exhibits a kink. This behavior hints to an essential change of the electronic and/or magnetic properties crossing the region near $T^{*}$. In the temperature range $T_{rm s} gtrsim T gtrsim T^{*}$ the muon spin depolarization rate follows a critical behavior $Lambda propto T^{-0.4}$. The observed non-Fermi liquid behavior with a cutoff at $T^{*}$ indicates that FeSe is in the vicinity to a antiferromagnetic quantum critical point. Our analysis is suggestive for $T^{*}$ triggered by the Lifshitz transition.
We study superconducting FeSe (Tc = 9 K) exhibiting the tetragonal-orthorhombic structural transition (Ts = 90 K) without any antiferromagnetic ordering, by utilizing angle-resolved photoemission spectroscopy. In the detwinned orthorhombic state, the energy position of the dyz orbital band at the Brillouin zone corner is 50 meV higher than that of dxz, indicating the orbital order similar to NaFeAs and BaFe2As2 families. Evidence of orbital order also appears in the hole bands at the Brillouin zone center. Precisely measured temperature dependence using strain-free samples shows that the onset of the orbital ordering (To) occurs very close to Ts, thus suggesting that the electronic nematicity above Ts is considerably weaker in FeSe compared to BaFe2As2 family.
The improved resolution of laser-based angle-resolved photoemission spectroscopy (ARPES) allows reliable access to fine structures in the spectrum. We present a systematic, doping-dependent study of a recently discovered low-energy kink in the nodal dispersion of Bi2Sr2CaCu2O8+d (Bi-2212), which demonstrates the ubiquity and robustness of this kink in underdoped Bi-2212. The renormalization of the nodal velocity due to this kink becomes stronger with underdoping, revealing that the nodal Fermi velocity is non-universal, in contrast to assumed phenomenology. This is used together with laser-ARPES measurements of the gap velocity, v2, to resolve discrepancies with thermal conductivity measurements.
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