Large field-induced gap of Kitaev-Heisenberg paramagnons in $alpha$-RuCl$_{3}$


Abstract in English

The honeycomb Kitaev-Heisenberg model is a source of a quantum spin liquid with Majorana fermions and gauge flux excitations as fractional quasiparticles. In the quest of finding a pertinent material, $alpha$-RuCl$_{3}$ recently emerged as a prime candidate. Here we unveil highly unusual low-temperature heat conductivity $kappa$ of $alpha$-RuCl$_{3}$: beyond a magnetic field of $B_capprox$ 7.5 T, $kappa$ increases by about one order of magnitude, resulting in a large magnetic field dependent peak at about 7 K, both for in-plane as well as out-of-plane transport. This clarifies the unusual magnetic field dependence unambiguously to be the result of severe scattering of phonons off putative Kitaev-Heisenberg excitations in combination with a drastic field-induced change of the magnetic excitation spectrum. In particular, an unexpectedly large energy gap arises, which increases approximately linearly with the magnetic field and reaches a remarkably large $hbaromega_0/k_Bapprox $ 50 K at 18 T.

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