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Register a new userProbing interactions of thermal Sr Rydberg atoms using simultaneous optical and ion detection
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We demonstrate a method for probing interaction effects in a thermal beam of strontium atoms using simultaneous measurements of Rydberg EIT and spontaneously created ions or electrons. We present a Doppler-averaged optical Bloch equation model that reproduces the optical signals and allows us to connect the optical coherences and the populations. We use this to determine that the spontaneous ionization process in our system occurs due to collisions between Rydberg and ground state atoms in the EIT regime. We measure the cross section of this process to be 0.6 $pm$ 0.2 $sigma_{rm{geo}}$, where $sigma_{rm{geo}}$ is the geometrical cross section of the Rydberg atom. This results adds complementary insight to a range of recent studies of interacting thermal Rydberg ensembles.
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We demonstrate microwave-to-optical conversion using six-wave mixing in $^{87}$Rb atoms where the microwave field couples to two atomic Rydberg states, and propagates collinearly with the converted optical field. We achieve a photon conversion efficiency of ~5% in the linear regime of the converter. In addition, we theoretically investigate all-resonant six-wave mixing and outline a realistic experimental scheme for reaching efficiencies greater than 60%.
We develop a formalism for photoionization (PI) and potential energy curves (PECs) of Rydberg atoms in ponderomotive optical lattices and apply it to examples covering several regimes of the optical-lattice depth. The effect of lattice-induced PI on Rydberg-atom lifetime ranges from noticeable to highly dominant when compared with natural decay. The PI behavior is governed by the generally rapid decrease of the PI cross sections as a function of angular-momentum ($ell$), and by lattice-induced $ell$-mixing across the optical-lattice PECs. In GHz-deep lattices, $ell$-mixing leads to a rich PEC structure, and the significant low-$ell$ PI cross sections are distributed over many lattice-mixed Rydberg states. In lattices less than several tens-of-MHz deep, atoms on low-$ell$ PECs are essentially $ell$-mixing-free and maintain large PI cross sections, while atoms on high-$ell$ PECs trend towards being PI-free. Characterization of PI in GHz-deep Rydberg-atom lattices may be beneficial for optical control and quantum-state manipulation of Rydberg atoms, while data on PI in shallower lattices are potentially useful in high-precision spectroscopy and quantum-computing applications of lattice-confined Rydberg atoms.
We report on the observation of interactions between ultracold Rydberg atoms and ions in a Paul trap. The rate of observed inelastic collisions, which manifest themselves as charge transfer between the Rydberg atoms and ions, exceeds that of Langevin collisions for ground state atoms by about three orders of magnitude. This indicates a huge increase in interaction strength. We study the effect of the vacant Paul traps electric fields on the Rydberg excitation spectra. To quantitatively describe the exhibited shape of the ion loss spectra, we need to include the ion-induced Stark shift on the Rydberg atoms. Furthermore, we demonstrate Rydberg excitation on a dipole-forbidden transition with the aid of the electric field of a single trapped ion. Our results confirm that interactions between ultracold atoms and trapped ions can be controlled by laser coupling to Rydberg states. Adding dynamic Rydberg dressing may allow for the creation of spin-spin interactions between atoms and ions, and the elimination of collisional heating due to ionic micromotion in atom-ion mixtures.
We present a novel spectroscopic method for probing the insitu~density of quantum gases. We exploit the density-dependent energy shift of highly excited {Rydberg} states, which is of the order $10$MHz,/,1E14,cm$^{text{-3}}$ for rubidium~for triplet s-wave scattering. The energy shift combined with a density gradient can be used to localize Rydberg atoms in density shells with a spatial resolution less than optical wavelengths, as demonstrated by scanning the excitation laser spatially across the density distribution. We use this Rydberg spectroscopy to measure the mean density addressed by the Rydberg excitation lasers, and to monitor the phase transition from a thermal gas to a Bose-Einstein condensate (BEC).
We theoretically analyze the interactions and decay rates for atoms dressed by multiple laser fields to strongly interacting Rydberg states using a quantum master equation approach. In this framework a comparison of two-level and three-level Rydberg-dressing schemes is presented. We identify a resonant enhancement of the three-level dressed interaction strength which originates from cooperative multiphoton couplings as well as small distance dependent decay rates. In this regime the soft-core shape of the potential is independent of the sign of the bare Rydberg-Rydberg interaction, while its sign can be repulsive or attractive depending on the intermediate state detuning. As a consequence, near-resonant Rydberg dressing in three-level atomic systems may enable the realization of laser driven quantum fluids with long-range and anisotropic interactions and with controllable dissipation.
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