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Register a new userAnalytic model of a multi-electron atom
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A fully analytical approximation for the observable characteristics of many-electron atoms is developed via a complete and orthonormal hydrogen-like basis with a single-effective charge parameter for all electrons of a given atom. The basis completeness allows us to employ the secondary-quantized representation for the construction of regular perturbation theory, which includes in a natural way correlation effects, converges fast and enables an effective calculation of the subsequent corrections. The hydrogen-like basis set provides a possibility to perform all summations over intermediate states in closed form, including both the discrete and continuous spectra. This is achieved with the help of the decomposition of the multi-particle Green function in a convolution of single-electronic Coulomb Green functions. We demonstrate that our fully analytical zeroth-order approximation describes the whole spectrum of the system, provides accuracy, which is independent of the number of electrons and is important for applications where the Thomas-Fermi model is still utilized. In addition already in second-order perturbation theory our results become comparable with those via a multi-configuration Hartree-Fock approach.
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A relativistic version of the effective charge model for computation of observable characteristics of multi-electron atoms and ions is developed. A complete and orthogonal Dirac hydrogen basis set, depending on one parameter -- effective nuclear charge $Z^{*}$ -- identical for all single-electron wave functions of a given atom or ion, is employed for the construction of the secondary-quantized representation. The effective charge is uniquely determined by the charge of the nucleus and a set of electron occupation numbers for a given state. We thoroughly study the accuracy of the leading-order approximation for the total binding energy and demonstrate that it is independent of the number of electrons of a multi-electron atom. In addition, it is shown that the fully analytical leading-order approximation is especially suited for the description of highly charged ions since our wave functions are almost coincident with the Dirac-Hartree-Fock ones for the complete spectrum. Finally, we evaluate various atomic characteristics, such as scattering factors and photoionization cross-sections, and thus envisage that the effective charge model can replace other models of comparable complexity, such as the Thomas-Fermi-Dirac model for all applications where it is still utilized.
Strong interaction between the light field and an atom is often achieved with cavities. Recent experiments have used a different configuration: a propagating light field is strongly focused using a system of lenses, the atom being supposed to sit at the focal position. In reality, this last condition holds only up to some approximation; in particular, at any finite temperature, the atom position fluctuates. We present a formalism that describes the focalized field and the atom sitting at an arbitrary position. As a first application, we show that thermal fluctuations do account for the extinction data reported in M. K. Tey et al., Nature Physics 4, 924 (2008).
Tailoring the interactions between quantum emitters and single photons constitutes one of the cornerstones of quantum optics. Coupling a quantum emitter to the band edge of a photonic crystal waveguide (PCW) provides a unique platform for tuning these interactions. In particular, the crossover from propagating fields $E(x) propto e^{pm ik_x x}$ outside the bandgap to localized fields $E(x) propto e^{-kappa_x |x|}$ within the bandgap should be accompanied by a transition from largely dissipative atom-atom interactions to a regime where dispersive atom-atom interactions are dominant. Here, we experimentally observe this transition for the first time by shifting the band edge frequency of the PCW relative to the $rm D_1$ line of atomic cesium for $bar{N}=3.0pm 0.5$ atoms trapped along the PCW. Our results are the initial demonstration of this new paradigm for coherent atom-atom interactions with low dissipation into the guided mode.
Deterministic quantum interactions between single photons and single quantum emitters are a vital building block towards the distribution of quantum information between remote systems. Deterministic photon-atom state transfer has been demonstrated by using protocols that include active feedback or synchronized control pulses. Here we demonstrate a completely passive swap gate between the states of a single photon and a single atom. The underlying mechanism is single-photon Raman interaction (SPRINT) - an interference-based effect in which a photonic qubit deterministically controls the state of a material qubit encoded in the two ground states of a {Lambda} system, and vice versa. Using a nanofiber-coupled microsphere resonator coupled to single Rb atoms we swap a photonic qubit into the atom and back, demonstrating nonclassical fidelities in both directions. Requiring no control fields or feedback protocol, the gate takes place automatically at the timescale of the atoms cavity- enhanced spontaneous emission time. Applicable to any waveguide-coupled {Lambda} system, this scheme provides a versatile building block for the modular scaling up of quantum information processing systems.
Precision sensing, and in particular high precision magnetometry, is a central goal of research into quantum technologies. For magnetometers, often trade-offs exist between sensitivity, spatial resolution, and frequency range. The precision, and thus the sensitivity of magnetometry, scales as $1/sqrt {T_2}$ with the phase coherence time, $T_2$, of the sensing system playing the role of a key determinant. Adapting a dynamical decoupling scheme that allows for extending $T_2$ by orders of magnitude and merging it with a magnetic sensing protocol, we achieve a measurement sensitivity even for high frequency fields close to the standard quantum limit. Using a single atomic ion as a sensor, we experimentally attain a sensitivity of $4.6$ pT $/sqrt{Hz}$ for an alternating-current magnetic field near 14 MHz. Based on the principle demonstrated here, this unprecedented sensitivity combined with spatial resolution in the nanometer range and tunability from direct-current to the gigahertz range could be used for magnetic imaging in as of yet inaccessible parameter regimes.
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