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Chiral spin liquid on kagome antiferromagnet induced by Dzyaloshinskii-Moriya interaction

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 Added by Laura Messio
 Publication date 2017
  fields Physics
and research's language is English




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The quantum spin liquid material herbertsmithite is described by an antiferromagnetic Heisenberg model on the kagome lattice with non-negligible Dzyaloshinskii-Moriya interaction~(DMI). A well established phase transition to the $mathbf q=0$ long-range order occurs in this model when the DMI strength increases, but the precise nature of a small-DMI phase remains controversial. Here, we describe a new phase obtained from Schwinger-boson mean-field theory that is stable at small DMI, and which can explain the dispersionless spectrum seen in inelastic neutron scattering experiment by Han et al (Nature (London) 492, 406 (2012)}). It is a time-reversal symmetry breaking $mathbb Z_2$ spin liquid, with the unique property of a small and constant spin gap in an extended region of the Brillouin zone. The phase diagram as a function of DMI and spin size is given, and dynamical spin structure factors are presented.



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A preponderance of evidence suggests that the ground state of the nearest-neighbor $S = 1/2$ antiferromagnetic Heisenberg model on the kagome lattice is a gapless spin liquid. Many candidate materials for the realization of this model possess in addition a Dzyaloshinskii-Moriya (DM) interaction. We study this system by tensor-network methods and deduce that a weak but finite DM interaction is required to destabilize the gapless spin-liquid state. The critical magnitude, $D_c/J simeq 0.012(2)$, lies well below the DM strength proposed in the kagome material herbertsmithite, indicating a need to reassess the apparent spin-liquid behavior reported in this system.
We performed a comprehensive electron spin resonance, magnetization and heat capacity study on the field-induced magnetic phase transitions in the kagome antiferromagnet $alpha-Cu_3Mg(OH)_6Br_2$. With the successful preparation of single crystals, we mapped out the magnetic phase diagrams under the $c$-axis and $ab$-plane directional magnetic fields $B$. For $B|c$, the three-dimensional (3D) magnon Bose-Einstein condensation (BEC) is evidenced by the power law scaling of the transition temperature, $T_cpropto (B_c-B)^{2/3}$. For $B|ab$, the transition from the canted antiferromagetic (CAFM) state to the fully polarized (FP) state is a crossover rather than phase transition, and the characteristic temperature has a significant deviation from the 3D BEC scaling. The different behaviors of the field-induced magnetic transitions for $B|c$ and $B|ab$ could result from the Dzyaloshinkii-Moriya (DM) interaction with the DM vector along the $c$-axis, which preserves the $c$-axis directional spin rotation symmetry and breaks the spin rotation symmetry when $B|ab$. The 3D magnon BEC scaling for $B|c$ is immune to the off-stoichiometric disorder in our sample $alpha-Cu_{3.26}Mg_{0.74}(OH)_6Br_2$. Our findings have the potential to shed light on the investigations of the magnetic anisotropy and disorder effects on the field-induced magnon BEC in the quantum antiferromagnet.
Recently, antiferromagnets have received revived interest due to their significant potential for developing next-generation ultrafast magnetic storage. Here we report dc spin pumping by the acoustic resonant mode in a canted easy-plane antiferromagnet {alpha}-Fe2O3 enabled by the Dzyaloshinskii-Moriya interaction. Systematic angle and frequency dependent measurements demonstrate that the observed spin pumping signals arise from resonance-induced spin injection and inverse spin Hall effect in {alpha}-Fe2O3/metal heterostructures, mimicking the behavior of spin pumping in conventional ferromagnet/nonmagnet systems. The pure spin current nature is further corroborated by reversal of the polarity of spin pumping signals when the spin detector is switched from platinum to tungsten which has an opposite sign of the spin Hall angle. Our results highlight the potential opportunities offered by the low-frequency acoustic resonant mode in canted easy-plane antiferromagnets for developing next-generation, functional spintronic devices.
98 - F. Azizi , H. Rezania 2021
We have theoretically studied the spin structure factors of Heisenberg model on honeycomb lattice in the presence of longitudinal magnetic field, i.e. magnetic field perpendicular to the honeycomb plane, and Dzyaloshinskii-Moriya interaction. The possible effects of next nearest neighbor exchange constant are investigated in terms of anisotropy in the Heisenberg interactions. This spatial anisotropy is due to the difference between nearest neighbor exchange coupling constant and next nearest neighbor exchange coupling constant. The original spin model hamiltonian is mapped to a bosonic model via a hard core bosonic transformation where an infinite hard core repulsion is imposed to constrain one boson occupation per site. Using Greens function approach, the energy spectrum of quasiparticle excitation has been obtained. The spectrum of the bosonic gas has been implemented in order to obtain two particle propagator which corresponds to spin structure factor of original Heisenberg chain model Hamiltonian. The results show the position of peak in the dynamical transverse spin structure factor at fixed value for Dzyaloshinskii Moriya interaction moves to higher frequency with magnetic field. Also the intensity of dynamical transverse spin structure factor is not affected by magnetic field. However the Dzyaloshinskii Moriya interaction strength causes to decrease the intensity of dynamical transverse spin structure factor. The increase of magnetic field does not varied the frequency position of peaks in dynamical longitudinal spin susceptibility however the intensity reduces with magnetic field. Our results show static transverse structure factor is found to be monotonically decreasing with magnetic field and temperature for different vlaues of next nearest neighbor coupling exchange constant.
We study $S=1$ spin liquid states on the kagome lattice constructed by Gutzwiller-projected $p_x+ip_y$ superconductors. We show that the obtained spin liquids are either non-Abelian or Abelian topological phases, depending on the topology of the fermionic mean-field state. By calculating the modular matrices $S$ and $T$, we confirm that projected topological superconductors are non-Abelian chiral spin liquid (NACSL). The chiral central charge and the spin Hall conductance we obtained agree very well with the $SO(3)_1$ (or, equivalently, $SU(2)_2$) field theory predictions. We propose a local Hamiltonian which may stabilize the NACSL. From a variational study we observe a topological phase transition from the NACSL to the $Z_2$ Abelian spin liquid.
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