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Metallic atomic junctions pose the ultimate limit to the scaling of electrical contacts. They serve as model systems to probe electrical and thermal transport down to the atomic level as well as quantum effects occurring in one-dimensional systems. Charge transport in atomic junctions has been studied intensively in the last two decades. However, heat transport remains poorly characterized because of significant experimental challenges. Specifically the combination of high sensitivity to small heat fluxes and the formation of stable atomic contacts has been a major hurdle for the development of this field. Here we report on the realization of heat transfer measurements through atomic junctions and analyze the thermal conductance of single atomic gold contacts at room temperature. Simultaneous measurements of charge and heat transport reveal the proportionality of electrical and thermal conductance, quantized with the respective conductance quanta. This constitutes an atomic scale verification of the well-known Wiedemann-Franz law. We anticipate that our findings will be a major advance in enabling the investigation of heat transport properties in molecular junctions, with meaningful implications towards the manipulation of heat at the nanoscale
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We report on the fabrication, transport measurements, and density functional theory (DFT) calculations of atomic size contacts made out of gadolinium (Gd). Gd is known to have local moments mainly associated with $f$ electrons. These coexist with itinerant $s$ and $d$ bands that account for its metallic character. Here we explore whether and how the local moments influence electronic transport properties at the atomic scale. Using both Scanning Tunneling Microscope (STM) and lithographic Mechanically Controllable Break Junction (MCBJ) techniques under cryogenic conditions, we study the conductance of Gd when only few atoms form the junction between bulk electrodes made out of the very same material. Thousands of measurements shows that Gd has an average lowest conductance, attributed to an atom-size contact, below $frac{2e^2}{h}$. Our DFT calculations for monostrand chains anticipate that the $f$ bands are fully spin polarized and insulating, and that the conduction may be dominated by $s$, $p$, and $d$ bands. DFT quantum transport calculations quantitatively reproduce the experimental results for zero bias and reveal that, while $s-p$ bands are dominant for transport, $d$ orbitals seem to have a relevant contribution in some cases.
We study the transport of charge carriers through finite graphene structures. The use of numerical exact kernel polynomial and Green function techniques allows us to treat actual sized samples beyond the Dirac-cone approximation. Particularly we investigate disordered nanoribbons, normal-conductor/graphene interfaces and normal-conductor/graphene/normal-conductor junctions with a focus on the behavior of the local density of states, single-particle spectral function, optical conductivity and conductance. We demonstrate that the contacts and bulk disorder will have a major impact on the electronic properties of graphene-based devices.
Linear and non-linear transport properties through an atomic-size point contact based on oxides two-dimensional electron gas is examined using the tight-binding method and the $mathbf{kcdot p}$ approach. The ballistic transport is analyzed in contacts realized at the (001) interface between band insulators $LaAlO_3$ and $SrTiO_3$ by using the Landauer-Buttiker method for many sub-bands derived from three Ti 3d orbitals ($d_{yz}$, $d_{zx}$ and $d_{xy}$) in the presence of an out-of-plane magnetic field. We focus especially on the role played by the atomic spin-orbit coupling and the inversion symmetry breaking term pointing out three transport regimes: the first, at low energies, involving the first $d_{xy}$-like sub-bands, where the conductance quantization is robust; a second one, at intermediate energies, entailing further $d_{xy}$-like sub-bands, where the sub-band splitting induced by the magnetic field is quenched; the third one, where the mixing between light $d_{xy}$-like, heavy $d_{yz}$-like and $d_{zx}$-like sub-bands is so strong that the conductance plateaus turn out to be very narrow. Very good agreement is found with recent experiments exploring the transport properties at low energies.
We report a numerical investigation on the heat transfer through one dimensional arrays of metallic nanoparticles closely spaced in a host material. Our simulations show that the multipolar interactions play a crucial role in the heat transport via collective plasmons. Calculations of the plasmonic thermal conductance and of the thermal conductivity in ballistic and diffusive regime, respectively have been carried out. (a) Using the Landauer-Buttiker formalism we have found that, when the host material dielectric constant takes positive values, the multipolar interactions drastically enhance by several order of magnitude the ballistic thermal conductance of collective plasmons compared with that of a classical dipolar chain. On the contrary, when the host material dielectric constant takes negative values, we have demonstrated the existence of non-ballistic multipolar modes which annihilate the heat transfer through the chains. (b) Using the kinetic theory we have also examined the thermal behavior of chains in the diffusion approximation. We have shown that the plasmonic thermal conductivity of metallic nanoparticle chains can reach 1% of the bulk metal thermal conductivity . This result could explain the anomalously high thermal conductivity observed in many colloidal suspensions, the so called nanofluids.
We investigate heat circulators where a phase coherent region is contacted by three leads that are either normal- or superconducting. A magnetic field, and potentially the superconducting phases, allow to control the preferential direction of the heat flow between the three-different temperature-biased contacts. The main goal of this study is to analyze the requirements for heat circulation in non-ideal devices, in particular focusing on sample-to-sample variations. Quite generally, we find that the circulation performance of the devices is good as long as only a few transport channels are involved. We compare the performance of circulators with normalconducting contacts to those with superconducting contacts and find that the circulation coefficient are essentially unchanged.
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