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Register a new userEvolution of Superconducting Gaps in Th-Substituted Sm$_{1-x}$Th$_x$OFeAs Studied by Multiple Andreev Reflection Spectroscopy
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Using intrinsic multiple Andreev reflections effect (IMARE) spectroscopy, we studied SnS contacts in the layered oxypnictide superconductors Sm$_{1-x}$Th$_x$OFeAs with various thorium doping and critical temperatures $T_C = 21-54$ K. We observe a scaling between both superconducting gaps and $T_C$. The determined BCS-ratio for the large gap $2Delta_L/k_BT_C = 5.0-5.7$ and its eigen BCS-ratio (in a hypothetical case of zero interband coupling) $2Delta_L/k_BT_C^L = 4.1-4.6$ both exceeding the weak-coupling limit 3.52, and for the small gap $2Delta_S/k_BT_C = 1.2-1.6$ remain nearly constant within all the $T_C$ range studied. The temperature dependences $Delta_{L,S}(T)$ agree well with a two-band BCS-like Moskalenko and Suhl model. We prove intraband coupling to be stronger than interband coupling, whereas and Coulomb repulsion constants $mu^{ast}$ are finite in Sm-based oxypnictides.
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We studied a reproducible fine structure observed in dynamic conductance spectra of Andreev arrays in Sm$_{1-x}$Th$_x$OFeAs superconductors with various thorium concentrations ($x = 0.08 - 0.3$) and critical temperatures $T_c = 26-50$,K. This structure is unambiguously caused by a multiple boson emission (of the same energy) during the process of multiple Andreev reflections. The directly determined energy of the bosonic mode reaches $varepsilon_0 = 14.8 pm 2.2$,meV for optimal compound. Within the studied range of $T_c$, this energy as well as the large $Delta_L$ and the small $Delta_S$ superconducting gaps, nearly scales with critical temperature with the characteristic ratio $varepsilon_0/k_BT_c approx 3.2$ (and $2Delta_L/k_BT_c approx 5.3$, correspondingly) resembling the expected energy $Delta_L + Delta_S$ of spin resonance and spectral density enhancement in $s^{pm}$ and $s^{++}$ states, respectively.
We studied SNS- and S-N-S-N-...-S contacts (where S - superconductor, N - normal metal) formed by break-junction technique in polycrystalline Sm$_{1-x}$Th$_x$OFeAs superconductor samples with critical temperatures $T_C = (34 div 45)$ K. In such contacts (intrinsic) multiple Andreev reflections effects were observed. Using spectroscopies based on these effects, we detected two independent bulk order parameters and determined their magnitudes. Theoretical analysis of the large and the small gap temperature dependences revealed superconducting properties of Sm$_{1-x}$Th$_x$OFeAs to be driven by intraband coupling, and $sqrt{V_{11}V_{22}}/V_{12} approx 14$ (where $V_{ij}$ - electron-boson interaction matrix elements), whereas the ratio between density of states for the bands with the small and the large gap, $N_2/N_1$, correspondingly, was roughly of an order. We estimated solo BCS-ratio values in a hypothetic case of zero interband coupling ($V_{i e j} = 0$) for each condensate as $2Delta_{L,S}/k_BT_C^{L,S} le 4.5$. The values are constant within the range of critical temperatures studied, and correspond to a case of strong intraband electron-phonon coupling.
FeSe single crystals have been studied by soft point-contact Andreev-reflection spectroscopy. Superconducting gap features in the differential resistance dV/dI(V) of point contacts such as a characteristic Andreev-reflection double-minimum structure have been measured versus temperature and magnetic field. Analyzing dV/dI within the extended two-gap Blonder-Tinkham-Klapwijk model allows to extract both the temperature and magnetic field dependence of the superconducting gaps. The temperature dependence of both gaps is close to the standard BCS behavior. Remarkably, the magnitude of the double-minimum structure gradually vanishes in magnetic field, while the minima position only slightly shifts with field indicating a weak decrease of the superconducting gaps. Analyzing the dV/dI(V) spectra for 25 point contacts results in the averaged gap values <Delta_L> = 1.8+/-0.4meV and <Delta_S>=1.0+/-0.2 meV and reduced values 2<Delta_L>/kTc=4.2+/-0.9 and 2<Delta_S>/kTc=2.3+/-0.5 for the large (L) and small (S) gap, respectively. Additionally, the small gap contribution was found to be within tens of percent decreasing with both temperature and magnetic field. No signatures in the dV/dI spectra were observed testifying a gapless superconductivity or presence of even smaller gaps.
Point contact Andreev reflection studies have been conducted on FeSe single crystals by lowering the temperatures down to 0.5 K. The point contact Andreev reflection spectra were analyzed in the framework of the two-band model. As a result, the presence of two anisotropic superconducting gaps in FeSe were certainly established and their BCS-like temperature dependencies were obtained. The weights of each gap have been determined and the anisotropy parameter has been calculated. It is shown, that sub-kelvin temperatures are necessary to ascertain details of the superconducting gap structure, especially for multiband materials when Andreev reflection spectroscopy is applied.
A deep understanding of the character of superconductivity in the recently discovered Fe-based oxypnictides ReFeAsO1-xFx (Re = rare-earth) necessarily requires the determination of the number of the gaps and their symmetry in k space, which are fundamental ingredients of any model for the pairing mechanism in these new superconductors. In the present paper, we show that point-contact Andreev-reflection experiments performed on LaFeAsO1-xFx (La-1111) polycrystals with Tc ~ 27 K and SmFeAsO0.8F0.2 (Sm-1111) ones with Tc ~ 53 K gave differential conductance curves exhibiting two peaks at low bias and two additional structures (peaks or shoulders) at higher bias, an experimental situation quite similar to that observed by the same technique in pure and doped MgB2. The single-band Blonder-Tinkham-Klapwijk model is totally unable to properly fit the conductance curves, while the two-gap one accounts remarkably well for the shape of the whole experimental dI/dV vs. V curves. These results give direct evidence of two nodeless gaps in the superconducting state of ReFeAsO1-xFx (Re = La, Sm): a small gap, Delta1, smaller than the BCS value (2Delta1/kBTc ~ 2.2 - 3.2) and a much larger gap Delta2 which gives a ratio 2Delta2/kBTc ~ 6.5 - 9. In Sm-1111 both gaps close at the same temperature, very similar to the bulk Tc, and follow a BCS-like behaviour, while in La-1111 the situation is more complex, the temperature dependence of the gaps showing remarkable deviations from the BCS behaviour at T close to Tc. The normal-state conductance reproducibly shows an unusual, but different, shape in La-1111 and Sm-1111 with a depression or a hump at zero bias, respectively. These structures survive up to T* ~ 140 K, close to the temperatures at which structural and magnetic transitions occur in the parent, undoped compound.
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