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Register a new userQuasifission dynamics and stability of superheavy systems
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Recent experiments revealed intriguing similarities in the $^{64}$Ni+$^{207}$Pb, $^{132}$Xe+$^{208}$Pb, and $^{238}$U+$^{238}$U reactions at energies around the Coulomb barrier. The experimental data indicate that for all systems substantial energy dissipation takes place, in the first stage of the reaction, although the number of transferred nucleons is small. On the other hand, in the second stage, a large number of nucleons are transferred with small friction and small consumption of time. To understand the observed behavior, various reactions were analyzed based on the microscopic time-dependent Hartree-Fock (TDHF) theory. From a systematic analysis for $^{40,48}$Ca+$^{124}$Sn, $^{40}$Ca+$^{208}$Pb, $^{40}$Ar+$^{208}$Pb, $^{58}$Ni+$^{208}$Pb, $^{64}$Ni+$^{238}$U, $^{136}$Xe+ $^{198}$Pt, and $^{238}$U+$^{238}$U reactions, we find that TDHF reproduces well the measured trends. In addition, the Balian-Veneroni variational principle is applied to head-on collisions of $^{238}$U+$^{238}$U, and the variance of the fragment masses is compared with the experimental data, showing significant improvement. The underlying reaction mechanisms and possible future studies are discussed.
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The synthesis of superheavy elements stimulates the effort to study the peculiarities of the complete fusion with massive nuclei and to improve theoretical models in order to extract knowledge about reaction mechanism in heavy ion collisions at low energies. We compare the theoretical results of the compound nucleus (CN) formation and evaporation residue (ER) cross sections obtained for the $^{48}$Ca+$^{248}$Cm and $^{58}$Fe+$^{232}$Th reactions leading to the formation of the isotopes A=296 and A=290, respectively, of the new superheavy element Lv (Z=116). The ER cross sections, which can be measured directly, are determined by the complete fusion and survival probabilities of the heated and rotating compound nucleus. That probabilities can not be measured unambiguously but the knowledge about them is important to study the formation mechanism of the observed products. For this aim, the $^{48}$Ca+$^{249}$Cf and $^{64}$Ni+$^{232}$Th reactions have been considered too. The use of the mass values of superheavy nuclei calculated in the framework of the macroscopic-microscopic model by Warsaw group leads to smaller ER cross section for all of the reactions (excluding the $^{64}$Ni+$^{232}$Th reaction) in comparison with the case of using the masses calculated by Peter Moller {it et al}.
The internal conversion coefficients for the elements 104 <= Z <= 126 are presented.
The internal conversion coefficients (ICC) were calculated for all atomic subshells of the elements with 104<=Z<=126, the E1...E4, M1...M4 multipolarities and the transition energies between 10 and 1000 keV. The atomic screening was treated in the relativistic Hartree-Fock-Slater model. The Tables comprising almost 90000 subshell and total ICC were recently deposited at LANL preprint server.
The angular distributions of fission fragments for the $^{32}$S+$^{184}$W reaction at center-of-mass energies of 118.8, 123.1, 127.3, 131.5, 135.8, 141.1 and 144.4 MeV were measured. The experimental fission excitation function is obtained. The fragment angular anisotropy ($mathcal{A}_{rm exp}$) is found by extrapolating the each fission angular distributions. The measured fission cross sections of the $^{32}$S+$^{182,184}$W reaction are decomposed into fusion-fission, quasifission and fast fission contributions by the dinuclear system model. The total evaporation residue excitation function for the $^{32}$S+$^{184}$W reaction calculated in the framework of the advanced statistical model is in good agreement with the available experimental data up to about $E_{rm c.m.}approx 160$ MeV. The theoretical descriptions of the experimental capture excitation functions for both reactions and quantities $K_0^2$, $<ell^2>$ and $mathcal{A}_{rm exp}$ which characterize angular distributions of the fission products were performed by the same partial capture cross sections at the considered range of beam energy.
Potential energy surfaces and fission barriers of superheavy nuclei are analyzed in the macroscopic-microscopic model. The Lublin-Strasbourg Drop (LSD) is used to obtain the macroscopic part of the energy, whereas the shell and pairing energy corrections are evaluated using the Yukawa-folded potential. A standard flooding technique has been used to determine the barrier heights. It was shown the Fourier shape parametrization containing only three deformation parameters reproduces well the nuclear shapes of nuclei on their way to fission. In addition, the non-axial degree of freedom is taken into account to describe better the form of nuclei around the ground state and in the saddles region. Apart from the symmetric fission valley, a new very asymmetric fission mode is predicted in most superheavy nuclei. The fission fragment mass distributions of considered nuclei are obtained by solving the 3D Langevin equations.
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