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Register a new userLimits on dynamically generated spin-orbit coupling: Absence of $l=1$ Pomeranchuk instabilities in metals
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Added by
Mathias S. Scheurer
Publication date
2016
fields
Physics
and research's language is
English
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An ordered state in the spin sector that breaks parity without breaking time-reversal symmetry, i.e., that can be considered as dynamically generated spin-orbit coupling, was proposed to explain puzzling observations in a range of different systems. Here we derive severe restrictions for such a state that follow from a Ward identity related to spin conservation. It is shown that $l=1$ spin-Pomeranchuk instabilities are not possible in non-relativistic systems since the response of spin-current fluctuations is entirely incoherent and non-singular. This rules out relativistic spin-orbit coupling as an emergent low-energy phenomenon. We illustrate the exotic physical properties of the remaining higher angular momentum analogues of spin-orbit coupling and derive a geometric constraint for spin-orbit vectors in lattice systems.
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We perform a microscropic analysis of how the constraints imposed by conservation laws affect $q=0$ Pomeranchuk instabilities in a Fermi liquid. The conventional view is that these instabilities are determined by the static interaction between low-energy quasiparticles near the Fermi surface, in the limit of vanishing momentum transfer $q$. The condition for a Pomeranchuk instability is set by $F^{c(s)}_l =-1$, where $F^{c(s)}_l$ (a Landau parameter) is a properly normalized partial component of the anti-symmetrized static interaction $F(k,k+q; p,p-q)$ in a charge (c) or spin (s) sub-channel with angular momentum $l$. However, it is known that conservation laws for total spin and charge prevent Pomeranchuk instabilities for $l=1$ spin- and charge- current order parameters. Our study aims to understand whether this holds only for these special forms of $l=1$ order parameters, or is a more generic result. To this end we perform a diagrammatic analysis of spin and charge susceptibilities for charge and spin density order parameters, as well as perturbative calculations to second order in the Hubbard $U$. We argue that for $l=1$ spin-current and charge-current order parameters, certain vertex functions, which are determined by high-energy fermions, vanish at $F^{c(s)}_{l=1}=-1$, preventing a Pomeranchuk instability from taking place. For an order parameter with a generic $l=1$ form-factor, the vertex function is not expressed in terms of $F^{c(s)}_{l=1}$, and a Pomeranchuk instability does occur when $F^{c(s)}_1=-1$. We argue that for other values of $l$, a Pomeranchuk instability occurs at $F^{c(s)}_{l} =-1$ for an order parameter with any form-factor
In contrast to conventional assumptions, we show that the Dzyaloshinskii-Moriya interaction can be of non-relativistic origin, in particular in materials with a non-collinear magnetic configuration, where non-relativistic contributions can dominate over spin-orbit effects. The weak antiferromagnetic phase of Mn$_{3}$Sn is used to illustrate these findings. Using electronic structure theory as a conceptual platform, all relevant exchange interactions are derived for a general, non-collinear magnetic state. It is demonstrated that non-collinearity influences all three types of exchange interaction and that physically distinct mechanisms, which connect to electron- and spin-density and currents, may be used as a general way to analyze and understand magnetic interactions of the solid state.
In the present paper we extend the method to detect Pomeranchuk instabilities in lattice systems developed in previous works to study more general situations. The main result presented here is the extension of the method to include finite temperature effects, which allows to compute critical temperatures as a function of interaction strengths and density of carriers. Furthermore, it can be applied to multiband problems which would be relevant to study systems with spin/color degrees of freedom. Altogether, the present extended version provides a potentially powerful technique to investigate microscopic realistic models relevant to e.g. the Fermi liquid to nematic transition extensively studied in connection with different materials such as cuprates, ruthenates, etc.
Motivated by the recently synthesized insulating nickelate Ni$_2$Mo$_3$O$_8$, which has been reported to have an unusual non-collinear magnetic order of Ni$^{2+}$ $S=1$ moments with a nontrivial angle between adjacent spins, we construct an effective spin-1 model on the honeycomb lattice, with the exchange parameters determined with the help of first principles electronic structure calculations. The resulting bilinear-biquadratic model, supplemented with the realistic crystal-field induced anisotropy, favors the collinear Neel state. We find that the crucial key to explaining the observed noncollinear spin structure is the inclusion of the Dzyaloshinskii--Moriya (DM) interaction between the neighboring spins. By performing the variational mean-field and linear spin-wave theory (LSWT) calculations, we determine that a realistic value of the DM interaction $Dapprox 2.78$ meV is sufficient to quantitatively explain the observed angle between the neighboring spins. We furthermore compute the spectrum of magnetic excitations within the LSWT and random-phase approximation (RPA) which should be compared to future inelastic neutron measurements.
Motivated by the recent experiments on the kagome metals $Atext{V}_3text{Sb}_5$ with $A=text{K}, text{Rb}, text{Cs}$, which see onset of charge density wave (CDW) order at $sim$ $100$ K and superconductivity at $sim$ $1$ K, we explore the onset of superconductivity, taking the perspective that it descends from a parent CDW state. In particular, we propose that the pairing comes from the Pomeranchuk fluctuations of the reconstructed Fermi surface in the CDW phase. This scenario naturally explains the large separation of energy scale from the parent CDW. Remarkably, the phase diagram hosts the double-dome superconductivity near two reconstructed Van Hove singularities. These singularities occur at the Lifshitz transition and the quantum critical point of the parent CDW. The first dome is occupied by the $d_{xy}$-wave nematic spin-singlet superconductivity. Meanwhile, the $(s+d_{x^2-y^2})$-wave nematic spin-singlet superconductivity develops in the second dome. Our work sheds light on an unconventional pairing mechanism with strong evidences in the kagome metals $Atext{V}_3text{Sb}_5$.
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