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Register a new userRadiative lifetimes of dipolar excitons in double quantum-wells
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Spatially indirect excitons in semiconducting double quantum wells have been shown to exhibit rich collective many-body behavior that result from the nature of the extended dipole-dipole interactions between particles. For many spectroscopic studies of the emission from a system of such indirect excitons, it is crucial to separate the single particle properties of the excitons from the many-body effects arising from their mutual interactions. In particular, knowledge of the relation between the emission energy of indirect excitons and their radiative lifetime could be highly beneficial for control, manipulation, and analysis of such systems. Here we study a simple analytic approximate relation between the radiative lifetime of indirect excitons and their emission energy. We show, both numerically and experimentally, the validity and the limits of this approximate relation. This relation between the emission energy and the lifetime of indirect excitons can be used to tune and determine their lifetime and their resulting dynamics without the need of directly measuring it, and as a tool for design of indirect exciton based devices.
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We investigate the transport of dipolar indirect excitons along the growth plane of polar (Al,Ga)N/GaN quantum well structures by means of spatially- and time-resolved photoluminescence spectroscopy. The transport in these strongly disordered quantum wells is activated by dipole-dipole repulsion. The latter induces an emission blue shift that increases linearly with exciton density, whereas the radiative recombination rate increases exponentially. Under continuous, localized excitation, we measure a continuous red shift of the emission, as excitons propagate away from the excitation spot. This shift corresponds to a steady-state gradient of exciton density, measured over several tens of micrometers. Time-resolved micro-photoluminescence experiments provide information on the dynamics of recombination and transport of dipolar excitons. We account for the ensemble of experimental results by solving the nonlinear drift-diffusion equation. Quantitative analysis suggests that in such structures, exciton propagation on the scale of 10 to 20 microns is mainly driven by diffusion, rather than by drift, due to the strong disorder and the presence of nonradiative defects. Secondary exciton creation, most probably by the intense higher-energy luminescence, guided along the sample plane, is shown to contribute to the exciton emission pattern on the scale up to 100 microns. The exciton propagation length is strongly temperature dependent, the emission being quenched beyond a critical distance governed by nonradiative recombination.
Resonance dielectric response of excitons is studied for the high-quality GaAs/InGaAs heterostructures with wide asymmetric quantum wells (QWs). To highlight effects of the QW asymmetry, we have grown and studied several heterostructures with nominally square QWs as well as with triangle-like QWs. Several quantum confined exciton states are experimentally observed as narrow exciton resonances with various profiles. A standard approach for the phenomenological analysis of the profiles is generalized by introducing of different phase shifts for the light waves reflected from the QWs at different exciton resonances. Perfect agreement of the phenomenological fit to the experimentally observed exciton spectra for high-quality structures allowed us to obtain reliable parameters of the exciton resonances including the exciton transition energies, the radiative broadenings, and the phase shifts. A direct numerical solution of Schr{o}dinger equation for the heavy-hole excitons in asymmetric QWs is used for microscopic modeling of the exciton resonances. Remarkable agreement with the experiment is achieved when the effect of indium segregation during the heterostructure growth is taken into account. The segregation results in a modification of the potential profile, in particular, in an asymmetry of the nominally square QWs.
Emergence of algebraic quasi-long-range order is a key feature of superfluid phase transitions at two dimensions. For this reduced dimensionality interactions prevent Bose-Einstein condensation with true long range order, at any finite temperature. Here, we report the occurence of algebraic order in a strongly interacting quantum liquid formed by dipolar excitons confined in a bilayer semiconductor heterostructure. We observe a transition from exponential to algebraic decay of the excitons temporal coherence, accompanied by a universal scaling behaviour of the equation of state. Our results provide strong evidence for a Berezinskii-Kosterlitz-Thouless (BKT) transition in a multi-component boson-like system governed by strong dipolar interactions.
In this work we investigate the different states of a system of spin-1 bosons in two potential wells connected by tunneling, with spin-dependent interaction. The model utilizes the well-known Bose-Hubbard Hamiltonian, adding a local interaction term that depends on the modulus of the total spin in a well, favoring a high- or low-spin state for different signs of the coupling constant. We employ the concept of fidelity to detect critical values of parameters for which the ground state undergoes significant changes. The nature of the states is investigated through evaluation of average occupation numbers in the wells and of spin correlations. A more detailed analysis is done for a two-particle system, but a discussion of the three-particle case and some results for larger numbers are also presented.
The formation of a dense Bose-Einstein condensate in dark spin states of two-dimensional dipolar excitons is shown to be driven by a dynamical transition to the long-lived dark states. The condensate is stabilized by strong dipole-dipole interactions up to densities high enough for a dark quantum liquid to form. The persistence of dark condensation was observed in recent experiments. A model describing the non-equilibrium dynamics of externally driven coupled dark and bright condensates reproduces the step-like dependence of the exciton density on the pump power or on temperature. This unique condensate dynamics demonstrates the possibility of observing new unexpected collective phenomena in coupled condensed Bose systems, where the particle number is not conserved.
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