Subscribe to the gold package and get unlimited access to Shamra Academy
Register a new userSignal line shapes of Fourier transform cavity-enhanced frequency modulation spectroscopy with optical frequency combs
90
0
0.0
(
0
)
Added by
Aleksandra Foltynowicz
Publication date
2016
fields
Physics
and research's language is
English
Ask ChatGPT about the research
No Arabic abstract
We present a thorough analysis of the signal line shapes of Fourier transform-based noise-immune cavity-enhanced optical frequency comb spectroscopy (NICE-OFCS). We discuss the signal dependence on the ratio of the modulation frequency, f${_m}$, to the molecular line width, {Gamma}. We compare a full model of the signals and a simplified absorption-like analytical model that has high accuracy for low f${_m}$/{Gamma} ratios and is much faster to compute. We verify the theory experimentally by measuring and fitting NICE-OFCS spectra of CO${_2}$ at 1575 nm using a system based on an Er:fiber femtosecond laser and a cavity with a finesse of ~11000.
rate research
Read More
Fourier transform spectroscopy based on incoherent light sources is a well-established tool in research fields from molecular spectroscopy and atmospheric monitoring to material science and biophysics. It provides broadband molecular spectra and information about the molecular structure and composition of absorptive media. However, the spectral resolution is fundamentally limited by the maximum delay range ({Delta}$_{max}$) of the interferometer, so acquisition of high-resolution spectra implies long measurement times and large instrument size. We overcome this limit by combining the Fourier transform spectrometer with an optical frequency comb and measuring the intensities of individual comb lines by precisely matching the {Delta}$_{max}$ to the comb line spacing. This allows measurements of absorption lines narrower than the nominal (optical path-limited) resolution without ringing effects from the instrumental lineshape and reduces the acquisition time and interferometer length by orders of magnitude.
Kerr optical frequency combs generated in a coherently driven Kerr nonlinear resonator has the potential for a wide range of applications. However, in a single cavity which is a widely adopted configuration for Kerr optical frequency combs generation, modulation instability is suppressed in normal dispersion regime and the pump-to-comb conversion efficiency is extremely low for a single dissipative Kerr soliton in anomalous dispersion regime. Dual-coupled cavities have been proposed to generate Kerr optical frequency combs in normal dispersion regime, and have potential to remarkably increase conversion efficiency for Kerr optical frequency combs. Here, we investigate modulation instability and Kerr optical frequency-comb formation in dual-coupled cavities. Based on solutions of the continuous-wave steady state, we obtain a quadric algebraic equation describing the modulation instability gain, and we find that it is intensely influenced by the group velocity mismatch between the two cavities. Our numerical simulations demonstrate that platicons can be generated via pump scanning scheme for the case that both the two cavities possess normal dispersion, and a single dissipative Kerr soliton can be generated in the cavity with anomalous dispersion while the dispersion of the other cavity is normal. Our analysis of modulation instability provides a powerful tool for Kerr optical frequency-comb generation via pump modulation and cavity detuning tuning scheme in dual-coupled cavities.
We demonstrate a method for accurately locking the frequency of a continuous-wave laser to an optical frequency comb in conditions where the signal-to-noise ratio is low, too low to accommodate other methods. Our method is typically orders of magnitude more accurate than conventional wavemeters and can considerably extend the usable wavelength range of a given optical frequency comb. We illustrate our method by applying it to the frequency control of a dipole lattice trap for an optical lattice clock, a representative case where our method provides significantly better accuracy than other methods.
Presented here is the development and demonstration of a tunable cavity-enhanced terahertz frequency-domain optical Hall effect technique. The cavity consists of at least one fixed and one tunable Fabry-Perot resonator. The approach is suitable for enhancement of the optical signatures produced by the optical Hall effect in semi-transparent conductive layer structures with plane parallel interfaces. The physical principle is the constructive interference of electric field components that undergo multiple optical Hall effect induced polarization rotations upon multiple light passages through the conductive layer stack. Tuning one of the cavity parameters, such as the external cavity thickness, permits shifting of the frequencies of the constructive interference, and enhancement of the optical signatures produced by the optical Hall effect can be obtained over large spectral regions. A cavity-tuning optical stage and gas flow cell are used as examples of instruments that exploit tuning an external cavity to enhance polarization changes in a reflected terahertz beam. Permanent magnets are used to provide the necessary external magnetic field. Conveniently, the highly reflective surface of a permanent magnet can be used to create the tunable external cavity. The signal enhancement allows the extraction of the free charge carrier properties of thin films, and can eliminate the need for expensive super-conducting magnets. Furthermore, the thickness of the external cavity establishes an additional independent measurement condition, similar to, for example, the magnetic field strength, terahertz frequency, and angle of incidence. A high electron mobility transistor structure and epitaxial graphene are studied as examples. We discuss the theoretical background, instrument design, data acquisition, and data analysis procedures.
Broadband precision spectroscopy is indispensable for providing high fidelity molecular parameters for spectroscopic databases. We have recently shown that mechanical Fourier transform spectrometers based on optical frequency combs can measure broadband high-resolution molecular spectra undistorted by the instrumental line shape (ILS) and with a highly precise frequency scale provided by the comb. The accurate measurement of the power of the comb modes interacting with the molecular sample was achieved by acquiring single-burst interferograms with nominal resolution precisely matched to the comb mode spacing. Here we give a full theoretical description of this sub-nominal resolution method and describe in detail the experimental and numerical steps needed to retrieve ILS-free molecular spectra, i.e. with ILS-induced distortion below the noise level. We investigate the accuracy of the transition line centers retrieved by fitting to the absorption lines measured using this method. We verify the performance by measuring an ILS-free cavity-enhanced low-pressure spectrum of the 3{ u}1+{ u}3 band of CO2. We observe and quantify collisional narrowing of absorption line shape, for the first time with a comb-based spectroscopic technique. Thus retrieval of line shape parameters with accuracy not limited by the Voigt profile is now possible for entire absorption bands acquired simultaneously.
Log in to be able to interact and post comments
comments
Fetching comments
Sign in to be able to follow your search criteria
