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Experimental observation of coherent cavity soliton frequency combs in silica microspheres

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 Added by Karen Webb
 Publication date 2016
  fields Physics
and research's language is English




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We report on the experimental observation of coherent cavity soliton frequency combs in silica microspheres. Specifically, we demonstrate that careful alignment of the microsphere relative to the coupling fiber taper allows for the suppression of higher-order spatial modes, reducing mode interactions and enabling soliton formation. Our measurements show that the temporal cavity solitons have sub-100-fs durations, exhibit considerable Raman self-frequency shift, and generally come in groups of three or four, occasionally with equidistant spacing in the time domain. RF amplitude noise measurements and spectral interferometry confirm the high coherence of the observed soliton frequency combs, and numerical simulations show good agreement with experiments.



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The field of micro-cavity based frequency combs, or micro-combs[1,2], has recently witnessed many fundamental breakthroughs[3-19] enabled by the discovery of temporal cavity-solitons, self-localised waves sustained by a background of radiation usually containing 95% of the total power[20]. Simple methods for their efficient generation and control are currently researched to finally establish micro-combs as out-of-the-lab widespread tools[21]. Here we demonstrate micro-comb laser cavity-solitons, an intrinsically highly-efficient, background free class of solitary waves. Laser cavity-solitons have underpinned key breakthroughs in semiconductor lasers[22,23] and photonic memories[24-26]. By merging their properties with the physics of both micro-resonators[1,2] and multi-mode systems[27], we provide a new paradigm for the generation and control of self-localised pulses in micro-cavities. We demonstrate 50 nm wide soliton combs induced with average powers one order of magnitude lower than those typically required by state-of-the-art approaches[26]. Furthermore, we can tune the repetition-rate to well over a megahertz with no-active feedback.
With demonstrated applications ranging from metrology to telecommunications, soliton microresonator frequency combs have emerged over the past decade as a remarkable new technology. However, standard implementations only allow for the generation of combs whose repetition rate is tied close to the fundamental resonator free-spectral range (FSR), offering little or no dynamic control over the comb line spacing. Here we propose and experimentally demonstrate harmonic and rational harmonic driving as novel techniques that allow for the robust generation of soliton frequency combs with discretely adjustable frequency spacing. By driving an integrated Kerr microresonator with a periodic train of picosecond pulses whose repetition rate is set close to an integer harmonic of the 3.23 GHz cavity FSR, we deterministically generate soliton frequency combs with frequency spacings discretely adjustable between 3.23 GHz and 19.38 GHz. More remarkably, we also demonstrate that driving the resonator at rational fractions of the FSR allows for the generation of combs whose frequency spacing corresponds to an integer harmonic of the pump repetition rate. By measuring the combs radio-frequency spectrum, we confirm operation in the low-noise soliton regime with no supermode noise. The novel techniques demonstrated in our work provide new degrees of freedom for the design of synchronously pumped soliton frequency combs.
Normal mode splitting is observed in a cavity QED system, in which nitrogen vacancy centers in diamond nanocrystals are coupled to whispering gallery modes in a silica microsphere. The composite nanocrystal-microsphere system takes advantage of the exceptional spin properties of nitrogen vacancy centers as well as the ultra high quality factor of silica microspheres. The observation of the normal mode splitting indicates that the dipole optical interaction between the relevant nitrogen vacancy center and whispering gallery mode has reached the strong coupling regime of cavity QED.
A tunable, all-optical, coupling method has been realized for a high-textit{Q} silica microsphere and an optical waveguide. By means of a novel optical nanopositioning method, induced thermal expansion of an asymmetric microsphere stem for laser powers up to 171~mW has been observed and used to fine tune the microsphere-waveguide coupling. Microcavity displacements ranging from (0.612~$pm$~0.13) -- (1.5 $pm$ 0.13) $mu$m and nanometer scale sensitivities varying from (2.81 $pm$ 0.08) -- (7.39 $pm$ 0.17) nm/mW, with an apparent linear dependency of coupling distance on stem laser heating, were obtained. Using this method, the coupling was altered such that different coupling regimes could be explored for particular samples. This tunable coupling method, in principle, could be incorporated into lab-on-a-chip microresonator systems, photonic molecule systems, and other nanopositioning frameworks.
Electro-optic frequency combs were employed to rapidly interrogate an optomechanical sensor, demonstrating spectral resolution substantially exceeding that possible with a mode-locked frequency comb. Frequency combs were generated using an integrated-circuit-based direct digital synthesizer and utilized in a self-heterodyne configuration. Unlike approaches based upon laser locking or sweeping, the present approach allows rapid, parallel measurements of full optical cavity modes, large dynamic range of sensor displacement, and acquisition across a wide frequency range between DC and 500 kHz. In addition to being well suited to measurements of cavity optomechanical sensors, this optical frequency comb-based approach can be utilized for interrogation in a wide range of physical and chemical sensors.
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