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Register a new userSpatially and spectrally resolved quantum path interference with chirped driving pulses
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Added by
Stefanos Carlstr\\\"om
Publication date
2016
fields
Physics
and research's language is
English
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We measure spectrally and spatially resolved high-order harmonics generated in argon using chirped multi-cycle laser pulses. Using a stable, high-repetition rate laser we observe detailed interference structures in the far-field. The structures are of two kinds; off-axis interference from the long trajectory only and on-axis interference including the short and long trajectories. The former is readily visible in the far-field spectrum, modulating both the spectral and spatial profile. To access the latter, we vary the chirp of the fundamental, imparting different phases on the different trajectories, thereby changing their relative phase. Using this method together with an analytical model, we are able to explain the on-axis behaviour and access the dipole phase parameters for the short ((alpha_s)) and long ((alpha_l)) trajectories. The extracted results compare very well with phase parameters calculated by solving the time-dependent Schrodinger equation. Going beyond the analytical model, we are also able to successfully reproduce the off-axis interference structure.
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We investigate the electron quantum path interference effects during high harmonic generation in atomic gas medium driven by ultrashort chirped laser pulses. To achieve that, we identify and vary the different experimentally relevant control parameters of such a driving laser pulse influencing the high harmonic spectra. Specifically, the impact of the pulse duration, peak intensity and instantaneous frequency is studied in a self-consistent manner based on Lewenstein formalism. Simulations involving macroscopic propagation effects are also considered. The study aims to reveal the microscopic background behind a variety of interference patterns capturing important information both about the fundamental laser field and the generation process itself. The results provide guidance towards experiments with chirp control as a tool to unravel, explain and utilize the rich and complex interplay between quantum path interferences including the tuning of the periodicity of the intensity dependent oscillation of the harmonic signal, and the curvature of spectrally resolved Maker fringes.
NOON state interference (NOON-SI) is a powerful tool to improve the phase sensing precision, and plays an important role in quantum measurement. In most of the previous NOON-SI experiments, the measurements were performed in time domain where the spectral information of the involved photons was integrated and lost during the measurement. In this work, we experimentally measured the joint spectral intensities (JSIs) at different positions of the interference patterns in both time and frequency domains. It was observed that the JSIs were phase-dependent and show odd (even)-number patterns at $0$ ($pi$) phase shift; while no interference appeared in time domain measurement, the interference pattern clearly appeared in frequency domain. To our best knowledge, the latter is the first observation of the spectrally resolved NOON state interference, which provides alternative information that cannot be extracted from the time-domain measurement. To explore its potential applications, we considered the interferometric sensing with our setup. From the Fisher information-based analysis, we show that the spectrally resolved NOON-SI has a better performance at non-zero-delay position than its non-spectrally resolved counterpart. The spectrally resolved NOON-SI scheme may be useful for quantum metrology applications such as quantum phase sensing, quantum spectroscopy, and remote synchronization.
We report on the dynamics of ultracold collisions induced by near-resonant frequency-chirped light. A series of identical chirped pulses, separated by a variable delay, is applied to an ultracold sample of 85Rb, and the rate of inelastic trap-loss collisions is measured. For small detunings of the chirped light below the atomic resonance, we observe that the rate of collisions induced by a given pulse can be increased by the presence of an earlier pulse. We attribute this to the enhancement of short-range collisional flux by the long-range excitation of atom pairs to an attractive molecular potential. For larger detunings and short delays, we find that a leading pulse can suppress the rate of collisions caused by a following pulse. This is due to a depletion of short-range atom pairs by the earlier pulse. Comparison of our data to classical Monte-Carlo simulations of the collisions yields reasonable agreement.
We introduce and implement an interferometric technique based on chirped femtosecond laser pulses and nonlinear optics. The interference manifests as a high-visibility (> 85%) phase-insensitive dip in the intensity of an optical beam when the two interferometer arms are equal to within the coherence length of the light. This signature is unique in classical interferometry, but is a direct analogue to Hong-Ou-Mandel quantum interference. Our technique exhibits all the metrological advantages of the quantum interferometer, but with signals at least 10^7 times greater. In particular we demonstrate enhanced resolution, robustness against loss, and automatic dispersion cancellation. Our interferometer offers significant advantages over previous technologies, both quantum and classical, in precision time delay measurements and biomedical imaging.
Pairs of photons entangled in their time-frequency degree of freedom are of great interest in quantum optics research and applications, due to their relative ease of generation and their high capacity for encoding information. Here we analyze, both theoretically and experimentally, the behavior of phase-insensitive spectrally-resolved interferences arising from two pairs of time-frequency entangled photons. At its core, this is a multimode entanglement swapping experiment, whereby a spectrally resolved joint measurement on the idler photons from both pairs results in projecting the signal photons onto a Bell state whose form depends on the measurement outcome. Our analysis is a thorough exploration of what can be achieved using time-frequency entanglement and spectrally-resolved Bell-state measurements.
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