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Magnetic hyperfine structure of the ground-state doublet in highly charged ions $^{229}$Th$^{89+,87+}$ and the Bohr-Weisskopf effect

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 Added by Eugene Tkalya
 Publication date 2016
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and research's language is English




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The magnetic hyperfine (MHF) structure of the $5/2^+$(0.0 eV) ground state and the low-lying $3/2^+$(7.8 eV) isomeric state of the $^{229}$Th nucleus in highly charged ions Th$^{89+}$ and Th$^{87+}$ is calculated. The distribution of the nuclear magnetization (the Bohr-Weisskopf effect) is accounted for in the framework of the collective nuclear model with the wave functions of the Nilsson model for the unpaired neutron. The deviations of the MHF structure for the ground and isomeric states from their values in the model of point-like nuclear magnetic dipole are calculated. The influence of the mixing of the states with the same quantum number $F$ on the energy of sublevels is studied. Taking into account the mixing of states, the probabilities of the transitions between the components of MHF structure are found.



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A method is proposed to determine the $M1$ nuclear transition amplitude and hence the lifetime of the nuclear clock transition between the low-lying ($sim 8$ eV) first isomeric state and the ground state of $^{229}$Th from a measurement of the ground-state $g$ factor of few-electron $^{229}$Th ions. As a tool, the effect of nuclear hyperfine mixing (NHM) in highly charged $^{229}$Th-ions such as $^{229}$Th$^{89+}$ or $^{229}$Th$^{87+}$ is utilized. The ground-state-only $g$-factor measurement would also provide first experimental evidence of NHM in atomic ions. Combining the measurements for H-, Li-, and B-like $^{229}$Th ions has a potential to improve the initial result for a single charge state and to determine the nuclear magnetic moment to a higher accuracy than that of the currently accepted value. The calculations include relativistic, interelectronic-interaction, QED, and nuclear effects.
$^{229}$Th is a promising candidate for developing a nuclear optical clock and searching the new physics beyond the standard model. Accurate knowledge of the nuclear properties of $^{229}$Th is very important. In this work, we calculate hyperfine-structure constants for the first four states of $^{229}$Th$^{3+}$ using the relativistic coupled-cluster method based on the Gauss basis set. The no-pair Dirac-Coulomb-Breit Hamiltonian with the lowest-order quantum electrodynamics (QED) correction is the starting point, together with all linear and non-linear terms of single and double excitations are included in coupled-cluster calculation. With the measured value of the hyperfine-structure constants [Phys. Rev. Lett. 106. 223001(2011)], we get the magnetic dipole moment, $mu=0.359(9)$, and the electric quadrupole moment, $Q=2.95(7)$, of the $^{229}$Th nucleus. Our magnetic dipole moment is perfectly consistent with the recommended values, $mu=0.360(7)$, from the all-order calculation by Safronova textit{et. al.}[Phys.Rev.A 88, 060501 (2013)], but our electric quadrupole moment is smaller than their recommended value, $Q=3.11(6)$, about 5%. Our results show that the non-linear terms of single and double excitations, which were not included in the all-order calculation by Safronova textit{et. al.}, are very crucial to produce a precise $Q$ value of $^{229}$Th. Additionally, we also present magnetic octupole hyperfine-structure constants and some important non-diagonal hyperfine transition matrix elements, which are required for further extracting the magnetic octupole moment $Omega$ of $^{229}$Th nucleus.
305 - V.I. Isakov 2017
Electromagnetic properties of the deformed neutron-odd nucleus $^{229}$Th are investigated in the framework of the unified model, with primary emphasis upon the properties of the low-lying isomeric state.
The hyperfine structure (hfs) of electron levels of $^{238}_{92}$U ions with the nucleus excited in the low-lying rotational $2^+$ state with an energy $E_{2^+} = 44.91$ keV is investigated. In hydrogenlike uranium, the hfs splitting for the $1s_{1/2}$-ground state of the electron constitutes 1.8 eV. The hyperfine-quenched (hfq) lifetime of the $1s2p ^3P_0$ state has been calculated for heliumlike $^{238}_{92}$U and was found to be two orders of magnitude smaller than for the ion with the nucleus in the ground state. The possibility of a precise determination of the nuclear $g_r$ factor for the rotational $2^+$ state by measurements of the hfq lifetime is discussed.
127 - D.L. Moskovkin , V.M. Shabaev , 2007
The fully relativistic theory of the Zeeman splitting of the $(1s)^2 2s$ hyperfine-structure levels in lithiumlike ions with $Z=6 - 32$ is considered for the magnetic field magnitude in the range from 1 to 10 T. The second-order corrections to the Breit -- Rabi formula are calculated and discussed including the one-electron contributions as well as the interelectronic-interaction effects of order 1/Z. The 1/Z corrections are evaluated within a rigorous QED approach. These corrections are combined with other interelectronic-interaction, QED, nuclear recoil, and nuclear size corrections to obtain high-precision theoretical values for the Zeeman splitting in Li-like ions with nonzero nuclear spin. The results can be used for a precise determination of nuclear magnetic moments from $g$-factor experiments.
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