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Register a new userLevel sequence and splitting identification of closely-spaced energy levels by angle-resolved analysis of the fluorescence light
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The angular distribution and linear polarization of the fluorescence light following the resonant photoexcitation is investigated within the framework of the density matrix and second-order perturbation theory. Emphasis has been placed on signatures for determining the level sequence and splitting of intermediate (partially) overlapping resonances, if analyzed as a function of the photon energy of the incident light. Detailed computations within the multiconfiguration Dirac-Fock method have been performed especially for the $1s^{2}2s^{2}2p^{6}3s;, J_{i}=1/2 ,+, gamma_{1} :rightarrow: (1s^{2}2s2p^{6}3s)_{1}3p_{3/2};, J=1/2, , 3/2 :rightarrow: 1s^{2}2s^{2}2p^{6}3s;, J_{f}=1/2 ,+, gamma_{2}$ photoexcitation and subsequent fluorescence emission of atomic sodium. A remarkably strong dependence of the angular distribution and linear polarization of the $gamma_{2}$ fluorescence emission is found upon the level sequence and splitting of the intermediate $(1s^{2}2s2p^{6}3s)_{1}3p_{3/2};, J=1/2, , 3/2$ overlapping resonances owing to their finite lifetime (linewidth). We therefore suggest that accurate measurements of the angular distribution and linear polarization might help identify the sequence and small splittings of closely-spaced energy levels, even if they can not be spectroscopically resolved.
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In this paper, we present experimental techniques to resolve the closely spaced hyperfine levels of a weak transition by eliminating the residual/partial two-photon Doppler broadening and cross-over resonances in a wavelength mismatched double resonance spectroscopy. The elimination of the partial Doppler broadening is based on velocity induced population oscillation (VIPO) and velocity selective saturation (VSS) effect followed by the subtraction of the broad background of the two-photon spectrum. Since the VIPO and VSS effect are the phenomena for near zero velocity group atoms, the subtraction gives rise to Doppler-free peaks and the closely spaced hyperfine levels of the $6text{P}_{3/2}$ state in Rb are well resolved. The double resonance experiment is conducted on $5text{S}_{1/2}rightarrow5text{P}_{3/2}$ strong transition (at 780~nm) and $5text{S}_{1/2}rightarrow6text{P}_{3/2}$ weak transition (at 420~nm) at room temperature.
In this review article we provide an overview of the field of atomic structure of light atoms in strong magnetic fields. There is a very rich history of this field which dates back to the very birth of quantum mechanics. At various points in the past significant discoveries in science and technology have repeatedly served to rejuvenate interest in atomic structure in strong fields, broadly speaking, resulting in three eras in the development of this field; the historical, the classical and the modern eras. The motivations for studying atomic structure have also changed significantly as time progressed. The review presents a chronological summary of the major advances that occurred during these eras and discusses new insights and impetus gained. The review is concluded with a description of the latest findings and the future prospects for one of the most remarkably cutting-edge fields of research in science today.
Anisotropic plasmon coupling in closely-spaced chains of Ag nanoparticles was visualized using the electron energy loss spectroscopy in a scanning transmission electron microscope. For dimers as the simplest chain, mapping the plasmon excitations with nanometers spatial resolution and 0.27 eV energy resolution intuitively identified two coupling plasmons. The in-phase mode redshifted from the ultraviolet region as the inter-particle spacing was reduced, reaching the visible range at 2.7 eV. Calculations based on the discrete dipole approximation confirmed its optical activeness, where the longitudinal direction was constructed as the path for light transportation. Two coupling paths were then observed in an inflexed 4-particle chain.
A quantum-mechanical formulation of energy transfer between closely-spaced surfaces is given. Coupling between the two surfaces arises from the atomic dipole-dipole interaction involving transverse-photon exchange. The exchange of photons at resonance greatly enhances the radiation transfer. The spacing (distance) dependence is derived for the quantum well - quantum well situation. The interaction between two planar quantum wells, separated by a gap is found to be proportional to the 4th power of the wavelength-to-gapwidth ratio and to the radiation tunneling factor for the evanescent waves. Expressions for the net power transfer, in the near-field regime, from hot to cold surface for this case is given and evaluated for representative materials. Computational modeling of selected, but realizable, emitter and detector structures and materials shows the benefits of both near-field and resonance coupling (e.g., with 0.1 micron gaps).
Electromagnetically induced transparency (EIT) is a well-known phenomenon due in part to its applicability to quantum devices such as quantum memories and quantum gates. EIT is commonly modeled with a three-level lambda system due to the simplicity of the calculations. However, this simplified model does not capture all the physics of EIT experiments with real atoms. We present a theoretical study of the effect of two closely-spaced excited states on EIT and off-resonance Raman transitions. We find that the coherent interaction of the fields with two excited states whose separation is smaller than their Doppler broadened linewidth can enhance the EIT transmission and broaden the width of the EIT peak. However, a shift of the two-photon resonance frequency for systems with transitions of unequal dipole strengths leads to a reduction of the maximum transparency that can be achieved when Doppler broadening is taken into account even under ideal conditions of no decoherence. As a result, complete transparency cannot be achieved in a vapor cell. Only when the separation between the two excited states is of the order of the Doppler width or larger can complete transparency be recovered. In addition, we show that off-resonance Raman absorption is enhanced and its resonance frequency is shifted. Finally, we present experimental EIT measurements on the D1 line of $^{85}$Rb that agree with the theoretical predictions when the interaction of the fields with the four levels is taken into account.
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