Do you want to publish a course? Click here

Evolution of the thermodynamic properties and inelastic neutron scattering intensities for spin-1/2 antiferromagnetic quantum rings

99   0   0.0 ( 0 )
 Publication date 2016
  fields Physics
and research's language is English




Ask ChatGPT about the research

This study examines the increasing complexity in the magnetic properties of small $n$ = 3, 4, 5, 6 spin-1/2 quantum rings. Using an exact diagonalization of the isotropic Heisenberg Hamiltonian with nearest and next-nearest neighbor interactions, the energy eigenstates, magnetic specific heat capacity, magnetic susceptibility, and inelastic neutron scattering structure factors are determined for variable next-nearest neighbor interactions. Here, it is shown that the presence of a complex spin-mixing, multiple ground states, and non-zero ground states greatly complicate the spin Hamiltonian. Overall, the energy eigenstates and structure factor intensities are presented in closed form, while the thermodynamic properties detail the effect of a crossing interaction in the rings. The goal of this work is to provide insight into the evolution of the magnetic properties and spin excitations within these systems.



rate research

Read More

We report detailed temperature-dependent inelastic neutron scattering and ab-initio lattice dynamics investigation of magnetic perovskites YCrO3 and LaCrO3. The magnetic neutron scattering from the Cr ions exhibits significant changes with temperature and dominates at low momentum transfer regime. Ab-inito calculations performed including magnetic interactions show that the effect of magnetic interaction is very signicant on the low- as well as high-energy phonon modes. We have also shown that the inelastic neutron spectrum of YCrO3 mimics the magnon spectrum from a G-type antiferromagnetic system, which is consistent with previously reported magnetic structure in the compound. The ab-initio lattice dynamics calculations in both the compounds exhibit anisotropic thermal expansion behaviour in the orthorhombic structure and predict negative thermal expansion along the crystallographic a-axis at low temperatures. We identify the anharmonic phonon modes responsible for this anamolous behaviour in LaCrO3 involving low-energy La vibrations and distortions of the CrO6 octahedra.
We have studied the longitudinal spin Seebeck effect in a polar antiferromagnet $alpha$-Cu$_{2}$V$_{2}$O$_{7}$ in contact with a Pt film. Below the antiferromagnetic transition temperature of $alpha$-Cu$_{2}$V$_{2}$O$_{7}$, spin Seebeck voltages whose magnetic field dependence is similar to that reported in antiferromagnetic MnF$_{2}$$mid$Pt bilayers are observed. Though a small weak-ferromagnetic moment appears owing to the Dzyaloshinskii-Moriya interaction in $alpha$-Cu$_{2}$V$_{2}$O$_{7}$, the magnetic field dependence of spin Seebeck voltages is found to be irrelevant to the weak ferromagnetic moments. The dependences of the spin Seebeck voltages on magnetic fields and temperature are analyzed by a magnon spin current theory. The numerical calculation of spin Seebeck voltages using magnetic parameters of $alpha$-Cu$_{2}$V$_{2}$O$_{7}$ determined by previous neutron scattering studies reveals that the magnetic-field and temperature dependences of the spin Seebeck voltages for $alpha$-Cu$_{2}$V$_{2}$O$_{7}$$mid$Pt are governed by the changes in magnon lifetimes with magnetic fields and temperature.
Antiferromagnetic insulators (AFIs) are of significant interest due to their potential to develop next-generation spintronic devices. One major effort in this emerging field is to harness AFIs for long-range spin information communication and storage. Here, we report a non-invasive method to optically access the intrinsic spin transport properties of an archetypical AFI {alpha}-Fe2O3 via nitrogen-vacancy (NV) quantum spin sensors. By NV relaxometry measurements, we successfully detect the time-dependent fluctuations of the longitudinal spin density of {alpha}-Fe2O3. The observed frequency dependence of the NV relaxation rate is in agreement with a theoretical model, from which an intrinsic spin diffusion constant of {alpha}-Fe2O3 is experimentally measured in the absence of external spin biases. Our results highlight the significant opportunity offered by NV centers in diagnosing the underlying spin transport properties in a broad range of high-frequency magnetic materials, which are challenging to access by more conventional measurement techniques.
Quantum states induced by single-atomic impurities are at the frontier of physics and material science. While such states have been reported in high-temperature superconductors and dilute magnetic semiconductors, they are unexplored in topological magnets which can feature spin-orbit tunability. Here we use spin-polarized scanning tunneling microscopy/spectroscopy (STM/S) to study the engineered quantum impurity in a topological magnet Co3Sn2S2. We find that each substituted In impurity introduces a striking localized bound state. Our systematic magnetization-polarized probe reveals that this bound state is spin-down polarized, in lock with a negative orbital magnetization. Moreover, the magnetic bound states of neighboring impurities interact to form quantized orbitals, exhibiting an intriguing spin-orbit splitting, analogous to the splitting of the topological fermion line. Our work collectively demonstrates the strong spin-orbit effect of the single-atomic impurity at the quantum level, suggesting that a nonmagnetic impurity can introduce spin-orbit coupled magnetic resonance in topological magnets.
Electrical manipulation of emergent phenomena due to nontrivial band topology is a key to realize next-generation technology using topological protection. A Weyl semimetal is a three-dimensional gapless system that hosts Weyl fermions as low-energy quasiparticles. It exhibits various exotic phenomena such as large anomalous Hall effect (AHE) and chiral anomaly, which have robust properties due to the topologically protected Weyl nodes. To manipulate such phenomena, the magnetic version of Weyl semimetals would be useful as a magnetic texture may provide a handle for controlling the locations of Weyl nodes in the Brillouin zone. Moreover, given the prospects of antiferromagnetic (AF) spintronics for realizing high-density devices with ultrafast operation, it would be ideal if one could electrically manipulate an AF Weyl metal. However, no report has appeared on the electrical manipulation of a Weyl metal. Here we demonstrate the electrical switching of a topological AF state and its detection by AHE at room temperature. In particular, we employ a polycrystalline thin film of the AF Weyl metal Mn$_3$Sn, which exhibits zero-field AHE. Using the bilayer device of Mn$_3$Sn and nonmagnetic metals (NMs), we find that an electrical current density of $sim 10^{10}$-$10^{11}$ A/m$^2$ in NMs induces the magnetic switching with a large change in Hall voltage, and besides, the current polarity along a bias field and the sign of the spin Hall angle $theta_{rm SH}$ of NMs [Pt ($theta_{rm SH} > 0$), Cu($theta_{rm SH} sim 0$), W ($theta_{rm SH} < 0$)] determines the sign of the Hall voltage. Notably, the electrical switching in the antiferromagnet is made using the same protocol as the one used for ferromagnetic metals. Our observation may well lead to another leap in science and technology for topological magnetism and AF spintronics.
comments
Fetching comments Fetching comments
mircosoft-partner

هل ترغب بارسال اشعارات عن اخر التحديثات في شمرا-اكاديميا