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Register a new userElectronic specific heat in BaFe$_{2-x}$Ni$_x$As$_2$
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We have systematically studied the low-temperature specific heat of the BaFe$_{2-x}$Ni$_x$As$_2$ single crystals covering the whole superconducting dome. Using the nonsuperconducting heavily overdoped x = 0.3 sample as a reference for the phonon contribution to the specific heat, we find that the normal-state electronic specific heats in the superconducting samples may have a nonlinear temperature dependence, which challenges previous results in the electron-doped Ba-122 iron-based superconductors. A model based on the presence of ferromagnetic spin fluctuations may explain the data between x = 0.1 and x = 0.15, suggesting the important role of Fermi-surface topology in understanding the normal-state electronic states.
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We have systematically studied the nematic fluctuations in the electron-doped iron-based superconductor BaFe$_{2-x}$Ni$_x$As$_2$ by measuring the in-plane resistance change under uniaxial pressure. While the nematic quantum critical point can be identified through the measurements along the (110) direction as studied previously, quantum and thermal critical fluctuations cannot be distinguished due to similar Curie-Weiss-like behaviors. Here we find that a sizable pressure-dependent resistivity along the (100) direction is present in all doping levels, which is against the simple picture of an Ising-type nematic model. The signal along the (100) direction becomes maximum at optimal doping, suggesting that it is associated with nematic quantum critical fluctuations. Our results indicate that thermal fluctuations from striped antiferromagnetic order dominate the underdoped regime along the (110) direction. We argue that either there is a strong coupling between the quantum critical fluctuations and the fermions, or more exotically, a higher symmetry may be present around optimal doping.
A series of 122 phase BaFe$_{2-x}$Ni$_x$As$_2$ ($x$ = 0, 0.055, 0.096, 0.18, 0.23) single crystals were grown by self flux method and a dome-like Ni doping dependence of superconducting transition temperature is discovered. The transition temperature $T_c^{on}$ reaches a maximum of 20.5 K at $x$ = 0.096, and it drops to below 4 K as $x$ $geq$ 0.23. The negative thermopower in the normal state indicates that electron-like charge carrier indeed dominates in this system. This Ni-doped system provides another example of superconductivity induced by electron doping in the 122 phase.
Inelastic neutron scattering measurements on Ba(Fe$_{0.963}$Ni$_{0.037}$)$_2$As$_2$ manifest a neutron spin resonance in the superconducting state with anisotropic dispersion within the Fe layer. Whereas the resonance is sharply peaked at Q$_{AFM}$ along the orthorhombic a axis, the resonance disperses upwards away from Q$_{AFM}$ along the b axis. In contrast to the downward dispersing resonance and hour-glass shape of the spin excitations in superconducting cuprates, the resonance in electron-doped BaFe$_2$As$_2$ compounds possesses a magnon-like upwards dispersion.
We study systematically transport, susceptibility and heat capacity for BaFe$_{2-x}$Co$_x$As$_2$ single crystals. In the underdoped region, spin density wave (SDW) transition is observed in both resistivity and susceptibility. The magnetic susceptibility shows unusual T-linear dependence above SDW transition up to 700 K. With Co doping, SDW ordering is gradually suppressed and superconductivity emerges with a dome-like shape. Electrical transport, specific heat and magnetic susceptibility indicate that SDW and superconductivity coexist in the sample BaFe$_{2-x}$Co$_x$As$_2$ around x = 0.17, being similar with (Ba,K)Fe$_2$As$_2$. When x$>$0.34, the superconductivity completely disappears. A crossover from non-Fermi-liquid state to Fermi-liquid state is observed with increasing Co doping. A detailed electronic phase diagram about evolution from SDW to superconducting state is given.
We use neutron diffraction and muon spin relaxation to study the effect of in-plane uniaxial pressure on the antiferromagnetic (AF) orthorhombic phase in BaFe$_2$As$_2$ and its Co- and Ni-substituted members near optimal superconductivity. In the low temperature AF ordered state, uniaxial pressure necessary to detwin the orthorhombic crystals also increases the magnetic ordered moment, reaching an 11$%$ increase under 40 MPa for BaFe$_{1.9}$Co$_{0.1}$As$_2$, and a 15$%$ increase for BaFe$_{1.915}$Ni$_{0.085}$As$_2$. We also observe an increase of the AF ordering temperature ($T_N$) of about 0.25 K/MPa in all compounds, consistent with density functional theory calculations that reveal better Fermi surface nesting for itinerant electrons under uniaxial pressure. The doping dependence of the magnetic ordered moment is captured by combining dynamical mean field theory with density functional theory, suggesting that the pressure-induced moment increase near optimal superconductivity is closely related to quantum fluctuations and the nearby electronic nematic phase.
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