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Register a new userPressure induced re-emergence of superconductivity in superconducting topological insulator Sr0.065Bi2Se3
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The recent-discovered Sr$_x$Bi$_2$Se$_3$ superconductor provides an alternative and ideal material base for investigating possible topological superconductivity. Here, we report that in Sr$_{0.065}$Bi$_{2}$Se$_3$, the ambient superconducting phase is gradually depressed upon the application of external pressure. At high pressure, a second superconducting phase emerges at above 6 GPa, with a maximum $T_c$ value of $sim$8.3 K. The joint investigations of the high-pressure synchrotron x-ray diffraction and electrical transport properties reveal that the re-emergence of superconductivity in Sr$_{0.065}$Bi$_{2}$Se$_3$ is closely related to the structural phase transition from ambient rhombohedral phase to high-pressure monoclinic phase around 6 GPa, and further to another high-pressure tetragonal phase above 25 GPa.
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Simultaneous low-temperature electrical resistivity and Hall effect measurements were performed on single-crystalline Bi2Se3 under applied pressures up to 50 GPa. As a function of pressure, superconductivity is observed to onset above 11 GPa with a transition temperature Tc and upper critical field Hc2 that both increase with pressure up to 30 GPa, where they reach maximum values of 7 K and 4 T, respectively. Upon further pressure increase, Tc remains anomalously constant up to the highest achieved pressure. Conversely, the carrier concentration increases continuously with pressure, including a tenfold increase over the pressure range where Tc remains constant. Together with a quasi-linear temperature dependence of Hc2 that exceeds the orbital and Pauli limits, the anomalously stagnant pressure dependence of Tc points to an unconventional pressure-induced pairing state in Bi2Se3 that is unique among the superconducting topological insulators.
Bi2Te3 compound has been theoretically predicted (1) to be a topological insulator, and its topologically non-trivial surface state with a single Dirac cone has been observed in photoemission experiments (2). Here we report that superconductivity (Tc^~3K) can be induced in Bi2Te3 as-grown single crystal (with hole-carriers) via pressure. The first-principles calculations show that the electronic structure under pressure remains to be topologically nontrivial, and the Dirac-type surface states can be well distinguished from bulk states at corresponding Fermi level. The proximity effect between superconducting bulk states and Dirac-type surface state could generate Majorana fermions on the surface. We also discuss the possibility that the bulk state could be a topological superconductor.
Topological superconductivity with Majorana bound states, which are critical to implement nonabelian quantum computation, may be realized in three-dimensional semimetals with nontrivial topological feature, when superconducting transition occurs in the bulk. Here, we report pressure-induced superconductivity in a transition-metal dipnictide NbAs2. The emergence of superconductivity is not accompanied by any structural phase transition up to the maximum experimental pressure of 29.8 GPa, as supported by pressure-dependent synchrotron X-ray diffraction and Raman spectroscopy. Intriguingly, the Raman study reveals rapid phonon mode hardening and broadening above 10 GPa, in coincident with the superconducting transition. Using first principle calculations, we determine Fermi surface change induced by pressure, which steadily increases the density of states without breaking the electron-hole compensation. Noticeably, the main hole pocket of NbAs2 encloses one time-reversal-invariant momenta of the monoclinic lattice, suggesting NbAs2 as a candidate of topological superconductors.
Superconductivity and topological quantum states are two frontier fields of research in modern condensed matter physics. The realization of superconductivity in topological materials is highly desired, however, superconductivity in such materials is typically limited to two- or three-dimensional materials and is far from being thoroughly investigated. In this work, we boost the electronic properties of the quasi-one-dimensional topological insulator bismuth iodide b{eta}-Bi4I4 by applying high pressure. Superconductivity is observed in b{eta}-Bi4I4 for pressures where the temperature dependence of the resistivity changes from a semiconducting-like behavior to that of a normal metal. The superconducting transition temperature Tc increases with applied pressure and reaches a maximum value of 6 K at 23 GPa, followed by a slow decrease. Our theoretical calculations suggest the presence of multiple pressure-induced topological quantum phase transitions as well as a structural-electronic instability.
Topological superconductivity is one of most fascinating properties of topological quantum matters that was theoretically proposed and can support Majorana Fermions at the edge state. Superconductivity was previously realized in a Cu-intercalated Bi2Se3 topological compound or a Bi2Te3 topological compound at high pressure. Here we report the discovery of superconductivity in the topological compound Sb2Te3 when pressure was applied. The crystal structure analysis results reveal that superconductivity at a low-pressure range occurs at the ambient phase. The Hall coefficient measurements indicate the change of p-type carriers at a low-pressure range within the ambient phase, into n-type at higher pressures, showing intimate relation to superconducting transition temperature. The first principle calculations based on experimental measurements of the crystal lattice show that Sb2Te3 retains its Dirac surface states within the low-pressure ambient phase where superconductivity was observed, which indicates a strong relationship between superconductivity and topology nature.
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