Subscribe to the gold package and get unlimited access to Shamra Academy
Register a new userVogel-Fulcher-Tammann Freezing of a Thermally Fluctuating Artificial Spin Ice Probed by X-ray Photon Correlation Spectroscopy
89
0
0.0
(
0
)
Ask ChatGPT about the research
No Arabic abstract
We report on the crossover from the thermal to athermal regime of an artificial spin ice formed from a square array of magnetic islands whose lateral size, 30~nm~$times$~70~nm, is small enough that they are superparamagnetic at room temperature. We used resonant magnetic soft x-ray photon correlation spectroscopy (XPCS) as a method to observe the time-time correlations of the fluctuating magnetic configurations of spin ice during cooling, which are found to slow abruptly as a freezing temperature $T_0 = 178 pm 5$~K is approached. This slowing is well-described by a Vogel-Fulcher-Tammann law, implying that the frozen state is glassy, with the freezing temperature being commensurate with the strength of magnetostatic interaction energies in the array. The activation temperature, $T_mathrm{A} = 40 pm 10$~K, is much less than that expected from a Stoner-Wohlfarth coherent rotation model. Zero-field-cooled/field-cooled magnetometry reveals a freeing up of fluctuations of states within islands above this temperature, caused by variation in the local anisotropy axes at the oxidised edges. This Vogel-Fulcher-Tammann behavior implies that the system enters a glassy state on freezing, which is unexpected for a system with a well-defined ground state.
rate research
Read More
We develop a gauge theory of the critical behavior of the topological excitations-driven Berezinskii-Kosterlitz-Thouless (BKT) phase transition in the XY model with weak quenched disorder. We find that while in two-dimensions the liquid of topological defects exhibits the BKT critical behavior, the three-dimensional system shows more singular Vogel-Fulcher-Tamman criticality heralding its freezing into a spin glass. Our findings provide insights into the topological origin of spin glass formation.
We report an artificial geometrically frustrated magnet based on an array of lithographically fabricated single-domain ferromagnetic islands. The islands are arranged such that the dipole interactions create a two-dimensional analogue to spin ice. Images of the magnetic moments of individual elements in this correlated system allow us to study the local accommodation of frustration. We see both ice-like short-range correlations and an absence of long-range correlations, behaviour which is strikingly similar to the lowtemperature state of spin ice. These results demonstrate that artificial frustrated magnets can provide an uncharted arena in which the physics of frustration can be directly visualized.
We use X-Ray Photon Correlation Spectroscopy to investigate the structural relaxation process in a metallic glass on the atomic length scale. We report evidence for a dynamical crossover between the supercooled liquid phase and the metastable glassy state, suggesting different origins of the relaxation process across the transition. Furthermore, using different cooling rates we observe a complex hierarchy of dynamic processes characterized by distinct aging regimes. Strong analogies with the aging dynamics of soft glassy materials, such as gels and concentrated colloidal suspensions, point at stress relaxation as a universal mechanism driving the relaxation dynamics of out-of-equilibrium systems.
Spin freezing in the $A$-site spinel FeAl$_2$O$_4$ which is a spin liquid candidate is studied using remnant magnetization and nonlinear magnetic susceptibility and isofield cooling and heating protocols. The remnant magnetization behavior of FeAl$_2$O$_4$ differs significantly from that of a canonical spin glass which is also supported by analysis of the nonlinear magnetic susceptibility term $chi_3 (T)$. Through the power-law analysis of $chi_3 (T)$, a spin-freezing temperature, $T_g$ = 11.4$pm$0.9~K and critical exponent, $gamma$ = 1.48$pm$0.59 are obtained. Cole-Cole analysis of magnetic susceptibility shows the presence of broad spin relaxation times in FeAl$_2$O$_4$, however, the irreversible dc susceptibility plot discourages an interpretation based on conventional spin glass features. The magnetization measured using the cooling-and-heating-in-unequal-fields protocol brings more insight to the magnetic nature of this frustrated magnet and reveals unconventional glassy behaviour. Combining our results, we arrive at the conclusion that the present sample of FeAl$_2$O$_4$ consists of a majority spin liquid phase with glassy regions embedded.
Artificial spin ice (ASI) are arrays on nanoscaled magnets that can serve both as models for frustration in atomic spin ice as well as for exploring new spin-wave-based strategies to transmit, process, and store information. Here, we exploit the intricate interplay of the magnetization dynamics of two dissimilar ferromagnetic metals arranged on complimentary lattice sites in a square ASI to effectively modulate the spin-wave properties. We show that the interaction between the two sublattices results in unique spectra attributed to each sublattice and we observe inter- and intra-lattice dynamics facilitated by the distinct magnetization properties of the two materials. The dynamic properties are systematically studied by angular-dependent broadband ferromagnetic resonance and confirmed by micromagnetic simulations. We show that the combination of materials with dissimilar magnetic properties enables the realization of a wide range of two-dimensional structures potentially opening the door to new concepts in nanomagnonics.
Log in to be able to interact and post comments
comments
Fetching comments
Sign in to be able to follow your search criteria
