No Arabic abstract
We present the mass excesses of 59-64Cr, obtained from recent time-of-flight nuclear mass measurements at the National Superconducting Cyclotron Laboratory at Michigan State University. The mass of 64Cr is determined for the first time, with an atomic mass excess of -33.48(44) MeV. We find a significantly different two-neutron separation energy S2n trend for neutron-rich isotopes of chromium, removing the previously observed enhancement in binding at N=38. Additionally, we extend the S2n trend for chromium to N=40, revealing behavior consistent with the previously identified island of inversion in this region. We compare our results to state-of-the-art shell-model calculations performed with a modified Lenzi-Nowacki-Poves-Sieja interaction in the fp shell, including the g9/2 and d5/2 orbits for the neutron valence space. We employ our result for the mass of 64Cr in accreted neutron star crust network calculations and find a reduction in the strength and depth of electron-capture heating from the A=64 isobaric chain, resulting in a cooler than expected accreted neutron star crust. This reduced heating is found to be due to the >1-MeV reduction in binding for 64Cr with respect to values from commonly used global mass models.
The region near Z=28, N=40 is a subject of great interest for nuclear structure studies due to spectroscopic signatures in $^{68}$Ni suggesting a subshell closure at N=40. Trends in nuclear masses and their derivatives provide a complementary approach to shell structure investigations via separation energies. Penning trap mass spectrometry has provided precise measurements for a number of nuclei in this region, however a complete picture of the mass surfaces has so far been limited by the large uncertainty remaining for nuclei with N > 40 along the iron and cobalt chains. Here we present the first Penning trap measurements of $^{68,69}$Co, performed at the Low-Energy Beam and Ion Trap facility at the National Superconducting Cyclotron Laboratory. In addition, we perform ab initio calculations of ground state and two-neutron separation energies of cobalt isotopes with the valence-space in-medium similarity renormalization group approach based on a particular set of two- and three-nucleon forces which predict saturation in infinite matter. We discuss the importance of these measurements and calculations for understanding the evolution of nuclear structure near $^{68}$Ni.
We report on the mass measurements of several neutron-rich $mathrm{Rb}$ and $mathrm{Sr}$ isotopes in the $A approx 100$ region with the TITAN Penning-trap mass spectrometer. Using highly charged ions in the charge state $q=10+$, the masses of $^{98,99}mathrm{Rb}$ and $^{98-100}mathrm{Sr}$ have been determined with a precision of $6 - 12 mathrm{keV}$, making their uncertainty negligible for r-process nucleosynthesis network calculations. The mass of $^{101}mathrm{Sr}$ has been determined directly for the first time with a precision eight times higher than the previous indirect measurement and a deviation of $3sigma$ when compared to the Atomic Mass Evaluation. We also confirm the mass of $^{100}mathrm{Rb}$ from a previous measurement. Furthermore, our data indicates the existance of a low-lying isomer with $80 mathrm{keV}$ excitation energy in $^{98}mathrm{Rb}$. We show that our updated mass values lead to minor changes in the r-process by calculating fractional abundances in the $Aapprox 100$ region of the nuclear chart.
The location of electron capture heat sources in the crust of accreting neutron stars depends on the masses of extremely neutron-rich nuclei. We present first results from a new implementation of the time-of-flight technique to measure nuclear masses of rare isotopes at the National Superconducting Cyclotron Laboratory. The masses of 16 neutron-rich nuclei in the scandium -- nickel range were determined simultaneously, improving the accuracy compared to previous data in 12 cases. The masses of $^{61}${V}, $^{63}${Cr}, $^{66}${Mn}, and $^{74}${Ni} were measured for the first time with mass excesses of $-30.510(890)$ MeV, $-35.280(650)$ MeV, $-36.900(790)$ MeV, and $-49.210(990)$ MeV, respectively. With the measurement of the $^{66}$Mn mass, the locations of the two dominant electron capture heat sources in the outer crust of accreting neutron stars that exhibit superbursts are now experimentally constrained. We find that the location of the $^{66}$Fe$rightarrow^{66}$Mn electron capture transition occurs significantly closer to the surface than previously assumed because our new experimental Q-value is 2.1 MeV (2.6$sigma$) smaller than predicted by the FRDM mass model.
The rare-earth peak in the $r$-process abundance pattern depends sensitively on both the astrophysical conditions and subtle changes in nuclear structure in the region. This work takes an important step elucidating the nuclear structure and reducing the uncertainties in $r$-process calculations via precise atomic mass measurements at the JYFLTRAP double Penning trap. $^{158}$Nd, $^{160}$Pm, $^{162}$Sm, and $^{164-166}$Gd have been measured for the first time and the precisions for $^{156}$Nd, $^{158}$Pm, $^{162,163}$Eu, $^{163}$Gd, and $^{164}$Tb have been improved considerably. Nuclear structure has been probed via two-neutron separation energies $S_{2n}$ and neutron pairing energy metrics $D_n$. The data do not support the existence of a subshell closure at $N=100$. Neutron pairing has been found to be weaker than predicted by theoretical mass models. The impact on the calculated $r$-process abundances has been studied. Substantial changes resulting in a smoother abundance distribution and a better agreement with the solar $r$-process abundances are observed.
We report high-precision mass measurements of $^{50-55}$Sc isotopes performed at the LEBIT facility at NSCL and at the TITAN facility at TRIUMF. Our results provide a substantial reduction of their uncertainties and indicate significant deviations, up to 0.7 MeV, from the previously recommended mass values for $^{53-55}$Sc. The results of this work provide an important update to the description of emerging closed-shell phenomena at neutron numbers $N=32$ and $N=34$ above proton-magic $Z=20$. In particular, they finally enable a complete and precise characterization of the trends in ground state binding energies along the $N=32$ isotone, confirming that the empirical neutron shell gap energies peak at the doubly-magic $^{52}$Ca. Moreover, our data, combined with other recent measurements, does not support the existence of closed neutron shell in $^{55}$Sc at $N=34$. The results were compared to predictions from both emph{ab initio} and phenomenological nuclear theories, which all had success describing $N=32$ neutron shell gap energies but were highly disparate in the description of the $N=34$ isotone.