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Hard crystalline lattice in the Weyl semimetal NbAs

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 Added by Yongkang Luo Dr.
 Publication date 2015
  fields Physics
and research's language is English




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We report the effect of hydrostatic pressure on the magnetotransport properties of the Weyl semimetal NbAs. Subtle changes can be seen in the $rho_{xx}(T)$ profiles with pressure up to 2.31 GPa. The Fermi surfaces undergo an anisotropic evolution under pressure: the extremal areas slightly increase in the $mathbf{k_x}$-$mathbf{k_y}$ plane, but decrease in the $mathbf{k_z}$-$mathbf{k_y}$($mathbf{k_x}$) plane. The topological features of the two pockets observed at atmospheric pressure, however, remain unchanged at 2.31 GPa. No superconductivity can be seen down to 0.3 K for all the pressures measured. By fitting the temperature dependence of specific heat to the Debye model, we obtain a small Sommerfeld coefficient $gamma_0=$ 0.09(1) mJ/(mol$cdot$K$^2$) and a large Debye temperature, $Theta_D=$ 450(9) K, confirming a hard crystalline lattice that is stable under pressure. We also studied the Kadowaki-Woods ratio of this low-carrier-density massless system, $R_{KW}=$ 3.2$times 10^4$ $muOmega$ cm mol$^2$ K$^2$ J$^{-2}$. After accounting for the small carrier density in NbAs, this $R_{KW}$ indicates a suppressed transport scattering rate relative to other metals.



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200 - J. Zhang , F. L. Liu , J. K. Dong 2015
We performed a series of high-pressure synchrotron X-ray diffraction (XRD) and resistance measurements on the Weyl semimetal NbAs. The crystal structure remains stable up to 26 GPa according to the powder XRD data. The resistance of NbAs single crystal increases monotonically with pressure at low temperature. Up to 20 GPa, no superconducting transition is observed down to 0.3 K. These results show that the Weyl semimetal phase is robust in NbAs, and applying pressure is not a good way to get a topological superconductor from a Weyl semimetal.
The non-centrosymmetric Weyl semimetal candidate, MoTe$_2$ was investigated through neutron diffraction and transport measurements at pressures up to 1.5 GPa and at temperatures down to 40 mK. Centrosymmetric and non-centrosymmetric structural phases were found to coexist in the superconducting state. Density Functional Theory (DFT) calculations reveal that the strength of the electron-phonon coupling is similar for both crystal structures. Furthermore, it was found that by controlling non-hydrostatic components of stress, it is possible to mechanically control the ground state crystal structure. This allows for the tuning of crystal symmetry in the superconducting phase from centrosymmetric to non-centrosymmetric. DFT calculations support this strain control of crystal structure. This mechanical control of crystal symmetry gives a route to tuning the band topology of MoTe$_2$ and possibly the topology of the superconducting state.
We apply moderate-high-energy inelastic neutron scattering (INS) measurements to investigate Yb$^{3+}$ crystalline electric field (CEF) levels in the triangular spin-liquid candidate YbMgGaO$_4$. Three CEF excitations from the ground-state Kramers doublet are centered at the energies $hbar omega$ = 39, 61, and 97,meV in agreement with the effective mbox{spin-1/2} $g$-factors and experimental heat capacity, but reveal sizable broadening. We argue that this broadening originates from the site mixing between Mg$^{2+}$ and Ga$^{3+}$ giving rise to a distribution of Yb--O distances and orientations and, thus, of CEF parameters that account for the peculiar energy profile of the CEF excitations. The CEF randomness gives rise to a distribution of the effective spin-1/2 $g$-factors and explains the unprecedented broadening of low-energy magnetic excitations in the fully polarized ferromagnetic phase of YbMgGaO$_4$, although a distribution of magnetic couplings due to the Mg/Ga disorder may be important as well.
The noncentrosymmetric transition metal monopnictides NbP, TaP, NbAs and TaAs are a family of Weyl semimetals in which pairs of protected linear crossings of spin-resolved bands occur. These so-called Weyl nodes are characterized by integer topological charges of opposite sign associated with singular points of Berry curvature in momentum space. In such a system anomalous magnetoelectric responses are predicted, which should only occur if the crossing points are close to the Fermi level and enclosed by Fermi surface pockets penetrated by an integer flux of Berry curvature, dubbed Weyl pockets. TaAs was shown to possess Weyl pockets whereas TaP and NbP have trivial pockets enclosing zero net flux of Berry curvature. Here, via measurements of the magnetic torque, resistivity and magnetisation, we present a comprehensive quantum oscillation study of NbAs, the last member of this family where the precise shape and nature of the Fermi surface pockets is still unknown. We detect six distinct frequency branches, two of which have not been observed before. A comparison to density functional theory calculations suggests that the two largest pockets are topologically trivial, whereas the low frequencies might stem from tiny Weyl pockets. The enclosed Weyl nodes are within a few meV of the Fermi energy.
Motivated by the proposal of a Weyl-semimetal phase in pyrochlore iridates, we consider a Hubbard-type model on the pyrochlore lattice. To shed light on the question as to why such a state has not been observed experimentally, its robustness is analyzed. On the one hand, we study the possible phases when the system is doped. Magnetic frustration favors several phases with magnetic and charge order that do not occur at half filling, including additional Weyl-semimetal states close to quarter filling. On the other hand, we search for density waves that break translational symmetry and destroy the Weyl-semimetal phase close to half filling. The uniform Weyl semimetal is found to be stable, which we attribute to the low density of states close to the Fermi energy.
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