The origin of the ultra-high-energy particles we receive on the Earth from the outer space such as EeV cosmic rays and PeV neutrinos remains an enigma. All mechanisms known to us currently make use of electromagnetic interaction to accelerate charged particles. In this paper we propose a mechanism exclusively based on gravity rather than electromagnetic interaction. We show that it is possible to generate ultra-high-energy particles starting from particles with moderate energies using the collisional Penrose process in an overspinning Kerr spacetime transcending the Kerr bound only by an infinitesimal amount, i.e., with the Kerr parameter $a=M(1+epsilon)$, where we take the limit $epsilon rightarrow 0^+$. We consider two massive particles starting from rest at infinity that collide at $r=M$ with divergent center-of-mass energy and produce two massless particles. We show that massless particles produced in the collision can escape to infinity with the ultra-high energies exploiting the collisional Penrose process with the divergent efficiency $eta sim {1}/{sqrt{epsilon}} rightarrow infty$. Assuming the isotropic emission of massless particles in the center-of-mass frame of the colliding particles, we show that half of the particles created in the collisions escape to infinity with the divergent energies. To a distant observer, ultra-high-energy particles appear to originate from a bright spot which is at the angular location $xi sim {2M}/{r_{obs}}$ with respect to the singularity on the side which is rotating towards the observer. We show that the anisotropy in emission in the center-of-mass frame, which is dictated by the differential cross-section of underlying particle physics process, leaves a district signature on the spectrum of ultra-high-energy massless particles. Thus, it provides a unique probe into fundamental particle physics.