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Inversion symmetry of Josephson current as test of chiral domain wall motion in Sr$_{2}$RuO$_{4}$

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 Added by Kohta Saitoh
 Publication date 2015
  fields Physics
and research's language is English




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Clarifying the chiral domains structure of superconducting Sr$_{2}$RuO$_{4}$ has been a long-standing issue in identifying its peculiar topological superconducting state. We evaluated the critical current $I_{c}$ versus the magnetic field $H$ of Nb/Sr$_{2}$RuO$_{4}$ Josephson junctions, changing the junction dimension in expectation of that the number of domains in the junction is controlled. $I_{c}(H)$ exhibits a recovery from inversion symmetry breaking to invariance when the dimension is reduced to several microns. This inversion invariant behavior indicates the disappearance of domain walls; thus, the size of a single domain is estimated at approximately several microns.

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Sr$_2$RuO$_4$ is the best candidate for spin-triplet superconductivity, an unusual and elusive superconducting state of fundamental importance. In the last three decades Sr$_2$RuO$_4$ has been very carefully studied and despite its apparent simplicity when compared with strongly correlated high-$T_{c}$ cuprates, for which the pairing symmetry is understood, there is no scenario that can explain all the major experimental observations, a conundrum that has generated tremendous interest. Here we present a density-functional based analysis of magnetic interactions in Sr$_{2}$RuO$_{4}$ and discuss the role of magnetic anisotropy in its unconventional superconductivity. Our goal is twofold. First, we access the possibility of the superconducting order parameter rotation in an external magnetic field of 200 Oe, and conclude that the spin-orbit interaction in this material is several orders of magnitude too strong to be consistent with this hypothesis. Thus, the observed invariance of the Knight shift across $T_{c}$ has no plausible explanation, and casts doubt on using the Knight shift as an ultimate litmus paper for the pairing symmetry. Second, we propose a quantitative double-exchange-like model for combining itinerant fermions with an anisotropic Heisenberg magnetic Hamiltonian. This model is complementary to the Hubbard-model-based calculations published so far, and forms an alternative framework for exploring superconducting symmetry in Sr$_{2}$RuO$_{4}.$ As an example, we use this model to analyze the degeneracy between various $p-$triplet states in the simplest mean-field approximation, and show that it splits into a single and two doublets with the ground state defined by the competition between the Ising and compass anisotropic terms.
There is intense controversy around the unconventional superconductivity in strontium ruthenate, where the various theoretical and experimental studies suggest diverse and mutually exclusive pairing symmetries. Currently, the investigation is solely focused on only one material, Sr2RuO4, and the field suffers from the lack of comparison targets. Here, employing a density functional theory based analysis, we show that the heterostructure composed of SrRuO3 and SrTiO3 is endowed with all the key characteristics of Sr2RuO4, and, in principle, can host superconductivity. Furthermore, we show that competing magnetic phases and associated frustration, naturally affecting the superconducting state, can be tuned by epitaxial strain engineering. This system thus offers an excellent platform for gaining more insight into superconductivity in ruthenates.
109 - Tetsuya Takimoto 2002
The mechanism of superconductivity in ${rm Sr}_{2}{rm RuO}_{4}$ is studied using a degenerate Hubbard model within the weak coupling theory. When the system approaches the orbital instability which is realized due to increasing the on-site Coulomb interaction between the electrons in the different orbitals, it is shown that the triplet superconductivity appears. This superconducting mechanism is only available in orbitally degenerate systems with multiple Fermi surfaces.
Sr$_{2}$RuO$_{4}$ is one of the most promising candidates of a topological superconductor with broken time-reversal symmetry, because a number of experiments have revealed evidences for a spin-triplet chiral $p$-wave superconductivity. In order to clarify the time-reversal symmetry of Sr$_{2}$RuO$_{4}$, we introduce a novel test that examines the invariance of the Josephson critical current under the inversion of both the current and magnetic fields, in contrast to the detection of a spontaneous magnetic field employed in past experiments. Analyses of the transport properties of the planar and corner Josephson junctions formed between Sr$_{2}$RuO$_{4}$ and Nb reveal the time-reversal invariant superconductivity, most probably helical $p$-wave, of Sr$_{2}$RuO$_{4}$. This state corresponds to a yet-to-be confirmed $topological crystalline superconductivity$ that can host two Majorana edge modes at the surface protected by crystalline mirror symmetry.
Sr$_{2}$RuO$_{4}$ (SRO) is the prime candidate for chiral $p$-wave superconductor with critical temperature $T_{c}(SRO)sim$1.5 K. Chiral domains with opposite chiralities $p_{x}pm ip_{y}$ were proposed, but yet to be confirmed. We measure the field dependence of the point contact (PC) resistance between a tungsten tip and the SRO-Ru eutectic crystal, where micrometer-sized Ru inclusions are embedded in SRO with atomic sharp interface. Ruthenium is an $s$-wave superconductor with $T_{c}(Ru)sim$0.5 K, flux pinned near the Ru inclusions can suppress its superconductivity as reflected from the PC resistance and spectra. This flux pinning effect is originated from SRO textit{underneath} the surface and is very strong. To fully remove it, one has to thermal cycle the sample above $T_{c}(SRO)$. This resembles the thermal demagnetization for a ferromagnet, where ferromagnetic domains are randomized above its Curie temperature. Another way is by applying alternating fields with decreasing amplitude, resembling field demagnetization for the ferromagnet. The observed hysteresis in magnetoresistance can be explained by domain dynamics, providing support for the existence of chiral domains. The origin of strong pinning textit{underneath} the surface is also discussed.
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