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In high-superconducting transition temperature ($T_{rm c}$) iron-based superconductors, interband sign reversal ($s_{rm pm}$) and sign preserving ($s_{rm ++}$) $s$-wave superconducting states have been primarily discussed as the plausible superconducting mechanism. We study Co impurity scattering effects on the superconductivity in order to achieve an important clue on the pairing mechanism using single crystal Fe$_{1-x}$Co$_x$Se and depict a phase diagram of a FeSe system. Both superconductivity and structural transition / orbital order are suppressed by the Co replacement on the Fe sites and disappear above $x$ = 0.036. These correlated suppressions represent a common background physics behind these physical phenomena in the multiband Fermi surfaces of FeSe. By comparing experimental data and theories so far proposed, the suppression of $T_{rm c}$ against the residual resistivity is shown to be much weaker than that predicted in the case of a general sign reversal and a full gap $s_{pm}$ models. The origin of the superconducting paring in FeSe is discussed in terms of its multiband electronic structure.
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The importance of the spin-orbit coupling (SOC) effect in Fe-based superconductors (FeSCs) has recently been under hot debate. Considering the Hunds coupling-induced electronic correlation, the understanding of the role of SOC in FeSCs is not trivial and is still elusive. Here, through a comprehensive study of 77Se and 57Fe nuclear magnetic resonance, a nontrivial SOC effect is revealed in the nematic state of FeSe. First, the orbital-dependent spin susceptibility, determined by the anisotropy of the 57Fe Knight shift, indicates a predominant role from the 3dxy orbital, which suggests the coexistence of local and itinerant spin degrees of freedom (d.o.f.) in the FeSe. Then, we reconfirm that the orbital reconstruction below the nematic transition temperature (Tnem ~ 90 K) happens not only on the 3dxz and 3dyz orbitals but also on the 3dxy orbital, which is beyond a trivial ferro-orbital order picture. Moreover, our results also indicate the development of a coherent coupling between the local and itinerant spin d.o.f. below Tnem, which is ascribed to a Hunds coupling-induced electronic crossover on the 3dxy orbital. Finally, due to a nontrivial SOC effect, sizable in-plane anisotropy of the spin susceptibility emerges in the nematic state, suggesting a spin-orbital-intertwined nematicity rather than simply spin- or orbital-driven nematicity}. The present work not only reveals a nontrivial SOC effect in the nematic state but also sheds light on the mechanism of nematic transition in FeSe.
Effects of disorder on electron-doped iron pnictides are investigated systematically based on self-consistent Bogoliubov-de Gennes equations. Multiply impurities with same scattering potential (SP) are randomly distributed in a square lattice. Probability distribution functions of normalized order parameters for different impurity concentrations $delta_{imp}$, different electron doping concentrations $delta$ are investigated for given SPs. Samples are found to be very robust against weak SP, in which order parameters do not have qualitative change even at very large $delta_{imp}$. While strong SP is able to easily break down the order parameters. For moderate SP, variations of order parameters on and around impurities strongly depend on $delta$, however the distribution functions of normalized order parameters have similar behavior as $delta_{imp}$ increases. Compared with superconducting (SC) order, the magnetic order is more sensitive to multi-impurity effect. The spatial spin density wave pattern has already been destroyed before the system loses its superconductivity. Dependence of SC order on temperature is similar to that of impurity-free case, with the critical temperature being remarkably suppressed for high $delta_{imp}$.
Single-layer FeSe films grown on the SrTiO3 substrate (FeSe/STO) have attracted much attention because of their possible record-high superconducting critical temperature Tc and distinct electronic structures in iron-based superconductors. However, it has been under debate on how high its Tc can really reach due to the inconsistency of the results obtained from the transport, magnetic and spectroscopic measurements. Here we report spectroscopic evidence of superconductivity pairing at 83 K in single-layer FeSe/STO films. By preparing high-quality single-layer FeSe/STO films, we observe for the first time strong superconductivity-induced Bogoliubov back-bending bands that extend to rather high binding energy ~100 meV by high-resolution angle-resolved photoemission measurements. The Bogoliubov back-bending band provides a new definitive benchmark of superconductivity pairing that is directly observed up to 83 K in the single-layer FeSe/STO films. Moreover, we find that the superconductivity pairing state can be further divided into two temperature regions of 64-83 K and below 64 K. We propose the 64-83 K region may be attributed to superconductivity fluctuation while the region below 64 K corresponds to the realization of long-range superconducting phase coherence. These results indicate that either Tc as high as 83 K is achievable in iron-based superconductors, or there is a pseudogap formation from superconductivity fluctuation in single-layer FeSe/STO films.
We report theoretical and experimental studies of the effect of Zn-impurity in Fe-based superconductors. Zn-impurity is expected to severely suppress sign reversed s$_pm$ wave pairing. The experimentally observed suppression of T$_c$ under Zn-doping strongly depends on the materials and the charge carrier contents, which suggests competition of $s_{++}$ and $s_{pm}$ pairings in Fe-base superconductors. We study a model incorporating both $s_{++}$ and $s_{pm}$ pairing couplings by using Bogoliubov de-Gennes equation, and show that the Zn-impurity strongly suppresses $s_{pm}$ pairing and may induce a transition from $s_{pm}$ to $s_{++}$-wave. Our theory is consistent with various experiments on the impurity effect. We present new experimental data on the Zn-doping SmFe$_{1-x}$Zn$_x$AsO$_{0.9}$F$_{0.1}$ of T$_c=$ 50K, in further support of our proposal.
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