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Register a new userBroadband perfect light trapping in the thinnest monolayer graphene-MoS$_{2}$ photovoltaic cell
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The light absorption of a monolayer graphene-molybdenum disulfide photovoltaic (GM-PV) cell in a wedge-shaped microcavity with a spectrum-splitting structure is investigated theoretically. The GM-PV cell, which is three times thinner than the traditional photovoltaic cell, exhibits up to 98% light absorptivity in a wide wavelength range. This rate exceeds the fundamental limit of nanophotonic light trapping in solar cells. The effects of defect layer thickness, GM-PV cell position in the microcavity, incident angle, and lens aberration on the light absorption rate of the GM-PV cell is explored. Regardless of errors, the GM-PV cell can still achieve at least 90% light absorptivity with the current technology. Our proposal provides different methods to design light-trapping structures and apply spectrum-splitting systems.
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Coherent perfect absorption (CPA) refers to interferometrically induced complete absorption of incident light by a partial absorber independently of its intrinsic absorption (which may be vanishingly small) or its thickness. CPA is typically realized in a resonant device, and thus cannot be achieved over a broad continuous spectrum, which thwarts its applicability to photodetectors and solar cells, for example. Here, we demonstrate broadband omni-resonant CPA by placing a thin weak absorber in a planar cavity and pre-conditioning the incident optical field by introducing judicious angular dispersion. We make use of monolayer graphene embedded in silica as the absorber and boost its optical absorption from ~1.6% to ~60% over a bandwidth of ~70 nm in the visible. Crucially, an analytical model demonstrates that placement of the graphene monolayer at a peak in the cavity standing-wave field is not necessary to achieve CPA, contrary to conventional wisdom.
Coherent perfect absorber (CPA) was proposed as the time-reversed counterpart to laser: a resonator containing lossy medium instead of gain medium can absorb the coherent optical fields completely. Here, we exploit a monolayer graphene to realize the CPA in a non-resonant manner. It is found that quasi-CPA point exists in the terahertz regime for suspending monolayer graphene, and the CPA can be implemented with the assistant of proper phase modulation among two incident beams at the quasi-CPA frequencies. The graphene based CPA is found of broadband angular selectivity: CPA point splits into two frequency bands for the orthogonal $s$ and $p$ polarizations at oblique incidence, and the two bands cover a wide frequency range starting from zero frequency. Furthermore, the coherent absorption can be tuned substantially by varying the gate-controlled Fermi energy. The findings of CPA with non-resonant graphene sheet can be generalized for potential applications in terahertz/infrared detections and signal processing with two-dimensional optoelectronic materials.
Chaos is a phenomenon that occurs in many aspects of contemporary science. In classical dynamics, chaos is defined as a hypersensitivity to initial conditions. The presence of chaos is often unwanted, as it introduces unpredictability, which makes it difficult to predict or explain experimental results. Conversely, we demonstrate here how chaos can be used to enhance the ability of an optical resonator to store energy. We combine analytic theory with ab-initio simulations and experiments in photonic crystal resonators to show that a chaotic resonator can store six times more energy than its classical counterpart of the same volume. We explain the observed increase with the equipartition of energy among all degrees of freedom of the chaotic resonator, i.e. the cavity modes, which is evident from the convergence of their lifetime towards a single value. A compelling illustration of the theory is provided by demonstrating enhanced absorption in deformed polystyrene microspheres.
Graphene is an ideal material for integrated nonlinear optics thanks to its strong light-matter interaction and large nonlinear optical susceptibility. Graphene has been used in optical modulators, saturable absorbers, nonlinear frequency converters, and broadband light emitters. For the latter application, a key requirement is the ability to control and engineer the emission wavelength and bandwidth, as well as the electronic temperature of graphene. Here, we demonstrate that the emission wavelength of graphene$$ s broadband hot carrier photoluminescence can be tuned by integration on photonic cavities, while thermal management can be achieved by out-of-plane heat transfer to hexagonal boron nitride. Our results pave the way to graphene-based ultrafast broadband light emitters with tunable emission.
Plasmonics can be used to improve absorption in optoelectronic devices and has been intensively studied for solar cells and photodetectors. Graphene has recently emerged as a powerful plasmonic material. It shows significantly less losses compared to traditional plasmonic materials such as gold and silver and its plasmons can be tuned by changing the Fermi energy with chemical or electrical doping. Here we propose the usage of graphene plasmonics for light trapping in optoelectronic devices and show that the excitation of localized plasmons in doped, nanostructured graphene can enhance optical absorption in its surrounding media including both bulky and two-dimensional materials by tens of times, which may lead to a new generation of highly efficient, spectrally selective photodetectors in mid-infrared and THz ranges. The proposed concept could even revolutionize the field of plasmonic solar cells if graphene plasmons in the visible and near-infrared are realized.
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