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Register a new userQuasi one-Dimensional Band Dispersion and Metallization In long Range Ordered Polymeric wires
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Added by
Yannick Fagot-Revurat
Publication date
2015
fields
Physics
and research's language is
English
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We study the electronic structure of an ordered array of poly(para-phenylene) chains produced by surface-catalyzed dehalogenative polymerization of 1,4-dibromobenzene on copper (110). The quantization of unoccupied molecular states is measured as a function of oligomer length by scanning tunneling spectroscopy, with Fermi level crossings observed for chains longer than ten phenyl rings. Angle-resolved photoelectron spectroscopy reveals a graphene-like quasi one-dimensional valence band as well as a direct gap of 1.15 eV, as the conduction band is partially filled through adsorption on the surface. Tight-binding modelling and ab initio density functional theory calculations lead to a full description of the organic band-structure, including the k dispersion, the gap size and electron charge transfer mechanisms which drive the system into metallic behaviour. Therefore the entire band structure of a carbon-based conducting wire has been fully determined. This may be taken as a fingerprint of {pi}-conjugation of surface organic frameworks.
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We study the weak antilocalization (WAL) effect in the magnetoresistance of narrow HgTe wires fabricated in quantum wells (QWs) with normal and inverted band ordering. Measurements at different gate voltages indicate that the WAL is only weakly affected by Rashba spin-orbit splitting and persists when the Rashba splitting is about zero. The WAL signal in wires with normal band ordering is an order of magnitude smaller than for inverted ones. These observations are attributed to a Dirac-like topology of the energy bands in HgTe QWs. From the magnetic-field and temperature dependencies we extract the dephasing lengths and band Berry phases. The weaker WAL for samples with a normal band structure can be explained by a non-universal Berry phase which always exceeds pi, the characteristic value for gapless Dirac fermions.
The excitation gap above the Majorana fermion (MF) modes at the ends of 1D topological superconducting (TS) semiconductor wires scales with the bulk quasiparticle gap E_{qp}. This gap, also called minigap, facilitates experimental detection of the pristine TS state and MFs at experimentally accessible temperatures T << E_{qp}. Here we show that the linear scaling of minigap with E_{qp} can fail in quasi-1D wires with multiple confinement bands when the applied Zeeman field is greater than or equal to about half of the confinement-induced bandgap. TS states in such wires have an approximate chiral symmetry supporting multiple near zero energy modes at each end leading to a minigap which can effectively vanish. We show that the problem of small minigap in such wires can be resolved by forcing the system to break the approximate chirality symmetry externally with a second Zeeman field. Although experimental signatures such as zero bias peak from the wire ends is suppressed by the second Zeeman field above a critical value, such a field is required in some important parameter regimes of quasi-1D wires to isolate the topological physics of end state MFs. We also discuss the crucial difference of our minigap calculations from the previously reported minigap results appropriate for idealized spinless p-wave superconductors and explain why the clustering of fermionic subgap states around the zero energy Majorana end state with increasing chemical potential seen in the latter system does not apply to the experimental TS states in spin-orbit coupled nanowires.
A time-reversal invariant topological superconductivity is suggested to be realized in a quasi-one dimensional structure on a plane, which is fabricated by filling the superconducting materials into the periodic channel of dielectric matrices like zeolite and asbestos under high pressure. The topological superconducting phase sets up in the presence of large spin-orbit interactions when intra-wire s-wave and inter-wire d-wave pairings take place. Kramers pairs of Majorana bound states emerge at the edges of each wire. We analyze effects of Zeeman magnetic field on Majorana zero-energy states. In-plane magnetic field was shown to make asymmetric the energy dispersion, nevertheless Majorana fermions survive due to protection of a particle-hole symmetry. Tunneling of Majorana quasi-particle from the end of one wire to the nearest-neighboring one yields edge fractional Josephson current with $4pi$-periodicity.
We calculate the plasmon dispersion in quasi-one-dimensional quantum wires, in the presence of non-magnetic impurities, taking into consideration the memory function formalism and the role of the forward scattering. The plasma frequency is reduced by the presence of impurities. We also calculate, analytically, the plasmon dispersion in the Born approximation, for the scattering of the electrons by the non-magnetic impurities. We compare our result with the numerical results of Sarma and Hwang.
Electron interactions in and between wires become increasingly complex and important as circuits are scaled to nanometre sizes, or employ reduced-dimensional conductors like carbon nanotubes, nanowires and gated high mobility 2D electron systems. This is because the screening of the long-range Coulomb potential of individual carriers is weakened in these systems, which can lead to phenomenon such as Coulomb drag: a current in one wire induces a voltage in a second wire through Coulomb interactions alone. Previous experiments have observed electron drag in wires separated by a soft electrostatic barrier $gtrsim$ 80 nm. Here, we measure both positive and negative drag between adjacent vertical quantum wires that are separated by $sim$ 15 nm and have independent contacts, which allows their electron densities to be tuned independently. We map out the drag signal versus the number of electron subbands occupied in each wire, and interpret the results in terms of momentum-transfer and charge-fluctuation induced transport models. For wires of significantly different subband occupancies, the positive drag effect can be as large as 25%.
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