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Register a new userDynamics of Fractionalization in Quantum Spin Liquids
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We present the theory of dynamical spin-response for the Kitaev honeycomb model, obtaining exact results for the structure factor (SF) in gapped and gapless, Abelian and non-Abelian quantum spin-liquid (QSL) phases. We also describe the advances in methodology necessary to compute these results. The structure factor shows signatures of spin-fractionalization into emergent quasiparticles -- Majorana fermions and fluxes of $Z_2$ gauge field. In addition to a broad continuum from spin-fractionalization, we find sharp ($delta$-function) features in the response. These arise in two distinct ways: from excited states containing only (static) fluxes and no (mobile) fermions; and from excited states in which fermions are bound to fluxes. The SF is markedly different in Abelian and non-Abelian QSLs, and bound fermion-flux composites appear only in the non-Abelian phase.
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Based on large-scale quantum Monte Carlo simulations, we examine the dynamical spin structure factor of the Balents-Fisher-Girvin kagome lattice quantum spin-$1/2$ model, which is known to harbor an extended $Z_2$ quantum spin liquid phase. We use a correlation-matrix sampling scheme combined with a stochastic analytic continuation method to resolve the spectral functions of this anisotropic quantum spin model with a three-site unit-cell. Based on this approach, we monitor the spin dynamics throughout the phase diagram of this model, from the XY-ferromagnetic region to the $Z_2$ quantum spin liquid regime. In the latter phase, we identify a gapped two-spinon continuum in the transverse scattering channel, which is faithfully modeled by an effective spinon tight-binding model. Within the longitudinal channel, we identify gapped vison excitations and exhibit indications for the translational symmetry fractionalization of the visons via an enhanced spectral periodicity.
Quantum spin liquids (QSLs) are intriguing phases of matter possessing fractionalized excitations. Several quasi-two dimensional materials have been proposed as candidate QSLs, but direct evidence for fractionalization in these systems is still lacking. In this paper, we show that the inter-plane thermal conductivity in layered QSLs carries a unique signature of fractionalization. We examine several types of gapless QSL phases - a $Z_2$ QSL with either a Dirac spectrum or a spinon Fermi surface, and a $U(1)$ QSL with a Fermi surface. In all cases, the in-plane and $c-$axis thermal conductivities have a different power law dependence on temperature, due to the different mechanisms of transport in the two directions: in the planes, the thermal current is carried by fractionalized excitations, whereas the inter-plane current is carried by integer (non-fractional) excitations. In layered $Z_2$ and $U(1)$ QSLs with a Fermi surface, the $c-$axis thermal conductivity is parametrically smaller than the in-plane one, but parametrically larger than the phonon contribution at low temperatures.
Spin liquids are quantum phases of matter that exhibit a variety of novel features associated with their topological character. These include various forms of fractionalization - elementary excitations that behave as fractions of an electron. While there is not yet entirely convincing experimental evidence that any particular material has a spin liquid ground state, in the past few years, increasing evidence has accumulated for a number of materials suggesting that they have characteristics strongly reminiscent of those expected for a quantum spin liquid.
Quantum spin liquids attract great interest due to their exceptional magnetic properties characterized by the absence of long-range order down to low temperatures despite the strong magnetic interaction. Commonly, these compounds are strongly correlated electron systems, and their electrodynamic response is governed by the Mott gap in the excitation spectrum. Here we summarize and discuss the optical properties of several two-dimensional quantum spin liquid candidates. First we consider the inorganic material Herbertsmithite ZnCu$_3$(OH)$_6$Cl$_2$ and related compounds, which crystallize in a kagome lattice. Then we turn to the organic compounds $beta^{prime}$-EtMe$_3$-Sb-[Pd(dmit)$_2$]$_2$, $kappa$-(BEDT-TTF)$_2$Ag$_2$(CN)$_3$ and $kappa$-(BEDT-TTF)$_2$Cu$_2$(CN)$_3$, where the spins are arranged in an almost perfect triangular lattice, leading to strong frustration. Due to differences in bandwidth, the effective correlation strength varies over a wide range, leading to a rather distinct behavior as far as the electrodynamic properties are concerned. We discuss the spinon contributions to the optical conductivity in comparison to metallic quantum fluctuations in the vicinity of the Mott transition.
We measure by inelastic neutron scattering the spin excitation spectra as a function of applied magnetic field in the quantum spin-ladder material (C5H12N)2CuBr4. Discrete magnon modes at low fields in the quantum disordered phase and at high fields in the saturated phase contrast sharply with a spinon continuum at intermediate fields characteristic of the Luttinger-liquid phase. By tuning the magnetic field, we drive the fractionalization of magnons into spinons and, in this deconfined regime, observe both commensurate and incommensurate continua.
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