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Register a new userOrder-by-disorder near criticality in $XY$ pyrochlore magnets
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We consider a system of spins on the sites of a three-dimensional pyrochlore lattice of corner-sharing tetrahedra interacting with a predominant effective $xy$ exchange. In particular, we investigate the selection of a long-range ordered state with broken discrete symmetry induced by thermal fluctuations near the critical region. At the standard mean-field theory (s-MFT) level, in a region of the parameter space of this Hamiltonian that we refer to as $Gamma_5$ region, the ordered state possesses an accidental $U(1)$ degeneracy. In this paper, we show that fluctuations beyond s-MFT lift this degeneracy by selecting one of two states (so-called $psi_2$ and $psi_3$) from the degenerate manifold, thus exposing a certain form of order-by-disorder (ObD). We analytically explore this selection at the microscopic level and close to criticality by elaborating upon and using an extension of the so-called TAP method, originally developed by Thouless, Anderson and Palmer to study the effect of fluctuations in spin glasses. We also use a single-tetrahedron cluster-mean-field theory (c-MFT) to explore over what minimal length scale fluctuations can lift the degeneracy. We find the phase diagrams obtained by these two methods to be somewhat different since c-MFT only includes the shortest-range fluctuations. General symmetry arguments used to construct a Ginzburg-Landau theory to lowest order in the order parameters predict that a weak magnetic moment, $m_z$, along the local $langle 111 rangle$ (${hat z}$) direction is generically induced for a system ordering into a $psi_2$ state, but not so for $psi_3$ ordering. Both E-TAP and c-MFT calculations confirm this weak fluctuation-induced $m_z$ moment. Using a Ginzburg-Landau theory, we discuss the phenomenology of multiple phase transitions below the paramagnetic phase transition and within the $Gamma_5$ long-range ordered phase.
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The recent determination of a robust spin Hamiltonian for the anti-ferromagnetic XY pyrochlore Er2Ti2O7 reveals a most convincing case of the order by quantum disorder (ObQD) mechanism for ground state selection. This mechanism relies on quantum fluctuations to remove an accidental symmetry of the magnetic ground state, and selects a particular ordered spin structure below T_N=1.2K. The removal of the continuous degeneracy results in an energy gap in the spectrum of spin wave excitations, long wavelength pseudo-Goldstone modes. We have measured the ObQD spin wave gap at a zone center in Er2Ti2O7, using low incident energy neutrons and the time-of-flight inelastic scattering method. We report a gap of Delta =0.053 +/- 0.006 meV, which is consistent with upper bounds placed on it from heat capacity measurements and roughly consistent with theoretical estimate of ~ 0.02 meV, further validating the spin Hamiltonian that led to that prediction. The gap is observed to vary with square of the order parameter, and goes to zero for T ~ T_N.
Conclusive evidence of order by disorder is scarce in real materials. Perhaps one of the strongest cases presented has been for the pyrochlore XY antiferromagnet Er2Ti2O7, with the ground state selection proceeding by order by disorder induced through the effects of quantum fluctuations. This identification assumes the smallness of the effect of virtual crystal field fluctuations that could provide an alternative route to picking the ground state. Here we show that this order by virtual crystal field fluctuations is not only significant, but competitive with the effects of quantum fluctuations. Further, we argue that higher-multipolar interactions that are generically present in rare-earth magnets can dramatically enhance this effect. From a simplified bilinear-biquadratic model of these multipolar interactions, we show how the virtual crystal field fluctuations manifest in Er2Ti2O7 using a combination of strong coupling perturbation theory and the random phase approximation. We find that the experimentally observed psi2 state is indeed selected and the experimentally measured excitation gap can be reproduced when the bilinear and biquadratic couplings are comparable while maintaining agreement with the entire experimental spin-wave excitation spectrum. Finally, we comments on possible tests of this scenario and discuss implications for other order-by-disorder candidates in rare-earth magnets.
We study the finite-temperature superfluid transition in a modified two-dimensional (2D) XY model with power-law distributed scratch-like bond disorder. As its exponent decreases, the disorder grows stronger and the mechanism driving the superfluid transition changes from conventional vortex-pair unbinding to a strong randomness criticality (termed scratched-XY criticality) characterized by a non-universal jump of the superfluid stiffness. The existence of the scratched-XY criticality at finite temperature and its description by an asymptotically exact semi-renormalization group theory, previously developed for the superfluid-insulator transition in one-dimensional disordered quantum systems, is numerically proven by designing a model with minimal finite size effects. Possible experimental implementations are discussed.
Examples of materials where an order by disorder mechanism is at play to select a particular ground state are scarce. It has recently been proposed, however, that the antiferromagnetic XY pyrochlore Er2Ti2O7, reveals a most convincing case of this mechanism. Observation of a spin gap at zone centers has recently been interpreted as a corroboration of this physics. In this paper, we argue, however, that the anisotropy generated by the interaction-induced admixing between the crystal-field ground and excited levels provides for an alternative mechanism. It especially predicts the opening of a spin gap of about 15 micro-eV, which is of the same order of magnitude as the one observed experimentally. We report new high resolution inelastic neutron scattering data which can be well understood within this scenario.
We develop a gauge theory of the critical behavior of the topological excitations-driven Berezinskii-Kosterlitz-Thouless (BKT) phase transition in the XY model with weak quenched disorder. We find that while in two-dimensions the liquid of topological defects exhibits the BKT critical behavior, the three-dimensional system shows more singular Vogel-Fulcher-Tamman criticality heralding its freezing into a spin glass. Our findings provide insights into the topological origin of spin glass formation.
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