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Register a new userExciting polaritons with quantum light
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We discuss the excitation of polaritons---strongly-coupled states of light and matter---by quantum light, instead of the usual laser or thermal excitation. As one illustration of the new horizons thus opened, we introduce Mollow spectroscopy, a theoretical concept for a spectroscopic technique that consists in scanning the output of resonance fluorescence onto an optical target, from which weak nonlinearities can be read with high precision even in strongly dissipative environments.
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Seeing macroscopic quantum states directly remains an elusive goal. Particles with boson symmetry can condense into such quantum fluids producing rich physical phenomena as well as proven potential for interferometric devices [1-10]. However direct imaging of such quantum states is only fleetingly possible in high-vacuum ultracold atomic condensates, and not in superconductors. Recent condensation of solid state polariton quasiparticles, built from mixing semiconductor excitons with microcavity photons, offers monolithic devices capable of supporting room temperature quantum states [11-14] that exhibit superfluid behaviour [15,16]. Here we use microcavities on a semiconductor chip supporting two-dimensional polariton condensates to directly visualise the formation of a spontaneously oscillating quantum fluid. This system is created on the fly by injecting polaritons at two or more spatially-separated pump spots. Although oscillating at tuneable THz-scale frequencies, a simple optical microscope can be used to directly image their stable archetypal quantum oscillator wavefunctions in real space. The self-repulsion of polaritons provides a solid state quasiparticle that is so nonlinear as to modify its own potential. Interference in time and space reveals the condensate wavepackets arise from non-equilibrium solitons. Control of such polariton condensate wavepackets demonstrates great potential for integrated semiconductor-based condensate devices.
We show that the use of momentum-space optical interferometry, which avoids any spatial overlap between two parts of a macroscopic quantum state, presents a unique way to study coherence phenomena in polariton condensates. In this way, we address the longstanding question in quantum mechanics: emph{Do two components of a condensate, which have never seen each other, possess a definitive phase?} [P. W. Anderson, emph{Basic Notions of Condensed Matter Physics} (Benjamin, 1984)]. A positive answer to this question is experimentally obtained here for light-matter condensates, created under precise symmetry conditions, in semiconductor microcavities taking advantage of the direct relation between the angle of emission and the in-plane momentum of polaritons.
A textbook example of quantum mechanical effects is the coupling of two states through a tunnel barrier. In the case of macroscopic quantum states subject to interactions, the tunnel coupling gives rise to Josephson phenomena including Rabi oscillations, the a.c. and d.c. effects, or macroscopic self-trapping depending on whether tunnelling or interactions dominate. Non-linear Josephson physics, observed in superfluid helium and atomic condensates, has remained inaccessible in photonic systems due to the required effective photon-photon interactions. We report on the observation of non-linear Josephson oscillations of two coupled polariton condensates confined in a photonic molecule etched in a semiconductor microcavity. By varying both the distance between the micropillars forming the molecule and the condensate density in each micropillar, we control the ratio of coupling to interaction energy. At low densities we observe coherent oscillations of particles tunnelling between the two micropillars. At high densities, interactions quench the transfer of particles inducing the macroscopic self-trapping of the condensate in one of the micropillars. The finite lifetime of polaritons results in a dynamical transition from self-trapping to oscillations with pi phase. Our results open the way to the experimental study of highly non-linear regimes in photonic systems, such as chaos or symmetry-breaking bifurcations.
The ultra-strong light-matter coupling regime has been demonstrated in a novel three-dimensional inductor-capacitor (LC) circuit resonator, embedding a semiconductor two-dimensional electron gas in the capacitive part. The fundamental resonance of the LC circuit interacts with the intersubband plasmon excitation of the electron gas at $omega_c = 3.3$~THz with a normalized coupling strength $2Omega_R/omega_c = 0.27$. Light matter interaction is driven by the quasi-static electric field in the capacitors, and takes place in a highly subwavelength effective volume $V_{mathrm{eff}} = 10^{-6}lambda_0^3$ . This enables the observation of the ultra-strong light-matter coupling with $2.4times10^3$ electrons only. Notably, our fabrication protocol can be applied to the integration of a semiconductor region into arbitrary nano-engineered three dimensional meta-atoms. This circuit architecture can be considered the building block of metamaterials for ultra-low dark current detectors.
We address the system with two species of vector bosons in an optical lattice. In addition to the the standard parameters characterizing such a system, we are dealing here with the degree of atomic nonidentity, manifesting itself in the difference of tunneling amplitudes and on-site Coulomb interactions. We obtain a cascade of quantum phase transitions occurring with the increase in the degree of atomic nonidentity. In particular, we show that the phase diagram for strongly distinct atoms is qualitatively different from that for (nearly) identical atoms considered earlier. The resulting phase diagrams evolve from the images similar to the J. Miro-like paintings to K. Malewicz-like ones.
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