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Dynamical properties of single-file diffusion

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 Added by Tridib Sadhu
 Publication date 2015
  fields Physics
and research's language is English




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We study the statistics of a tagged particle in single-file diffusion, a one-dimensional interacting infinite-particle system in which the order of particles never changes. We compute the two-time correlation function for the displacement of the tagged particle for an arbitrary single-file system. We also discuss single-file analogs of the arcsine law and the law of the iterated logarithm characterizing the behavior of Brownian motion. Using a macroscopic fluctuation theory we devise a formalism giving the cumulant generating functional. In principle, this functional contains the full statistics of the tagged particle trajectory---the full single-time statistics, all multiple-time correlation functions, etc. are merely special cases.



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In this work, we present an effective discrete Edwards-Wilkinson equation aimed to describe the single-file diffusion process. The key physical properties of the system are captured defining an effective elasticity, which is proportional to the single particle diffusion coefficient and to the inverse squared mean separation between particles. The effective equation gives a description of single-file diffusion using the global roughness of the system of particles, which presents three characteristic regimes, namely normal diffusion, subdiffusion and saturation, separated by two crossover times. We show how these regimes scale with the parameters of the original system. Additional repulsive interaction terms are also considered and we analyze how the crossover times depend on the intensity of the additional terms. Finally, we show that the roughness distribution can be well characterized by the Edwards-Wilkinson universal form for the different single-file diffusion processes studied here.
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Active particles may happen to be confined in channels so narrow that they cannot overtake each other (Single File conditions). This interesting situation reveals nontrivial physical features as a consequence of the strong inter-particle correlations developed in collective rearrangements. We consider a minimal model for active Brownian particles with the aim of studying the modifications introduced by activity with respect to the classical (passive) Single File picture. Depending on whether their motion is dominated by translational or rotational diffusion, we find that active Brownian particles in Single File may arrange into clusters which are continuously merging and splitting ({it active clusters}) or merely reproduce passive-motion paradigms, respectively. We show that activity convey to self-propelled particles a strategic advantage for trespassing narrow channels against external biases (e.g., the gravitational field).
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Single-file Brownian motion in periodic structures is an important process in nature and technology, which becomes increasingly amenable for experimental investigation under controlled conditions. To explore and understand generic features of this motion, the Brownian asymmetric simple exclusion process (BASEP) was recently introduced. The BASEP refers to diffusion models, where hard spheres are driven by a constant drag force through a periodic potential. Here, we derive general properties of the rich collective dynamics in the BASEP. Average currents in the steady state change dramatically with the particle size and density. For an open system coupled to particle reservoirs, extremal current principles predict various nonequilibrium phases, which we verify by Brownian dynamics simulations. For general pair interactions we discuss connections to single-file transport by traveling-wave potentials and prove the impossibility of current reversals in systems driven by a constant drag and by traveling waves.
59 - A. Kundu , J. Cividini 2016
We study the effect of a single driven tracer particle in a bath of other particles performing the random average process on an infinite line using a stochastic hydrodynamics approach. We consider arbitrary fixed as well as random initial conditions and compute the two-point correlations. For quenched uniform and annealed steady state initial conditions we show that in the large time $T$ limit the fluctuations and the correlations of the positions of the particles grow subdiffusively as $sqrt{T}$ and have well defined scaling forms under proper rescaling of the labels. We compute the corresponding scaling functions exactly for these specific initial configurations and verify them numerically. We also consider a non translationally invariant initial condition with linearly increasing gaps where we show that the fluctuations and correlations grow superdiffusively as $T^{3/2}$ at large times.
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