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Register a new userProbing the electron-phonon interaction in correlated systems with coherent lattice fluctuation spectroscopy
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Tailoring the properties of correlated oxides is accomplished by chemical doping, pressure, temperature or magnetic field. Photoexcitation is a valid alternative to reach out-of-equilibrium states otherwise inaccessible. Here, we quantitatively estimate the coupling between a lattice distortion and the charge-transfer excitation in (La$_2$CuO$_{4+delta}$). We photoinduce a coherent La ion vibration and monitor the response of the optical constants in a broad energy range, providing quantitative information on the electron-phonon matrix element that can be compared to theoretical models. We propose the same methodology to probe electron-electron interactions in other materials.
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We use a Luttinger-Ward functional approach to study the problem of phonon-mediated superconductivity in electron systems with strong electron-electron interactions (EEIs). Our derivation does not rely on an expansion in skeleton diagrams for the EEI and the resulting theory is therefore nonperturbative in the strength of the latter. We show that one of the building blocks of the theory is the irreducible six-leg vertex related to EEIs. Diagrammatically, this implies five contributions (one of the Fock and four of the Hartree type) to the electronic self-energy, which, to the best of our knowledge, have never been discussed in the literature. Our approach is applicable to (and in fact designed to tackle superconductivity in) strongly correlated electron systems described by generic lattice models, as long as the glue for electron pairing is provided by phonons.
We investigate the interplay of the electron-phonon and the spin fluctuation interaction for the superconducting state of YBa$_2$Cu$_3$O$_{7}$. The spin fluctuations are described within the nearly antiferromagnetic Fermi liquid theory, whereas the phonons are treated using a shell model calculation of all phonon branches. The electron-phonon coupling is calculated using rigidly displaced ionic potentials screened by a background dielectric constant $epsilon_infty$ and by holes within the CuO$_2$ planes. Taking into account both interactions we get a superconducting state with $d_{x^2-y^2}$-symmetry, whose origin are antiferromagnetic spin fluctuations. The investigation of all phonon modes of the system shows that the phononic contribution to the d-wave pairing interaction is attractive. This is a necessary prerequisite for a positive isotope effect. The size of the isotope exponent depends strongly on the relative strength of the electron-phonon and spin fluctuation coupling. Due to the strong electronic correlations no phononic induced superconducting state, which is always of s-wave character, is possible.
We use inelastic neutron scattering to study the evolution of the generalized phonon density of states (GDOS) of the $n$-type high-$T_c$ superconductor Nd$_{2-x}$Ce$_x$CuO$_{4+delta}$ (NCCO), from the half-filled Mott-insulator ($x=0$) to the $T_c=24$ K superconductor ($x=0.15$). Upon doping the CuO$_2$ planes in Nd$_2$CuO$_{4+delta}$ (NCO) with electrons by Ce substitution, the most significant change in the GDOS is the softening of the highest phonon branches associated with the Cu-O bond stretching and out-of-plane oxygen vibration modes. However, the softening occurs within the first few percent of Ce-doping and is not related to the electron doping induced nonsuperconducting-superconducting transition (NST) at $xapprox 0.12$. These results suggest that the electron-lattice coupling in the $n$-type high-$T_c$ superconductors is different from that in the $p$-type materials.
The effect of the resonance of electron scattering energy difference and phonon energy on the electron-phonon-electron interaction (EPEI) is studied. Results show that the resonance of electron transition energy and phonon energy can enhance EPEI by a magnitude of 1 to 2. Moreover, the anisotropic S-wave electron or dx2-y2 electron can enhance resonance EPEI, and the self-energy correction of the electron will weaken resonance EPEI. Particularly, the asymmetrical spin-flip scattering process in k space can reduce the effect of electronic self-energy to enhance resonance EPEI
We present an extension of the tunneling theory for scanning tunneling microcopy (STM) to include different types of vibrational-electronic couplings responsible for inelastic contributions to the tunnel current in the strong-coupling limit. It allows for a better understanding of more complex scanning tunneling spectra of molecules on a metallic substrate in separating elastic and inelastic contributions. The starting point is the exact solution of the spectral functions for the electronic active local orbitals in the absence of the STM tip. This includes electron-phonon coupling in the coupled system comprising the molecule and the substrate to arbitrary order including the anti-adiabatic strong coupling regime as well as the Kondo effect on a free electron spin of the molecule. The tunneling current is derived in second order of the tunneling matrix element which is expanded in powers of the relevant vibrational displacements. We use the results of an ab-initio calculation for the single-particle electronic properties as an adapted material-specific input for a numerical renormalization group approach for accurately determining the electronic properties of a NTCDA molecule on Ag(111) as a challenging sample system for our theory. Our analysis shows that the mismatch between the ab-initio many-body calculation of the tunnel current in the absence of any electron-phonon coupling to the experiment scanning tunneling spectra can be resolved by including two mechanisms: (i) a strong unconventional Holstein term on the local substrate orbital leads to reduction of the Kondo temperature and (ii) a different electron-vibrational coupling to the tunneling matrix element is responsible for inelastic steps in the $dI/dV$ curve at finite frequencies.
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