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Evolution of E2 transition strength in deformed hafnium isotopes from new measurements on $^{172}$Hf, $^{174}$Hf, and $^{176}$Hf

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 Added by Kosuke Nomura
 Publication date 2015
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and research's language is English




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The available data for E2 transition strengths in the region between neutron-deficient Hf and Pt isotopes are far from complete. More and precise data are needed to enhance the picture of structure evolution in this region and to test state-of-the-art nuclear models. In a simple model, the maximum collectivity is expected at the middle of the major shell. However, for actual nuclei, this picture may no longer be the case, and one should use a more realistic nuclear-structure model. We address this point by studying the spectroscopy of Hf. We remeasure the 2^+_1 half-lives of 172,174,176Hf, for which there is some disagreement in the literature. The main goal is to measure, for the first time, the half-lives of higher-lying states of the rotational band. The new results are compared to a theoretical calculation for absolute transition strengths. The half-lives were measured using gamma-gamma and conversion-electron-gamma delayed coincidences with the fast timing method. For the determination of half-lives in the picosecond region, the generalized centroid difference method was applied. For the theoretical calculation of the spectroscopic properties, the interacting boson model is employed, whose Hamiltonian is determined based on microscopic energy-density functional calculations. The measured 2^+_1 half-lives disagree with results from earlier gamma-gamma fast timing measurements, but are in agreement with data from Coulomb excitation experiments and other methods. Half-lives of the 4^+_1 and 6^+_1 states were measured, as well as a lower limit for the 8^+_1 states. We show the importance of the mass-dependence of effective boson charge in the description of E2 transition rates in chains of nuclei. It encourages further studies of the microscopic origin of this mass dependence. New data on transition rates in nuclei from neighboring isotopic chains could support these studies.



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The first ever search for $2varepsilon$ and $varepsilonbeta^+$ decay of $^{174}$Hf was realized using a high-pure sample of hafnium (with mass 179.8 g) and the ultra low-background HPGe-detector system located 225 m underground. After 75 days of data taking no indication of the double beta decay transitions could be detected but lower limits for the half-lives of the different channels and modes of the decays were set on the level of $lim T_{1/2}sim 10^{16}-10^{18}$ a.
This paper reports NMR measurements of the magnetic dipole moments of two high-K isomers, the 37/2$^-$, 51.4 m, 2740 keV state in $^{rm 177}$Hf and the 8$^-$, 5.5 h, 1142 keV state in $^{rm 180}$Hf by the method of on-line nuclear orientation. Also included are results on the angular distributions of gamma transitions in the decay of the $^{rm 177}$Hf isotope. These yield high precision E2/M1 multipole mixing ratios for transitions in bands built on the 23/2$^+$, 1.1 s, isomer at 1315 keV and on the 9/2$^+$, 0.663 ns, isomer at 321 keV. The new results are discussed in the light of the recently reported finding of systematic dependence of the behavior of the g$_{rm R}$ parameter upon the quasi-proton and quasi-neutron make up of high-K isomeric states in this region.
178m2-Hf is an extremely interesting isomeric state due to its potential energy capacity level. One possible way to obtain it is by irradiation of a nat-Ta sample with a high-current proton accelerator. Up to now, there was no information in the international experimental nuclear data base (EXFOR) for this reaction. Irradiations of nat-Ta samples performed for other purposes provide an opportunity to address this question. This paper presents the 172m2-Hf independent production cross-sections determined by gamma-ray spectrometry. The nat-Ta(p,x)172m2-Hf excitation function is studied in the 20-3500 MeV energy range. Comparisons with results by several nuclear models (ISABEL, Bertini, INCL4.5+ABLA07, PHITS, CASCADE07, and CEM03.02) used as event-generators in modern transport codes are also reported. However, since such models are generally not able to separately predict ground and isomeric states of reaction products, only 178-Hf independent and cumulative cross-section data are compared.
The ground-state bands (GSBs) in the even-even hafnium isotopes $^{170-184}$Hf are investigated by using the cranked shell model (CSM) with pairing correlations treated by the particle-number conserving (PNC) method. The experimental kinematic moments of inertia are reproduced very well by theoretical calculations. The second upbending of the GSB at high frequency $hbaromegaapprox0.5$ MeV observed (predicted) in $^{172}$Hf ($^{170,174-178}$Hf) attributes to the sudden alignments of the proton high-$j$ orbitals $pi1i_{13/2}$ $(1/2^{+}[660])$, $pi1h_{9/2}$ $(1/2^{-}[541])$ and orbital $pi1h_{11/2}$ $(7/2^{-}[523])$. The first upbendings of GSBs at low frequency $hbaromega=0.2-0.3$ MeV in $^{170-178}$Hf, which locate below the deformed neutron shell $N=108$, attribute to the alignment of the neutron orbital $ u1i_{13/2}$. For the heavier even-even isotopes $^{180-184}$Hf, compared to the lighter isotopes, the first band-crossing is delayed to the high frequency due to the existence of the deformed shells $N=108,116$. The upbendings of GSBs in $^{180-184}$Hf are predicted to occur at $hbaromegaapprox0.5$MeV, which come from the sharp raise of the simultaneous alignments of both proton $pi1i_{13/2}$, $pi1h_{9/2}$ and neutron $ u2g_{9/2}$ orbitals. The pairing correlation plays a very important role in the rotational properties of GSBs in even-even isotopes $^{180-184}$Hf. Its effects on upbendings and band-crossing frequencies are investigated.
160 - H.L. Liu , F.R. Xu , P.M. Walker 2011
We investigate the influence of deformation on the possible occurrence of long-lived $K$ isomers in Hf isotopes around N=116, using configuration-constrained calculations of potential-energy surfaces. Despite having reduced shape elongation, the multi-quasiparticle states in $^{186,188}$Hf remain moderately robust against triaxial distortion, supporting the long expected occurrence of exceptionally long-lived isomers. The calculations are compared with available experimental data.
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