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Register a new userDoping evolution of antiferromagnetism and transport properties in the non-superconducting BaFe2-2xNixCrxAs2
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We report elastic neutron scattering and transport measurements on the Ni and Cr equivalently doped iron pnictide BaFe$_{2-2x}$Ni$_{x}$Cr$_{x}$As$_{2}$. Compared with the electron-doped BaFe$_{2-x}$Ni$_{x}$As$_{2}$, the long-range antiferromagnetic (AF) order in BaFe$_{2-2x}$Ni$_{x}$Cr$_{x}$As$_{2}$ is gradually suppressed with vanishing ordered moment and N{e}el temperature near $x= 0.20$ without the appearance of superconductivity. A detailed analysis on the transport properties of BaFe$_{2-x}$Ni$_{x}$As and BaFe$_{2-2x}$Ni$_{x}$Cr$_{x}$As$_{2}$ suggests that the non-Fermi-liquid behavior associated with the linear resistivity as a function of temperature may not correspond to the disappearance of the static AF order. From the temperature dependence of the resistivity in overdoped compounds without static AF order, we find that the transport properties are actually affected by Cr impurity scattering, which may induce a metal-to-insulator crossover in highly doped BaFe$_{1.7-y}$Ni$_{0.3}$Cr$_{y}$As$_{2}$.
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We use inelastic neutron scattering to systematically investigate the Ni-doping evolution of the low-energy spin excitations in BaFe2-xNixAs2 spanning from underdoped antiferromagnet to overdoped superconductor (0.03< x < 0.18). In the undoped state, the low-energy (<80 meV) spin waves of BaFe2As2 form transversely elongated ellipses in the [H, K] plane of the reciprocal space. Upon Ni-doping, the c-axis magnetic exchange coupling is rapidly suppressed and the momentum distribution of spin excitations in the [H, K] plane is enlarged in both the transverse and longitudinal directions with respect to the in-plane AF ordering wave vector of the parent compound. As a function of increasing Ni-doping x, the spin excitation widths increase linearly but with a larger rate along the transverse direction. These results are in general agreement with calculations of dynamic susceptibility based on the random phase approximation (RPA) in an itinerant electron picture. For samples near optimal superconductivity at x= 0.1, a neutron spin resonance appears in the superconducting state. Upon further increasing the electron-doping to decrease the superconducting transition temperature Tc, the intensity of the low-energy magnetic scattering decreases and vanishes concurrently with vanishing superconductivity in the overdoped side of the superconducting dome. Comparing with the low-energy spin excitations centered at commensurate AF positions for underdoped and optimally doped materials (x<0.1), spin excitations in the over-doped side (x=0.15) form transversely incommensurate spin excitations, consistent with the RPA calculation. Therefore, the itinerant electron approach provides a reasonable description to the low-energy AF spin excitations in BaFe2-xNixAs2.
The normal-state charge transport is studied systematically in high-quality single crystals of BaFe$_2$(As$_{1-x}$P$_x$)$_2$ ($0 leq x leq 0.71$). By substituting isovalent P for As, the spin-density-wave (SDW) state is suppressed and the dome-shaped superconducting phase ($T_c lesssim 31$ K) appears. Near the SDW end point ($xapprox0.3$), we observe striking linear temperature ($T$) dependence of resistivity in a wide $T$-range, and remarkable low-$T$ enhancement of Hall coefficient magnitude from the carrier number estimates. We also find that the magnetoresistance apparently violates the Kohlers rule and is well scaled by the Hall angle $Theta_H$ as $Deltarho_{xx}/rho_{xx} propto tan^2Theta_H$. These non-Fermi liquid transport anomalies cannot be attributed to the simple multiband effects. These results capture universal features of correlated electron systems in the presence of strong antiferromagnetic fluctuations.
In iron pnictides, high temperature superconductivity emerges after suppressing antiferromagnetism by doping. Here we show that antiferromagnetism in Ca$_{1-x}$La$_x$FeAs$_2$ is robust against and even enhanced by doping. Using $^{75}$As-nuclear magnetic resonance and nuclear quadrupole resonance techniques, we find that an antiferromagnetic order occurs below the Neel temperature $T_{rm N}$ = 62 K at a high doping concentration ($x$ = 0.15) where superconductivity sets in at the transition temperature $T_{rm c}$ = 35 K. Unexpectedly, $T_{rm N}$ is enhanced with increasing doping, rising up to $T_{rm N}$ = 70 K at $x$ = 0.24. The obtained phase diagram of this new system enriches the physics of iron-based high-$T_{rm c}$ superconductors.
Thermal transport in the T -> 0 limit was measured as a function of doping in high-quality single crystals of the cuprate superconductor YBa_2Cu_3O_y. The residual linear term kappa_0/T is found to decrease as one moves from the overdoped regime towards the Mott insulator region of the phase diagram. The doping dependence of the low-energy quasiparticle gap extracted from kappa_0/T is seen to scale closely with that of the pseudogap, arguing against a non-superconducting origin for the pseudogap. The presence of a linear term for all dopings is evidence against the existence of a quantum phase transition to an order parameter with a complex (ix) component.
We generalize the theory of Cooper pairing by spin excitations in the metallic antiferromagnetic state to include situations with electron and/or hole pockets. We show that Cooper pairing arises from transverse spin waves and from gapped longitudinal spin fluctuations of comparable strength. However, each of these interactions, projected on a particular symmetry of the superconducting gap, acts primarily within one type of pocket. We find a nodeless $d_{x^2-y^2}$-wave state is supported primarily by the longitudinal fluctuations on the electron pockets, and both transverse and longitudinal fluctuations support nodeless odd-parity spin singlet $p-$wave symmetry on the hole pockets. Our results may be relevant to the asymmetry of the AF/SC coexistence state in the cuprate phase diagram, as well as for the nodal gap observed recently for strongly underdoped cuprates.
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